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Multiroute Synthesis of Porous Anionic Frameworks and Size-Tunable Extraframework Organic Cation-Controlled Gas Sorption Properties
Abstract
Under diverse and dramatically different chemical environments, including organic solvents, an ionic liquid, and a deep eutectic solvent, a series of porous anionic framework materials that contain size-tunable, ion-exchangeable extraframework organic cations have been prepared. Even though a large fraction of the pore space is occupied with charge-balancing cations, some of these materials exhibit a very high gas uptake capacity (e.g., 70.6 cm(3)/g for CO(2) at 1 atm and 273 K), suggesting that the charged anionic framework and extraframework cations may help to enhance the gas adsorption.
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Metadata
- Authors
- Chen, S., Zhang, J., Wu, T., Feng, P., & Bu, X.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-10-20
- Volume
- 131
- Issue
- 44
- Pages
- 16027-16029
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2094413846
- Cited by
- 262
- References
- 39
- FWCI
- 14.04
- Type
- journal article
- Language
- en
- Open access
- closed
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