Cited by 109Advanced Materials and MechanicsPolymer composites and self-healingShape Memory Alloy Transformations

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Investigation of parameters to achieve temperatures required to initiate the shape-memory effect of magnetic nanocomposites by inductive heating

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Weigel, Th, Mohr, R, Lendlein, A·2009·Smart Materials and Structures

DOI 10.1088/0964-1726/18/2/025011

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Abstract

The activation of the shape-memory effect of nanocomposites (NC) by alternating magnetic fields requires exceeding the switching temperature T s . Different factors, which can influence this process, have been investigated. The intrinsic properties of magnetic nanoparticles (MNP), their content and distribution in the polymer matrix as well as the heat transport conditions, which are essentially determined by the surface to volume ratio (S/V) of the specimens and their surroundings, influence the achievable temperature in an alternating magnetic field. We used MNP having an iron (II, III) oxide core embedded in amorphous silica, which was homogeneously distributed in a polymer matrix by extrusion moulding. The thermoplastic polymer matrix consists either of an aliphatic polyetherurethane (TFX) for demonstration of the basic correlations between magnetic field and the sample, or of a biodegradable multiblock copolymer (PDC), which is prepared from hard segment forming poly(p-dioxanone)diol (PPDO), switching segment forming poly(ε-caprolactone)diol (PCL) and 2,2(4),4-trimethylhexanediisocyanate (TMDI) as a junction unit. We could demonstrate that a nanoparticle content up to 10 wt% does not decisively change the shape-memory properties or mechanical properties of PDC-based materials.

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Authors: Weigel, T., Mohr, R., & Lendlein, A.
Affiliations: Research Institute Bioactive Polymer Systems (DE)
ORCID: Lendlein, A
Venue: Smart Materials and Structures
Publisher: IOP Publishing
Published: 2009-01-13
Volume: 18
Issue: 2
Pages: 025011
ISSN: 0964-1726 (ISSN-L)
1361-665X
DOI: 10.1088/0964-1726/18/2/025011
OpenAlex: W2017243495
Cited by: 109
References: 34
Citations by year: 2026: 2 · 2025: 6 · 2024: 3 · 2022: 2 · 2021: 5 · 2020: 6 · 2019: 5 · 2017: 3 · 2016: 9 · 2015: 5 · 2014: 12 · 2013: 10 · 2012: 11
FWCI: 26.72
Type: journal article
Language: en
Open access: bronze
doi.org
Locations: Smart Materials and Structures (publishedVersion)
Helmholtz-Zentrum Geesthacht Zentrum für Materialforschung und kustenforschung (The Helmholtz Center Geesthacht) (submittedVersion)
Funders: Bundesministerium für Wirtschaft und Technologie
Topics: Physical Sciences › Engineering › Mechanical Engineering › Advanced Materials and Mechanics
Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
Physical Sciences › Materials Science › Materials Chemistry › Shape Memory Alloy Transformations
Keywords: shape memory effect, magnetic nanocomposites, induction heating, alternating magnetic field, switching temperature, iron oxide nanoparticles, silica-coated nanoparticles, heat transport, surface-to-volume ratio, polyether polyurethane, poly(ε-caprolactone) diol, extrusion moulding, nanoparticle content, mechanical properties

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Investigation of parameters to achieve temperatures required to initiate the shape-memory effect of magnetic nanocomposites by inductive heating

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