The DOI matches its Crossref record; 15 of the 15 references it cites were found in a registry or an index.
Multilayer Electrolyzer Stack Converts Carbon Dioxide to Gas Products at High Pressure with High Efficiency
Open accessAbstract
Abstract Electrochemical reduction of CO2 is a value-added approach to both decrease the atmospheric emission of carbon dioxide and form valuable chemicals. We present a zero gap electrolyzer cell, which continuously converts gas phase CO2 to products without using any liquid catholyte. This is the first report of a multilayer CO2 electrolyzer stack for scaling up the electrolysis process. CO formation with partial current densities above 250 mA cm–2 were achieved routinely, which was further increased to 300 mA cm–2 (with ∼95% faradic efficiency) by pressurizing the CO2 inlet (up to 10 bar). Evenly distributing the CO2 gas among the layers, the electrolyzer operates identically to the sum of multiple single-layer electrolyzer cells. When passing the CO2 gas through the layers consecutively, the CO2 conversion efficiency increased. The electrolyzer simultaneously provides high partial current density, low cell voltage (−3.0 V), high conversion efficiency (up to 40%), and high selectivity for CO production.
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Cites
What would it take for renewably powered electrosynthesis to displace petrochemical processes?
De Luna, P., Hahn, C., Higgins, D., Jaffer, S. A., Jaramillo, T. F., & Sargent, E. H. (2019) · Science · doi:10.1126/science.aav3506 · Cited by 3,052
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
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General Techno-Economic Analysis of CO 2 Electrolysis Systems
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Highly selective plasma-activated copper catalysts for carbon dioxide reduction to ethylene
Mistry, H., Varela, A. S., Bonifacio, C. S., Zegkinoglou, I., Sinev, I., Choi, Y.-W., Kisslinger, K., Stach, E. A., Yang, J. C., Strasser, P., et al. (2016) · Nature Communications · doi:10.1038/ncomms12123 · Cited by 1,214
Technical photosynthesis involving CO2 electrolysis and fermentation
Haas, T., Krause, R., Weber, R., Demler, M., & Schmid, G. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0005-1 · Cited by 649
Verma, S., Lu, X., Ma, S., Masel, R. I., & Kenis, P. J. A. (2016) · Physical Chemistry Chemical Physics · doi:10.1039/c5cp05665a · Cited by 497
One-step electrosynthesis of ethylene and ethanol from CO2 in an alkaline electrolyzer
Ma, S., Sadakiyo, M., Luo, R., Heima, M., Yamauchi, M., & Kenis, P. J. A. (2016) · Journal of Power Sources · doi:10.1016/j.jpowsour.2015.09.124 · Cited by 488
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Microfluidic Reactor for the Electrochemical Reduction of Carbon Dioxide: The Effect of pH
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Electrolysis of CO2 to Syngas in Bipolar Membrane-Based Electrochemical Cells
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Cited by
What would it take for renewably powered electrosynthesis to displace petrochemical processes?
De Luna, P., Hahn, C., Higgins, D., Jaffer, S. A., Jaramillo, T. F., & Sargent, E. H. (2019) · Science · doi:10.1126/science.aav3506 · Cited by 3,052
Yang, K., Kas, R., Smith, W. A., & Burdyny, T. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.0c02184 · Cited by 474
Endrődi, B., Kecsenovity, E., Samu, A., Halmágyi, T., Rojas-Carbonell, S., Wang, L., Yan, Y., & Janáky, C. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02589e · Cited by 303
Self-citation
Metadata
- Authors
- Endrődi, B., Kecsenovity, E., Samu, A., Darvas, F., Jones, R. V., Török, V., Danyi, A., & Janáky, C.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-06-27
- Volume
- 4
- Issue
- 7
- Pages
- 1770-1777
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2954121723
- Cited by
- 359
- References
- 15
- FWCI
- 6.91
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Endrődi, B., Kecsenovity, E., Samu, A., Darvas, F., Jones, R. V., Török, V., Danyi, A., & Janáky, C. (2019). Multilayer Electrolyzer Stack Converts Carbon Dioxide to Gas Products at High Pressure with High Efficiency. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.9b01142
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