Cited by 1,142Quantum Information and CryptographyQuantum Mechanics and ApplicationsQuantum optics and atomic interactions

Ultrabright source of polarization-entangled photons

Open access
Kwiat, Paul G., Waks, Edo, White, Andrew G., Appelbaum, Ian, Eberhard, Philippe H.·1999·Physical Review A

Abstract

Using the process of spontaneous parametric down-conversion in a two-crystal geometry, we have generated a source of polarization-entangled photon pairs that is more than ten times brighter, per unit of pump power, than previous sources, with another factor of 30 to 75 expected to be readily achievable. We have measured a high level of entanglement between photons emitted over a relatively large collection angle, and over a 10-nm bandwidth. As a demonstration of the source capabilities, we obtained a 242-\ensuremath{\sigma} violation of Bell's inequalities in less than three minutes, and observed near-perfect photon correlations when the collection efficiency was reduced. In addition, both the degree of entanglement and the state purity should be readily tunable.

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Written from the paper’s full text.

TL;DR

A two-crystal type-I spontaneous parametric downconversion geometry produced polarization-entangled photon pairs over entire emission cones, yielding a source more than ten times brighter per pump power than previous sources. The authors measured high-visibility entanglement and a 242σ Bell-inequality violation in 160 s.

Key findings

  • The source was more than 10× brighter per unit pump power than previous sources, with another factor of 30–75 expected to be readily achievable; over a 30-nm bandwidth the authors estimate ∼60,000 s⁻¹ mW⁻¹, ∼300× brighter than the previous downconversion scheme (750× if scaled by crystal thickness).
  • Polarization entanglement showed visibility \(V = 99.6 \pm 0.3\%\) with accidental coincidences subtracted and \(98.8 \pm 0.2\%\) with them included, while singles were nearly unpolarized (\(V < 3.4\%\)).
  • At maximum aperture opening they observed over 140 coincidences per second per milliwatt of pump; for 150 mW this implies 21,000 s⁻¹, a ×10 increase over the previous type-II source.
  • A Bell-inequality measurement gave \(S = 2.7007 \pm 0.0029\), a 242σ violation obtained in only 160 s with coincidence rates over 10,000 s⁻¹.

Methods

  • Spontaneous parametric downconversion in two adjacent BBO crystals (8.0 × 8.0 × 0.59 mm, optic axis cut at \(\theta_{pm} = 33.9^\circ\)) oriented with optic axes in perpendicular planes; a 351.1-nm Ar⁺ pump at 45° polarization produced degenerate 702-nm photons in a cone of half-opening angle 3.0°.
  • Characterization used 5-nm or 10-nm interference filters centered at 702 nm, adjustable polarization analyzers (PBS plus HWP), irises, 35-mm doublet lenses, and silicon avalanche photodiodes with ∼65% efficiency and dark counts of order 100 s⁻¹; coincidences were recorded with a 7-ns time window and accidental rates <1 s⁻¹.
  • Measurements included polarization-correlation fringes versus analyzer angle, phase \(\phi\) tuning via a tilted waveplate, visibility versus collection-aperture size, and a Bell-inequality test using 16 analyzer-setting combinations.

Limitations

  • The paper states that dispersion makes the relative phase \(\phi\) wavelength-dependent; to keep all detected photons in essentially the same entangled state, the acceptance bandwidth must be restricted, crystal thicknesses reduced, or a birefringent compensation element included. An acceptable range (\(\phi \le 26^\circ\), \(V \ge 0.9\)) was maintained for a 30-nm bandwidth assuming no other visibility-degrading effects.
  • The paper states that the 1.76-mm irises gave only ∼10% collection efficiency, and the maximum iris size still accessed only ∼8% of the downconversion cone; maximum opening was limited by the collection lens. Some singles-rate net polarization may have come from unexpectedly high BBO background fluorescence, nearly one third of the true singles rate.
  • Evident from the text: most data considered photons from a single cone of colors, and the brightness estimates rely on scaling and the expectation that strong entanglement extends over the entire cone; azimuthal phase variation was <0.02° and could be eliminated with a compensation crystal.

Model-written summary. Check it against the paper before relying on it.

Integrity signals

Registry

Crossref · 10.1103/physreva.60.r773

Cites

37 of 37 references verified0 citation errors · 0 not checkable

Statistics

Nothing to recompute.

Claims the paper makes

0 of 31 cited sources checked · 0 supported · 0 flagged

  • Findingnone given
    § Ultra-bright source of polarization-entangled photons · p. 1

    The source is more than ten times brighter, per unit of pump power, than previous sources.

    “which is more than ten times brighter, per unit of pump power, than previous sources”
    Quote in the paperSubstantial claim
  • Findingown data
    § Ultra-bright source of polarization-entangled photons · p. 1

    Using spontaneous parametric downconversion in a two-crystal geometry, the authors generated a source of polarization-entangled photon pairs.

    “Using the process of spontaneous parametric downconversion in a novel two-crystal geometry, we have generated a source of polarization-entangled photon pairs”
    Quote in the paperSubstantial claim
  • Findingown data
    § Ultra-bright source of polarization-entangled photons · p. 1

    The authors measured a high level of entanglement between photons emitted over a relatively large collection angle and over a 10-nm bandwidth.

    “We have measured a high level of entanglement between photons emitted over a relatively large collection angle, and over a 10-nm bandwidth.”
    Quote in the paperSubstantial claim
  • Findingown data
    § Ultra-bright source of polarization-entangled photons · p. 1

    The source produced a 242σ violation of Bell's inequalities in less than three minutes.

    “we obtained a 242σ violation of Bell's inequalities in less than three minutes”
    Quote in the paperSubstantial claim
  • Findingnone given
    § Ultra-bright source of polarization-entangled photons · p. 1

    Near-perfect photon correlations were observed when the collection efficiency was reduced.

    “observed near-perfect photon correlations when the collection efficiency was reduced”
    Quote in the paperNot a substantial claim
  • May combine two claims. 18
  • Classified as probably not a substantial claim. 10
  • May combine two claims.

    Findingcitation
    § Ultra-bright source of polarization-entangled photons · p. 3

    Following [10], the measurements may be combined to yield S = 2.7007 ± 0.0029, where according to any local realistic theory |S| ≤ 2 and the maximum according to quantum mechanics is 2√2.

    “Following [10], these may be combined to yield a value for the parameter S = 2 . 7007 ± 0 . 0029, where according to any local realistic theory | S | ≤ 2 (and the maximum according to quantum mechanics is 2 √ 2).”
    Quote in the paperSubstantial claim0 of 1 sources checked
    • cites [10] source

      Not checked in the free run.

  • May combine two claims.

    Findingown data
    § Ultra-bright source of polarization-entangled photons · p. 3

    In the second set of measurements with a vertical slit of width 3.5 mm added after each iris and varying vertical dimension, the visibility stayed essentially constant at about 95%, but the coincidence rate still increased.

    “In the second set of measurements (Fig. 3b), a vertical slit of width 3.5mm was added after each iris, and the vertical dimension of the aperture was varied using the iris size; this effectively collects a larger portion of the same cone. The visibility then stayed essentially constant at ∼ 95%, but the coincidence rate still increased.”
    Quote in the paperSubstantial claim
  • Probably not a substantial claim: may not pass S3 (load-bearing). May combine two claims.

    Findingreasoning
    § Ultra-bright source of polarization-entangled photons · p. 3

    The collection irises for this data were both only 1.76 mm in diameter, and the resulting collection efficiency is then about 10%.

    “The collection irises for this data were both only 1.76 mm in diameter - the resulting collection efficiency (the probability of collecting one photon conditioned on collecting the other) is then ∼ 10%.”
    Quote in the paperNot a substantial claim
  • May combine two claims.

    Findingown data
    § Ultra-bright source of polarization-entangled photons · p. 2

    With the state set to HH - VV and the polarization analyzer in path 1 at -45°, the coincidence rate displayed sinusoidal fringes with nearly perfect visibility V = 99.6 ± 0.3% with accidental coincidences subtracted and 98.8 ± 0.2% with them included.

    “As expected, the coincidence rate displayed sinusoidal fringes with nearly perfect visibility ( V = 99 . 6 ± 0 . 3% with 'accidental' coincidences subtracted; 98 . 8 ± 0 . 2% with them included)”
    Quote in the paperSubstantial claim
  • May combine two claims.

    Findingown data
    § Ultra-bright source of polarization-entangled photons · p. 3

    In the first set of data with circular irises, the visibility decreased somewhat as the iris size increased, while the coincidence rate normalized by the input pump power increased.

    “In the first set of data (Fig. 3a), circular irises were used; the visibility decreased somewhat as the iris size increased, while the coincidence rate (normalized by the input pump power) increased.”
    Quote in the paperNot a substantial claim
  • Classified as probably not a substantial claim.

    Premisecitation
    § Ultra-bright source of polarization-entangled photons · p. 1

    The photons produced via the down-conversion process share nonclassical correlations.

    “It is now well known that the photons produced via the down-conversion process share nonclassical correlations [7].”
    Quote in the paperSubstantial claim0 of 1 sources checked
    • cites [7] source

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  • Probably not a substantial claim: may not pass S3 (load-bearing).

    Premisecitation
    § Ultra-bright source of polarization-entangled photons · p. 1

    When a pump photon splits into two daughter photons, conservation of energy and momentum lead to entanglements in two continuous degrees of freedom.

    “conservation of energy and momentum lead to entanglements in these two continuous degrees of freedom [8]”
    Quote in the paperNot a substantial claim0 of 1 sources checked
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  • Probably not a substantial claim: may not pass S4 (based).

    Interpretationnone given
    § Ultra-bright source of polarization-entangled photons · p. 1

    The new technique has the added advantage that the degree of entanglement and the purity of the state may be readily tunable, which was heretofore impossible.

    “The new technique has the added advantage that the degree of entanglement and the purity of the state may be readily tunable, heretofore impossible.”
    Quote in the paperNot a substantial claim
  • May combine two claims.

    Interpretationreasoning
    § Ultra-bright source of polarization-entangled photons · p. 1

    In the two-crystal geometry with type-I phase-matching, with a vertically polarized pump beam, down-conversion will only occur in crystal 1, where the pump is extraordinary polarized, and the resulting down-conversion light cones will be horizontally polarized.

    “With a vertically polarized pump beam, due to the type-I coupling, down-conversion will only occur in crystal 1, where the pump is extraordinary polarized - the resulting down-conversion light cones will be horizontally polarized.”
    Quote in the paperSubstantial claim
  • May combine two claims.

    Interpretationnone given
    § Ultra-bright source of polarization-entangled photons · p. 1

    φ is determined by the details of the phase-matching and the crystal thickness, but can be adjusted by tilting the BBO crystals themselves, by imposing a birefringent phase shift on one of the output beams, or by controlling the relative phase between the horizontal and vertical components of the pump light.

    “φ is determined by the details of the phase-matching and the crystal thickness, but can be adjusted by tilting the BBO crystals themselves (but this changes the cones' opening angles), by imposing a birefringent phase shift on one of the output beams, or by controlling the relative phase between the horizontal and vertical components of the pump light.”
    Quote in the paperSubstantial claim
  • May combine two claims.

    Interpretationreasoning
    § Ultra-bright source of polarization-entangled photons · p. 1

    Because nearly every pair of photons produced is polarization-entangled, the total flux of emitted polarization-entangled pairs should be hundreds of times greater than is achievable with the best previous source, for comparable pump powers.

    “Because nearly every pair of photons produced is polarization-entangled, the total flux of emitted polarization-entangled pairs should be hundreds of times greater than is achievable with the best previous source, for comparable pump powers.”
    Quote in the paperNot a substantial claim
  • Probably not a substantial claim: may not pass S3 (load-bearing), S4 (based). May combine two claims.

    Interpretationnone given
    § Ultra-bright source of polarization-entangled photons · p. 1

    Both the degree of entanglement and the state purity should be readily tunable.

    “both the degree of entanglement and the state purity should be readily tunable”
    Quote in the paperNot a substantial claim
  • Probably not a substantial claim: may not pass S3 (load-bearing), S4 (based).

    Interpretationnone given
    § Ultra-bright source of polarization-entangled photons · p. 1

    Another factor of 30 to 75 in brightness is expected to be readily achievable.

    “with another factor of 30 to 75 expected to be readily achievable”
    Quote in the paperNot a substantial claim
  • May combine two claims.

    Premisecitation
    § Ultra-bright source of polarization-entangled photons · p. 1

    To date there have been only two methods for producing polarization-entangled photon pairs, and each has fairly substantial limitations.

    “To date there have been only two methods for producing such polarization-entangled photon pairs, and each has fairly substantial limitations.”
    Quote in the paperSubstantial claim0 of 4 sources checked
    • cites [9] source

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    • cites [10] source

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    • cites [11] source

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    • cites [12] source

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  • May combine two claims.

    Premisecitation
    § Ultra-bright source of polarization-entangled photons · p. 1

    For two particular emission directions in the type-II source, the correlated photons are produced in the state HV + VH; additional birefringent elements in one or both beams allow the formation of all four Bell states.

    “For two particular emission directions, however, the correlated photons are produced in the state HV + V H ; additional birefringent elements in one or both beams allow the formation of all four Bell states.”
    Quote in the paperSubstantial claim0 of 1 sources checked
    • cites [12] source

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  • May combine two claims.

    Interpretationreasoning
    § Ultra-bright source of polarization-entangled photons · p. 3

    This is about 300 times brighter than the polarization-entangled photon-pair production rates obtainable with the previous down-conversion scheme, and 750 times brighter if scaled by the crystal thickness.

    “This is ∼ 300 times brighter than the polarization-entangled photon-pair production rates obtainable with the previous down-conversion scheme [12], (and 750 times brighter if scaled by the crystal thickness).”
    Quote in the paperSubstantial claim0 of 1 sources checked
    • cites [12] source

      Not checked in the free run.

  • May combine two claims.

    Interpretationreasoning
    § Ultra-bright source of polarization-entangled photons · p. 3

    For all detected down-conversion photons to be described by essentially the same polarization-entangled state, the bandwidth of acceptance needs to be restricted, the crystal thicknesses reduced, or a special birefringent compensation element included.

    “For all detected down-conversion photons to be described by essentially the same polarizationentangled state, the bandwidth of acceptance needs to be restricted, the crystal thicknesses reduced, or a special birefringent compensation element included.”
    Quote in the paperSubstantial claim
  • Probably not a substantial claim: may not pass S3 (load-bearing), S4 (based).

    Interpretationnone given
    § Ultra-bright source of polarization-entangled photons · p. 3

    The authors believe this to be the highest purity entangled state ever reported.

    “We believe this to be the highest purity entangled state ever reported.”
    Quote in the paperNot a substantial claim
  • May combine two claims.

    Interpretationnone given
    § Ultra-bright source of polarization-entangled photons · p. 3

    The source may be used to produce non-maximally entangled states of the form HH + ε VV, |ε| = 1, simply by rotating the pump polarization; for a pump polarized at angle θ to the vertical, ε = tan θ.

    “Another remarkable feature of this source is that it may be used to produce 'non-maximally entangled' states, i.e., states of the form HH + ǫV V , | ǫ | = 1, simply by rotating the pump polarization - for a pump polarized at angle θ to the vertical, ǫ = tan θ .”
    Quote in the paperSubstantial claim
  • Probably not a substantial claim: may not pass S3 (load-bearing).

    Interpretationcitation
    § Ultra-bright source of polarization-entangled photons · p. 3

    Just as with the previous type-II source, the other two Bell states HV ± VH may be prepared simply by inserting a half waveplate in one of the arms to exchange H and V polarization.

    “Just as with the previous typeII source [12], the other two Bell states HV ± V H may be prepared simply by inserting a half waveplate in one of the arms to exchange H and V polarization.”
    Quote in the paperNot a substantial claim0 of 1 sources checked
    • cites [12] source

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  • May combine two claims.

    Interpretationreasoning
    § Ultra-bright source of polarization-entangled photons · p. 3

    For 150-mW pump power, this implies a coincidence rate of 21,000 s−1, a ×10 increase over the previous type-II source, which used a BBO crystal 2.5 times longer.

    “For 150-mW pump power, this implies a coincidence rate of 21,000s -1 [22], a × 10 increase over the previous typeII source (which used a BBO crystal 2.5 times longer [12]).”
    Quote in the paperSubstantial claim0 of 2 sources checked
    • cites [12] source

      Not checked in the free run.

    • cites [22] Signficantly, this is roughly the minimum rate for quantum cryptography in an earth-to-satellite configuration [W. T. Buttler et al ., Phys. Rev. Lett. 81 , 3283 (1998)]. φ also depends on the azimuthal angle of production photons from crystal 1 are extraordinarily-polarized in crystal 2, so the refractive index depends on direction. Our total azimuthal variation in φ was &lt; 0 . 02 ◦ ; this could be eliminated entirely by adding a compensation crystal identical in size and orientation to crystal 2. source

      Not checked in the free run.

  • May combine two claims.

    Interpretationreasoning
    § Ultra-bright source of polarization-entangled photons · p. 3

    Given the symmetry of the arrangement, the authors expect strong entanglement over the entire cone, implying a total polarization-entangled pair production rate over the 5-nm bandwidth of about 10,000 s−1 mW−1, after dividing out filter transmissions and detector efficiencies.

    “Given the symmetry of the arrangement, we expect strong entanglement over the entire cone, implying a total polarization-entangled pair production rate (over the 5-nm bandwidth) of about 10,000 s -1 mW -1 , where we have divided out the filter transmissions and detector efficiencies.”
    Quote in the paperSubstantial claim
  • Probably not a substantial claim: may not pass S3 (load-bearing).

    Premisecitation
    § Ultra-bright source of polarization-entangled photons · p. 4

    Hyper-entangled states may benefit certain experiments in quantum information.

    “and it has been shown that such states may benefit certain experiments in quantum information [15,29].”
    Quote in the paperNot a substantial claim0 of 2 sources checked
    • cites [15] source

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    • cites [29] P. G. Kwiat and H. Weinfurter, Phys. Rev. A 58 , R2623 (1998). source

      Not checked in the free run.

  • May combine two claims.

    Interpretationreasoning
    § Ultra-bright source of polarization-entangled photons · p. 4

    Because the entanglement exists over the entire cones of emitted light, this source is much brighter than previous ones, allowing a tremendous Bell inequality violation in only minutes.

    “Because the entanglement exists over the entire cones of emitted light, this source is much brighter than previous ones, allowing a tremendous Bell inequality violation in only minutes.”
    Quote in the paperSubstantial claim
  • Classified as probably not a substantial claim. May combine two claims.

    Premisereasoning
    § Ultra-bright source of polarization-entangled photons · p. 4

    Such brightness is completely necessary for some applications, like quantum cryptography to a satellite, and very advantageous for others, like teleportation, which requires two pairs of entangled photons and hence scales as the square of the source intensity.

    “Such brightness is completely necessary for some applications (like quantum cryptography to a satellite), and very advantageous for others (like teleportation, which requires two pairs of entangled photons, and hence scales as the square of the source intensity).”
    Quote in the paperSubstantial claim0 of 2 sources checked
    • cites [22] Signficantly, this is roughly the minimum rate for quantum cryptography in an earth-to-satellite configuration [W. T. Buttler et al ., Phys. Rev. Lett. 81 , 3283 (1998)]. φ also depends on the azimuthal angle of production photons from crystal 1 are extraordinarily-polarized in crystal 2, so the refractive index depends on direction. Our total azimuthal variation in φ was &lt; 0 . 02 ◦ ; this could be eliminated entirely by adding a compensation crystal identical in size and orientation to crystal 2. source

      Not checked in the free run.

    • cites [5] source

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25 of 25
  • The authors state this as an assumption.

    No other visibility-degrading effects come into play for the 30 nm bandwidth.

    “assuming no other visibility-degrading effects come into play”
  • The authors state this as an assumption.

    Losses from passing through the first crystal are neglected when considering a 45°-polarized pump photon's equal likelihood to downconvert in either crystal.

    “neglecting losses from passing through the first”
2 of 2

Claims other papers make about this one

Each is checked against this paper’s own text: does it say what the citing paper says it does?

  • The optical system can generate pairs of qubits in an almost arbitrary quantum state of their polarization degrees of freedom.

    “An optical system consisting of lasers, polarization elements and non-linear optical crystals (and collectively characterized for the purposes of this paper as a 'black-box',) is used to generate pairs of qubits in an almost arbitrary quantum state of their polarization degrees of freedom.”

    From Measurement of qubits (2001) · cites this paper as [23]

    The paper describes a two-crystal optical source of photon pairs and says their polarization state can be tuned. On p. 3, however, it specifies non-maximally entangled states of the form HH + εVV and arbitrary (partially) mixed states of a particular form. That supports substantial control over the pairs’ polarization, but not the claim that the system generates almost any two-qubit polarization state. (LLM, conf=0.86)

    Experimental — accuracy not yet measured
  • Using the theory of measurement of qubits, including tomographic reconstruction from 16 polarization measurements together with maximum-likelihood numerical optimization, one can obtain and reconstruct the non-negative definite density operator.

    “It has been shown theoretically and experimentally [56], [57], [58] that using the theory of the measurement of qubits, which includes a tomographic reconstruction of the DMOS due to the linear set of 16 polarization-measurements together with the numerical optimization method, the so-called maximum-likelihood-technique (MLT), one can obtain and reconstruct the non-negative definite density operat”

    From Nonlocal realism tests and quantum state tomography in Sagnac-based type-II polarization-entanglement SPDC-source (2021) · cites this paper as [58]

    Split into 2 atoms — 0 confirmed, 1 partially supported, 0 disputed, 0 misattributed, 1 unverifiable. Expand the claim to see per-atom verdicts.

    Experimental — accuracy not yet measured
  • For a polarization angle of χ with respect to the vertical, the output state is |ψ> = (|HH> + ε e^{iφ}|VV>)/√(1+ε^2), where ε = tan χ.

    “For a polarization angle of χ with respect to the vertical, the output state is, | ψ 〉 = ( | HH 〉 + ε e i φ | VV 〉 ) / √ 1 + ε 2 , where the degree of entanglement, ε = tan χ [21].”
  • The measured GHZ state fidelity exceeds the 50% threshold by 15 standard deviations.

    “The measurements (see Fig. S1) yield a state fidelity of 0.65(1), which exceeds the threshold of 50% [23] by 15 standard deviations.”

Cites

Flagged first, then by citations

Research works printed but not linked: 1

  1. J. S. Bell, 1964, Physics (Long Island City, NY), 1, 195

Cited by

Sorted by citations

Authors
Kwiat, P. G., Waks, E., White, A. G., Appelbaum, I., & Eberhard, P. H.
Affiliations
  • Los Alamos National Laboratory (US)
  • Lawrence Berkeley National Laboratory (US)
Venue
Physical Review A
Published
1999-08-01
Volume
60
Issue
2
Pages
R773-R776
ISSN
  • 0556-2791 (ISSN-L)
  • 1050-2947
  • 1094-1622
OpenAlex
W4241462706
Cited by
1,142
References
37
Citations by year
2026: 35 · 2025: 64 · 2024: 43 · 2023: 65 · 2022: 47 · 2021: 51 · 2020: 55 · 2019: 40 · 2018: 39 · 2017: 51 · 2016: 48 · 2015: 50 · 2014: 45 · 2013: 44 · 2012: 37
FWCI
30.93
Type
journal article
Language
en
Open access
Locations
  • Physical Review A (publishedVersion)
  • arXiv (Cornell University) (submittedVersion)
  • CERN Document Server (European Organization for Nuclear Research) (submittedVersion)
  • arXiv (Cornell University)
Topics
  • Physical Sciences › Computer Science › Artificial Intelligence › Quantum Information and Cryptography
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum Mechanics and Applications
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum optics and atomic interactions
Keywords
polarization-entangled photons, spontaneous parametric down-conversion, entangled photon pairs, Bell inequality violation, photon correlations, source brightness, state purity, quantum optics

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