Simultaneous removal of As, Cd, Cr, Cu, Ni and Zn from stormwater: Experimental comparison of 11 different sorbents
Abstract
The potential of using alumina, activated bauxsol-coated sand (ABCS), bark, bauxsol-coated sand (BCS), fly ash (FA), granulated activated carbon (GAC), granulated ferric hydroxide (GFH), iron oxide-coated sand (IOCS), natural zeolite (NZ), sand, and spinel (MgAl(2)O(4)) as sorbents for removing heavy metals from stormwater are investigated in the present study. The ability of the sorbents to remove a mixture of As, Cd, Cr, Cu, Ni and Zn from synthetic stormwater samples were evaluated in batch tests at a starting pH of 6.5. The metal speciation and saturation data is obtained using the PHREEQ-C geochemical model and used to elucidate the sorption data. It is found that BCS, FA, and spinel have significantly higher affinity towards heavy metals mainly present as cationic or non-charged species (i.e. Cd, Cu, Ni and Zn) compared to those present as anionic species (i.e. As and Cr). However, IOCS, NZ and sand have higher affinity towards As and Cr, while alumina has equally high affinity to all tested heavy metals. The Freundlich isotherm model is found to fit the data in many cases, but ill fitted results are also observed, especially for FA, BCS and GAC, possibly due to leaching of some metals from the sorbents (i.e. for FA) and oversaturated conditions making precipitation the dominant removal mechanism over sorption in batches with high heavy metal concentrations and pH. Calculated sorption constants (i.e. K(d)) are used to compare the overall heavy metal removal efficiency o…
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Carbon-based sorbents are rarely studied to remove both heavy metals and PFAS simultaneously.
“Carbon-based sorbents in particular, including biochar and granular activated carbon (GAC), are commonly used to treat heavy metals or PFAS in stormwater,16–18 but are rarely studied to remove both broad classes of contaminants simultaneously.”
From Evaluation of sorbents and matrix effects for treating heavy metals and per- and polyfluoroalkyl substances as co-contaminants in stormwater (2023) · cites this paper as [18]
Carbon-based sorbents including biochar and GAC are commonly used to treat heavy metals or PFAS in stormwater.
“Carbon-based sorbents in particular, including biochar and granular activated carbon (GAC), are commonly used to treat heavy metals or PFAS in stormwater,16–18 but are rarely studied to remove both broad classes of contaminants simultaneously.”
From Evaluation of sorbents and matrix effects for treating heavy metals and per- and polyfluoroalkyl substances as co-contaminants in stormwater (2023) · cites this paper as [18]
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- Authors
- Genç-Fuhrman, H., Mikkelsen, P. S., & Ledin, A.
- Affiliations
- Technical University of Denmark (DK)
- Corresponding author
- Genç-Fuhrman, Hülya
- ORCID
- Mikkelsen, Peter S.
- Venue
- Water Research
- Publisher
- Elsevier BV
- Published
- 2007-02
- Volume
- 41
- Issue
- 3
- Pages
- 591-602
- ISSN
- 0043-1354 (ISSN-L)
- OpenAlex
- W2036209727
- Cited by
- 238
- References
- 33
- Citations by year
- 2026: 2 · 2025: 1 · 2024: 5 · 2023: 7 · 2022: 8 · 2021: 7 · 2020: 10 · 2019: 10 · 2018: 20 · 2017: 7 · 2016: 16 · 2015: 23 · 2014: 22 · 2013: 17 · 2012: 15
- FWCI
- 14.63
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Water Research (publishedVersion)
- PubMed (publishedVersion)
- Technical University of Denmark, DTU Orbit (Technical University of Denmark, DTU) (submittedVersion)
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Physical Sciences › Environmental Science › Environmental Engineering › Urban Stormwater Management Solutions
- Physical Sciences › Environmental Science › Water Science and Technology › Heavy Metal Pollution Remediation
- Keywords
- stormwater treatment, heavy metal removal, sorbents, arsenic, cadmium, chromium, copper, nickel, zinc, fly ash, granular activated carbon, spinel, natural zeolite, iron oxide-coated sand, alumina, Freundlich isotherm, metal speciation, sorption constants, metal leaching, precipitation chemistry
- MeSH terms
- Adsorption, Cadmium, Chromium, Copper, Hydrogen-Ion Concentration, Nickel, Water Pollutants, Chemical, Zinc, Water Purification, Metals, Heavy
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