The DOI matches its Crossref record; 8 of the 8 references it cites were found in a registry or an index.
Morphology‐Directed Selective Production of Ethylene or Ethane from CO2 on a Cu Mesopore Electrode
Abstract
The electrocatalytic conversion of CO 2 to value‐added hydrocarbons is receiving significant attention as a promising way to close the broken carbon‐cycle. While most metal catalysts produce C 1 species, such as carbon monoxide and formate, the production of various hydrocarbons and alcohols comprising more than two carbons has been achieved using copper (Cu)‐based catalysts only. Methods for producing specific C 2 reduction outcomes with high selectivity, however, are not available thus far. Herein, the morphological effect of a Cu mesopore electrode on the selective production of C 2 products, ethylene or ethane, is presented. Cu mesopore electrodes with precisely controlled pore widths and depths were prepared by using a thermal deposition process on anodized aluminum oxide. With this simple synthesis method, we demonstrated that C 2 chemical selectivity can be tuned by systematically altering the morphology. Supported by computational simulations, we proved that nanomorphology can change the local pH and, additionally, retention time of key intermediates by confining the chemicals inside the pores.
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Cites
New insights into the electrochemical reduction of carbon dioxide on metallic copper surfaces
Kuhl, K. P., Cave, E. R., Abram, D. N., & Jaramillo, T. F. (2012) · Energy & Environmental Science · doi:10.1039/c2ee21234j · Cited by 3,160
Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
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Highly selective plasma-activated copper catalysts for carbon dioxide reduction to ethylene
Mistry, H., Varela, A. S., Bonifacio, C. S., Zegkinoglou, I., Sinev, I., Choi, Y.-W., Kisslinger, K., Stach, E. A., Yang, J. C., Strasser, P., et al. (2016) · Nature Communications · doi:10.1038/ncomms12123 · Cited by 1,214
Theoretical Considerations on the Electroreduction of CO to C 2 Species on Cu(100) Electrodes
Calle‐Vallejo, F., & Koper, M. T. M. (2013) · Angewandte Chemie International Edition · doi:10.1002/anie.201301470 · Cited by 941
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Active and Selective Conversion of CO 2 to CO on Ultrathin Au Nanowires
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Probing the Active Surface Sites for CO Reduction on Oxide-Derived Copper Electrocatalysts
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Enhanced Electrochemical Methanation of Carbon Dioxide with a Dispersible Nanoscale Copper Catalyst
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Cited by
Progress and perspectives of electrochemical CO2 reduction on copper in aqueous electrolyte
Nitopi, S., Bertheussen, E., Scott, S. B., Liu, X., Engstfeld, A. K., Horch, S., Seger, B., Stephens, I. E. L., Chan, K., Hahn, C., et al. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00705 · Cited by 5,223
Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
Birdja, Y. Y., Pérez-Gallent, E., Figueiredo, M. C., Göttle, A. J., Calle-Vallejo, F., & Koper, M. T. M. (2019) · Nature Energy · doi:10.1038/s41560-019-0450-y · Cited by 2,747
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
CO2 Reduction: From the Electrochemical to Photochemical Approach
Wu, J., Huang, Y., Ye, W., & Li, Y. (2017) · Advanced Science · doi:10.1002/advs.201700194 · Cited by 937
Yang, P.-P., Zhang, X.-L., Gao, F.-Y., Zheng, Y.-R., Niu, Z.-Z., Yu, X., Liu, R., Wu, Z.-Z., Qin, S., Chi, L.-P., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c01699 · Cited by 709
Metadata
- Authors
- Yang, K. D., Ko, W. R., Lee, J. H., Kim, S. J., Lee, H., Lee, M. H., & Nam, K. T.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-12-21
- Volume
- 56
- Issue
- 3
- Pages
- 796-800
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2561747887
- Cited by
- 354
- References
- 8
- FWCI
- 6.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, K. D., Ko, W. R., Lee, J. H., Kim, S. J., Lee, H., Lee, M. H., & Nam, K. T. (2017). Morphology‐Directed Selective Production of Ethylene or Ethane from CO2 on a Cu Mesopore Electrode. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201610432
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