High-Sensitivity Atomic Magnetometer Unaffected by Spin-Exchange Relaxation
Abstract
Alkali-metal magnetometers compete with SQUID detectors as the most sensitive magnetic field sensors. Their sensitivity is limited by relaxation due to spin-exchange collisions. We demonstrate a K magnetometer in which spin-exchange relaxation is completely eliminated by operating at high K density and low magnetic field. Direct measurements of the signal-to-noise ratio give a magnetometer sensitivity of $10\text{ }\mathrm{f}\mathrm{T}\text{ }\mathrm{H}{\mathrm{z}}^{\mathrm{\ensuremath{-}}\mathrm{1}\mathrm{/}\mathrm{2}}$, limited by magnetic noise produced by Johnson currents in the magnetic shields. We extend a previous theoretical analysis of spin exchange in low magnetic fields to arbitrary spin polarizations and estimate the shot-noise limit of the magnetometer to be $2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}18}\text{ }\mathrm{T}\text{ }\mathrm{H}{\mathrm{z}}^{\mathrm{\ensuremath{-}}\mathrm{1}\mathrm{/}\mathrm{2}}$.
Integrity signals
Registry
Cites
Statistics
Claims the paper makes
Claims other papers make about this one
Each is checked against this paper’s own text: does it say what the citing paper says it does?
OPM-MEG requires a strict zero magnetic field environment to achieve sensitivity to MEG signals.
“However, to achieve sensitivity to the MEG signals, OPM-MEG requires a strict zero magnetic field environment [33].”
From Naturalistic Hyperscanning with Wearable Magnetoencephalography (2023) · cites this paper as [33]
Cites
Spin-exchange optical pumping of noble-gas nuclei
Walker, T. G., & Happer, W. (1997) · Reviews of Modern Physics · doi:10.1103/revmodphys.69.629 · Cited by 1,461 · see citing works
Theory of spin-exchange optical pumping of 3 He and 129 Xe
Appelt, S., Baranga, A. B.-A., Erickson, C., Romalis, M. V., Young, A. R., & Happer, W. (1998) · Physical Review A · doi:10.1103/physreva.58.1412 · Cited by 443 · see citing works
Self-citationSensitive magnetometry based on nonlinear magneto-optical rotation
Budker, D., Kimball, D. F. J., Rochester, S., Yashchuk, V. V., & Zolotorev, M. S. (2000) · Physical Review A · doi:10.1103/physreva.62.043403 · Cited by 335 · see citing works
Spin-Exchange Shift and Narrowing of Magnetic Resonance Lines in Optically Pumped Alkali Vapors
Happer, W., & Tang, H. (1973) · Physical Review Letters · doi:10.1103/physrevlett.31.273 · Cited by 332 · see citing works
Effect of rapid spin exchange on the magnetic-resonance spectrum of alkali vapors
Happer, W., & Tam, A. C. (1977) · Physical Review A · doi:10.1103/physreva.16.1877 · Cited by 291 · see citing works
Nonlinear Magneto-optic Effects with Ultranarrow Widths
Budker, D., Yashchuk, V. V., & Zolotorev, M. S. (1998) · Physical Review Letters · doi:10.1103/physrevlett.81.5788 · Cited by 240 · see citing works
New limits on the electron electric dipole moment from cesium
Murthy, S., Krause, D. E., Li, Z. L., et al. (1989) · Physical Review Letters · doi:10.1103/physrevlett.63.965 · Cited by 223 · see citing works
Application of superconducting quantum interference devices to nuclear magnetic resonance
Greenberg, Y. S. (1998) · Reviews of Modern Physics · doi:10.1103/revmodphys.70.175 · Cited by 217 · see citing works
Magnetic field fluctuations arising from thermal motion of electric charge in conductors
Varpula, T., & Poutanen, T. (1984) · Journal of Applied Physics · doi:10.1063/1.332990 · Cited by 137 · see citing works
Polarization of 3He by Spin Exchange with Optically Pumped Rb and K Vapors
Baranga, A. B.-A., Appelt, S., Romalis, M. V., et al. (1998) · Physical Review Letters · doi:10.1103/physrevlett.80.2801 · Cited by 117 · see citing works
Self-citationLaser optical pumping of high-density Rb in polarized He3 targets
Wagshul, M. E., & Chupp, T. E. (1994) · Physical Review A · doi:10.1103/physreva.49.3854 · Cited by 104 · see citing works
Thermal noise in biomagnetic measurements
Nenonen, J., Montonen, J., & Katila, T. (1996) · Review of Scientific Instruments · doi:10.1063/1.1147514 · Cited by 70 · see citing works
Measurement of Spin-Exchange Cross Sections for Cs133 , Rb87 , Rb85 , K39 , and Na23
Ressler, N., Sands, R. H., & Stark, T. E. (1969) · Physical Review · doi:10.1103/physrev.184.102 · Cited by 69 · see citing works
Foreign-Gas-Induced Cesium Hyperfine Relaxation
Beverini, N., Minguzzi, P., & Strumia, F. (1971) · Physical Review A · doi:10.1103/physreva.4.550 · Cited by 64 · see citing works
Spin Destruction in Collisions between Cesium Atoms
Bhaskar, N. D., Pietras, J., Camparo, J. C., et al. (1980) · Physical Review Letters · doi:10.1103/physrevlett.44.930 · Cited by 56 · see citing works
Measurement of potassium-potassium spin relaxation cross sections
Kadlecek, S. J., Anderson, L. W., & Walker, T. G. (1998) · Nuclear Instruments and Methods in Physics Research Section A Accelerators Spectrometers Detectors and Associated Equipment · doi:10.1016/s0168-9002(97)00836-x · Cited by 26 · see citing works
Electronic spin relaxation of the 4S122 state of K induced by K-He and K-Ne collisions
Franz, F. A., & Volk, C. H. (1982) · Physical Review A · doi:10.1103/physreva.26.85 · Cited by 21 · see citing works
Flagged first, then by citations
Cited by
Sorted by citations
A subfemtotesla multichannel atomic magnetometer
Kominis, I. K., Kornack, T. W., Allred, J. C., & Romalis, M. V. (2003) · Nature · doi:10.1038/nature01484 · Cited by 1,631 · see citing works
Self-citationMoving magnetoencephalography towards real-world applications with a wearable system
Boto, E., Holmes, N., Leggett, J., Roberts, G., Shah, V., Meyer, S. S., Muñoz, L. D., Mullinger, K. J., Tierney, T. M., Bestmann, S., et al. (2018) · Nature · doi:10.1038/nature26147 · Cited by 1,377 · see citing works
Ultrahigh sensitivity magnetic field and magnetization measurements with an atomic magnetometer
Dang, H. B., Maloof, A. C., & Romalis, M. V. (2010) · Applied Physics Letters · doi:10.1063/1.3491215 · Cited by 891 · see citing works
Self-citationOptically pumped magnetometers: from quantum origins to multi-channel magnetoencephalography
Tierney, T. M., Holmes, N., Mellor, S., López, J. D., Roberts, G., Hill, R. M., Boto, E., Leggett, J., Shah, V., Brookes, M. J., et al. (2019) · NeuroImage · doi:10.1016/j.neuroimage.2019.05.063 · Cited by 400 · see citing works
Subfemtotesla Scalar Atomic Magnetometry Using Multipass Cells
Sheng, D., Li, S., Dural, N., & Romalis, M. V. (2013) · Physical Review Letters · doi:10.1103/physrevlett.110.160802 · Cited by 364 · see citing works
Self-citationMeasuring MEG Closer to the Brain: Performance of on-Scalp Sensor Arrays
Iivanainen, J., Stenroos, M., & Parkkonen, L. (2017) · NeuroImage · doi:10.1016/j.neuroimage.2016.12.048 · Cited by 296 · see citing works
“Particularly OPMs operating in the spin-exchange relaxation-free (SERF) regime (Allred et al., 2002) could become a feasible, noncryogenic alternative to SQUIDs for neuromagnetic measurements as the combined dimensions and sensitivies of the SERF-OPMs are approaching those of SQUIDs (∼4–6 cm(2) and ∼3 − 5 fT/ Hz ).”
Unshielded three-axis vector operation of a spin-exchange-relaxation-free atomic magnetometer
Seltzer, S. J., & Romalis, M. V. (2004) · Applied Physics Letters · doi:10.1063/1.1814434 · Cited by 320 · see citing works
Self-citationMulti-Channel Whole-Head OPM-MEG: Helmet Design and a Comparison with a Conventional System
Hill, R. M., Boto, E., Rea, M., Holmes, N., Leggett, J., Coles, L. A., Papastavrou, M., Everton, S. K., Hunt, B. A. E., Sims, D., et al. (2020) · NeuroImage · doi:10.1016/j.neuroimage.2020.116995 · Cited by 285 · see citing works
Recording brain activities in unshielded Earth’s field with optically pumped atomic magnetometers
Zhang, R., Xiao, W., Ding, Y., Feng, Y., Peng, X., Shen, L., Sun, C., Wu, T., Wu, Y., Yang, Y., et al. (2020) · Science Advances · doi:10.1126/sciadv.aba8792 · Cited by 222 · see citing works
On the Potential of a New Generation of Magnetometers for MEG: A Beamformer Simulation Study
Boto, E., Bowtell, R., Krüger, P., Fromhold, T. M., Morris, P. G., Meyer, S. S., Barnes, G. R., & Brookes, M. J. (2016) · PLOS ONE · doi:10.1371/journal.pone.0157655 · Cited by 194 · see citing works
A microfabricated optically-pumped magnetic gradiometer
Sheng, D., Perry, A. R., Krzyzewski, S. P., Geller, S., Kitching, J., & Knappe, S. (2017) · Applied Physics Letters · doi:10.1063/1.4974349 · Cited by 179 · see citing works
A tool for functional brain imaging with lifespan compliance
Hill, R. M., Boto, E., Holmes, N., Hartley, C., Seedat, Z. A., Leggett, J., Roberts, G., Shah, V., Tierney, T. M., Woolrich, M. W., et al. (2019) · Nature Communications · doi:10.1038/s41467-019-12486-x · Cited by 180 · see citing works
Search for topological defect dark matter with a global network of optical magnetometers
Afach, S., Buchler, B. C., Budker, D., Dailey, C., Derevianko, A., Dumont, V., Figueroa, N. L., Gerhardt, I., Grujić, Z. D., Guo, H., et al. (2021) · Nature Physics · doi:10.1038/s41567-021-01393-y · Cited by 126 · see citing works
Self-citationA movable unshielded magnetocardiography system
Xiao, W., Sun, C., Shen, L., Feng, Y., Liu, M., Wu, Y., Liu, X., Wu, T., Peng, X., & Guo, H. (2023) · Science Advances · doi:10.1126/sciadv.adg1746 · Cited by 116 · see citing works
“The OPM used in the MCG system is based on a self-oscillating frequency tracking technique (see details in Materials and Methods), which is different from the conventionally used spin-exchange relaxation-free magne-tometer ( 38 , 39 ).”
A 90-Channel Triaxial Magnetoencephalography System Using Optically Pumped Magnetometers
Rea, M., Boto, E., Holmes, N., Hill, R., Osborne, J., Rhodes, N., Leggett, J., Rier, L., Bowtell, R., Shah, V., et al. (2022) · Annals of the New York Academy of Sciences · doi:10.1111/nyas.14890 · Cited by 102 · see citing works
Characterizing atomic magnetic gradiometers for fetal magnetocardiography
Sulai, I. A., DeLand, Z. J., Bulatowicz, M. D., Wahl, C. P., Wakai, R. T., & Walker, T. G. (2019) · Review of Scientific Instruments · doi:10.1063/1.5091007 · Cited by 79 · see citing works
Naturalistic Hyperscanning with Wearable Magnetoencephalography
Holmes, N., Rea, M., Hill, R. M., Boto, E., Leggett, J., Edwards, L. J., Rhodes, N., Shah, V., Osborne, J., Fromhold, T. M., et al. (2023) · Sensors · doi:10.3390/s23125454 · Cited by 52 · see citing works
“However, to achieve sensitivity to the MEG signal, OPM-MEG requires a strict zero magnetic field environment (Allred et al., 2002).”
BackgroundZhang, R., Mhaskar, R., Smith, K., & Prouty, M. (2020) · Applied Physics Letters · doi:10.1063/5.0004746 · Cited by 48 · see citing works
Perry, A. R., Bulatowicz, M. D., Larsen, M., Walker, T. G., & Wyllie, R. (2020) · Optics Express · doi:10.1364/oe.408486 · Cited by 39 · see citing works
A study of scalar optically-pumped magnetometers for use in magnetoencephalography without shielding
Clancy, R. J., Gerginov, V., Alem, O., Becker, S., & Knappe, S. (2021) · Physics in Medicine & Biology · doi:10.1088/1361-6560/ac18fb · Cited by 37 · see citing works
Four-channel optically pumped magnetometer for a magnetoencephalography sensor array
Iivanainen, J., Carter, T. R., Dhombridge, J. E., Read, T. S., Campbell, K., Abate, Q., Ridley, D. M., Borna, A., & Schwindt, P. D. D. (2024) · Optics Express · doi:10.1364/oe.517961 · Cited by 18 · see citing works
- Authors
- Allred, J. C., Lyman, R. N., Kornack, T. W., & Romalis, M. V.
- Affiliations
- University of Washington (US)
- Princeton University (US)
- ORCID
- Kornack, T. W.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2002-09-09
- Volume
- 89
- Issue
- 13
- Pages
- 130801-130801
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2077767829
- Cited by
- 1,049
- References
- 17
- Citations by year
- 2026: 88 · 2025: 116 · 2024: 111 · 2023: 105 · 2022: 104 · 2021: 82 · 2020: 54 · 2019: 82 · 2018: 44 · 2017: 32 · 2016: 39 · 2015: 28 · 2014: 22 · 2013: 20 · 2012: 25
- FWCI
- 3.56
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Subatomic Physics Research
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Cold Atom Physics and Bose-Einstein Condensates
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Magnetic Field Sensors Techniques
- Keywords
- atomic magnetometer, spin-exchange collisions, magnetic field sensitivity, shot-noise limit, thermal noise, magnetic shielding, weak magnetic field, spin polarization
- MeSH terms
- Magnetics, Models, Theoretical, Potassium
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review