The DOI matches its Crossref record; 28 of the 28 references it cites were found in a registry or an index.
Electrochemical CO2 reduction to C2+ species: Heterogeneous electrocatalysts, reaction pathways, and optimization strategies
Abstract
Abstract Electrochemical CO2 reduction to fuels and chemicals using renewable electricity offers a green and efficient tool/strategy to mitigate global warming and energy supply problems. Relative to C1 products, C2+ hydrocarbons and oxygenates containing two or more carbon atoms have higher energy densities. Also, many multi-carbon products are chemical feedstocks in high demand. However, C C bond formation competes with the H H and C H bond formation. H H and C H bonds have stronger bond energies and thus require lower energies for their formation than C C bonds. Therefore, to increase C2+ fuel selectivity and yield requires the design of advanced tailor-made electrocatalysts and electrolytes as well as optimization of electrochemical cells. An overarching aim of this article is to comprehensively summarize recent advances on the electrocatalytic conversion of CO2 to C2+ hydrocarbons (oxygenates) over various materials. The fundamentals of CO2 catalysis and possible C2+ reaction pathways are provided. We highlight strategies available for improving C2+ compound production.
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Cites
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Cited by
Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
Birdja, Y. Y., Pérez-Gallent, E., Figueiredo, M. C., Göttle, A. J., Calle-Vallejo, F., & Koper, M. T. M. (2019) · Nature Energy · doi:10.1038/s41560-019-0450-y · Cited by 2,747
Defect engineering of two-dimensional materials for advanced energy conversion and storage
Liu, F., & Fan, Z. (2023) · Chemical Society Reviews · doi:10.1039/d2cs00931e · Cited by 417
Design of Local Atomic Environments in Single‐Atom Electrocatalysts for Renewable Energy Conversions
Sun, T., Mitchell, S., Li, J., Lyu, P., Wu, X., Pérez‐Ramírez, J., & Lu, J. (2021) · Advanced Materials · doi:10.1002/adma.202003075 · Cited by 336
Making quantitative sense of electromicrobial production
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Role of oxygen-bound reaction intermediates in selective electrochemical CO 2 reduction
Zhi, X., Vasileff, A., Zheng, Y., Jiao, Y., & Qiao, S.-Z. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00740h · Cited by 149
Metadata
- Authors
- Fan, Q., Zhang, M., Jia, M., Liu, S., Qiu, J., & Sun, Z.
- Venue
- Materials Today Energy
- Publisher
- Elsevier BV
- Published
- 2018-12
- Volume
- 10
- Pages
- 280-301
- ISSN
- 2468-6069 (ISSN-L)
- OpenAlex
- W2898639152
- Cited by
- 269
- References
- 28
- FWCI
- 5.15
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fan, Q., Zhang, M., Jia, M., Liu, S., Qiu, J., & Sun, Z. (2018). Electrochemical CO2 reduction to C2+ species: Heterogeneous electrocatalysts, reaction pathways, and optimization strategies. Materials Today Energy. https://doi.org/10.1016/j.mtener.2018.10.003
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