Lorentz Meets Fano in Spectral Line Shapes: A Universal Phase and Its Laser Control
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A Phase for Fano: In spectroscopy, samples placed between a steady light source and a detector are characterized based on the relative intensities of light absorbed at different frequencies. Temporal behavior—the relaxation of a photoexcited state—can be indirectly inferred from the absorption band shapes. The advent of ultrafast laser technology has enabled increasingly sophisticated measurements directly in the time domain. Ott et al. (p. 716 ; see the Perspective by Lin and Chu ) present an analytical framework to account for asymmetric band shapes, termed Fano profiles, on the basis of a phase shift in the temporal dipole response.
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Controlled modification of lineshapes from Lorentz to Fano is found to be a natural result of the phase imparted by the optical pulse.
“Controlled modification of lineshapes from Lorentz to Fano [220] is found to be a natural result of the phase imparted by the optical pulse.”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [220]
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- Authors
- Ott, C., Kaldun, A., Raith, P., Meyer, K., Laux, M., Evers, J., Keitel, C. H., Greene, C. H., & Pfeifer, T.
- Affiliations
- Max Planck Society (DE)
- Purdue University West Lafayette (US)
- Corresponding author
- Pfeifer, Thomas
- ORCID
- Venue
- Science
- Published
- 2013-05-10
- Volume
- 340
- Issue
- 6133
- Pages
- 716-720
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1981611866
- Cited by
- 518
- References
- 30
- Citations by year
- 2026: 21 · 2025: 34 · 2024: 33 · 2023: 28 · 2022: 47 · 2021: 43 · 2020: 42 · 2019: 42 · 2018: 39 · 2017: 47 · 2016: 48 · 2015: 46 · 2014: 33 · 2013: 15
- FWCI
- 24.27
- Type
- journal article
- Language
- en
- Open access
- green
- arxiv.org
- Locations
- Science (publishedVersion)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- MPG.PuRe (Max Planck Society) (submittedVersion, other-oa)
- arXiv (Cornell University)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum optics and atomic interactions
- Keywords
- Fano line shape, Lorentzian line shape, attosecond pulses, extreme ultraviolet spectroscopy, resonant excitation
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