Cited by 138Supercapacitor Materials and FabricationElectrocatalysts for Energy ConversionMXene and MAX Phase Materials

Transforming polystyrene waste into 3D hierarchically porous carbon for high-performance supercapacitors

Ma, Changde, Min, Jiakang, Gong, Jiang, Liu, Xiaoguang, Mu, Xueying, Chen, Xuecheng, Tang, Tao·2020·Chemosphere

Abstract

Polystyrene (PS) is usually discarded as a solid waste after a short lifespan. Thus the disposal of waste PS is an inevitably worldwide issue because of their stable and non-biodegradable nature. Herein, a facile method was proposed to carbonize PS waste into novel three-dimensional (3D) hierarchically porous carbon using Fe 2 O 3 particles as both catalyst and template. Furthermore, KOH activation was applied to generate microporous and mesopores on the wall of macropores. As a result, the obtained 3D hierarchically porous carbon exhibits a high specific capacitance of 284.1 F g-1 at 0.5 A g-1 and good rate performance of 198 F g-1 at 20 A g-1 in a three-electrode device. Moreover, the assembled symmetrical capacitor displays a high energy density of 19.2 W h kg-1 at the power density of 200.7 W kg-1 in aqueous electrolyte. Therefore, the present research develops a sustainable way to recycle waste plastics into 3D hierarchically porous carbon for supercapacitors.

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Crossref · 10.1016/j.chemosphere.2020.126755

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  • Using iron oxide simultaneously as catalyst and template combined with KOH activation converts polystyrene waste into three-dimensional hierarchical porous carbon (3DHPC).

    “For example, Ma and colleagues used iron oxide simultaneously as both catalyst and template, combined with KOH activation, to convert polystyrene waste into three-dimensional hierarchical porous carbon (3DHPC) (Fig. 7a) [71] .”
  • Employing a urea-based nitrogen-doping strategy further enhanced the porosity, yielding a high-performance material (U-3DHPC).

    “Employing a urea-based nitrogen-doping strategy further enhanced the porosity, yielding a high-performance material (U-3DHPC).”

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Authors
Ma, C., Min, J., Gong, J., Liu, X., Mu, X., Chen, X., & Tang, T.
Affiliations
  • University of Science and Technology of China (CN)
  • Chinese Academy of Sciences (CN)
  • Huazhong University of Science and Technology (CN)
  • West Pomeranian University of Technology in Szczecin (PL)
Corresponding author
  • Chen, Xuecheng
  • Tang, Tao
Venue
Chemosphere
Publisher
Elsevier BV
Published
2020-08
Volume
253
Pages
126755
ISSN
0045-6535 (ISSN-L)
OpenAlex
W3016024486
Cited by
138
References
69
Citations by year
2026: 11 · 2025: 26 · 2024: 22 · 2023: 21 · 2022: 28 · 2021: 21 · 2020: 9
FWCI
13.62
Type
journal article
Language
en
Open access
closed
Locations
  • Chemosphere (publishedVersion)
  • PubMed (publishedVersion)
Funders
Narodowe Centrum Nauki
Topics
  • Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
  • Physical Sciences › Materials Science › Materials Chemistry › MXene and MAX Phase Materials
Keywords
polystyrene waste, plastic recycling, hierarchical porous carbon, supercapacitors, KOH activation, specific capacitance, rate capability, energy density, aqueous electrolyte solutions, symmetric supercapacitor
MeSH terms
Carbon, Electrodes, Electrolytes, Plastics, Polystyrenes, Water, Porosity, Electric Capacitance

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