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Enhanced Photocatalytic CO2-Reduction Activity of Anatase TiO2 by Coexposed {001} and {101} Facets
Abstract
Control of TiO2 crystal facets has attracted enormous interest due to the fascinating shape-dependent photocatalytic activity of this material. In this work, the effect of the ratio of {001} and {101} facets on the photocatalytic CO2-reduction performance of anatase TiO2 is reported. A new "surface heterojunction" concept is proposed on the basis of the density functional theory (DFT) calculations to explain the difference in the photocatalytic activity of TiO2 with coexposed {001} and {101} facets.
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Metadata
- Authors
- Yu, J., Low, J., Xiao, W., Zhou, P., & Jaroniec, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-06-16
- Volume
- 136
- Issue
- 25
- Pages
- 8839-8842
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1975109963
- Cited by
- 1,905
- References
- 15
- FWCI
- 60.69
- Type
- journal article
- Language
- en
- Open access
- closed
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