Dually actuated triple shape memory polymers of cross-linked polycyclooctene-carbon nanotube/polyethylene nanocomposites
Abstract
In this work, electrically and thermally actuated triple shape memory polymers (SMPs) of chemically cross-linked polycyclooctene (PCO)-multiwalled carbon nanotube (MWCNT)/polyethylene (PE) nanocomposites with co-continuous structure and selective distribution of fillers in PCO phase are prepared. We systematically studied not only the microstructure including morphology and fillers' selective distribution in one phase of the PCO/PE blends, but also the macroscopic properties including thermal, mechanical, and electrical properties. The co-continuous window of the immiscible PCO/PE blends is found to be the volume fraction of PCO (vPCO) of ca. 40-70 vol %. The selective distribution of fillers in one phase of co-continuous blends is obtained by a masterbatch technique. The prepared triple SMP materials show pronounced triple shape memory effects (SMEs) on the dynamic mechanical thermal analysis (DMTA) and the visual observation by both thermal and electric actuations. Such polyolefin samples with well-defined microstructure, electrical actuation, and triple SMEs might have potential applications as, for example, multiple autochoke elements for engines, self-adjusting orthodontic wires, and ophthalmic devices.
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Alternative methods for creating multiple, well-separated switching transitions in one system consist of laminating two SMPs with well-separated transition temperatures or developing hybrid SMPs with multiple thermal transitions.
“Alternative methods for creating multiple, well-separated switching transitions in one system consist of laminating two SMPs which have well-separated transition temperatures [76,77] or of developing hybrid SMPs with multiple thermal transitions [78-81].”
From Two-Way and Multiple-Way Shape Memory Polymers for Soft Robotics: An Overview (2020) · cites this paper as [80]
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- Authors
- Wang, Z., Zhao, J., Chen, M., Yang, M., Tang, L., Dang, Z.-M., Chen, F., Huang, M., & Dong, X.
- Affiliations
- University of Science and Technology Beijing (CN)
- Chinese Academy of Sciences (CN)
- Corresponding author
- Zhao, Jun
- Dang, Zhi-Min
- Dong, Xia
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-11-10
- Volume
- 6
- Issue
- 22
- Pages
- 20051-20059
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2054134514
- Cited by
- 73
- References
- 69
- Citations by year
- 2026: 3 · 2025: 3 · 2024: 5 · 2023: 2 · 2022: 6 · 2021: 5 · 2020: 10 · 2019: 10 · 2018: 2 · 2017: 10 · 2016: 8 · 2015: 8 · 2014: 1
- FWCI
- 9.82
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- ACS Applied Materials & Interfaces (publishedVersion)
- PubMed (publishedVersion)
- Funders
- Ministry of Science and Technology of the People's Republic of China (2014CB239500)
- Beijing National Laboratory for Molecular Sciences
- Topics
- Physical Sciences › Engineering › Mechanical Engineering › Advanced Materials and Mechanics
- Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
- Physical Sciences › Engineering › Biomedical Engineering › Dielectric materials and actuators
- Keywords
- shape memory polymers, multi-walled carbon nanotubes, polyethylene nanocomposites, electrical actuation, thermal actuation, triple shape memory effect
- MeSH terms
- Calorimetry, Differential Scanning, Electricity, Microscopy, Electron, Scanning, Polymers, Surface Properties, Temperature, Polyethylene, Cyclooctanes, Nanotubes, Carbon, Nanocomposites
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