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Nanoporous Graphitic-C3N4@Carbon Metal-Free Electrocatalysts for Highly Efficient Oxygen Reduction
Abstract
Based on theoretical prediction, a g-C(3)N(4)@carbon metal-free oxygen reduction reaction (ORR) electrocatalyst was designed and synthesized by uniform incorporation of g-C(3)N(4) into a mesoporous carbon to enhance the electron transfer efficiency of g-C(3)N(4). The resulting g-C(3)N(4)@carbon composite exhibited competitive catalytic activity (11.3 mA cm(-2) kinetic-limiting current density at -0.6 V) and superior methanol tolerance compared to a commercial Pt/C catalyst. Furthermore, it demonstrated significantly higher catalytic efficiency (nearly 100% of four-electron ORR process selectivity) than a Pt/C catalyst. The proposed synthesis route is facile and low-cost, providing a feasible method for the development of highly efficient electrocatalysts.
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Metadata
- Authors
- Zheng, Y., Jiao, Y., Chen, J., Liu, J., Liang, J., Du, A., Zhang, W., Zhu, Z., Smith, S. C., Jaroniec, M., Lu, G. Q. (., & Qiao, S. Z.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-11-29
- Volume
- 133
- Issue
- 50
- Pages
- 20116-20119
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2090689053
- Cited by
- 1,036
- References
- 3
- FWCI
- 26.40
- Type
- journal article
- Language
- en
- Open access
- closed
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