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Thermal conductance of interfaces between highly dissimilar materials

Lyeo, Ho-Ki, Cahill, David G.·2006·Physical Review B

DOI 10.1103/physrevb.73.144301

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Abstract

The thermal conductance of interfaces between materials with low Debye temperatures (Pb or Bi) and dielectrics or semiconductors with high Debye temperatures (hydrogen-terminated Si, $\mathrm{Si}{\mathrm{O}}_{2}$, the native oxide of Be, sapphire, or hydrogen-terminated diamond) is measured using time-domain thermoreflectance. The interface thermal conductance $G$ for these combinations of materials falls within a relatively narrow range, $8<G<30\phantom{\rule{0.3em}{0ex}}\mathrm{MW}\phantom{\rule{0.2em}{0ex}}{\mathrm{m}}^{\ensuremath{-}2}\phantom{\rule{0.2em}{0ex}}{\mathrm{K}}^{\ensuremath{-}1}$, at room temperature. Because the thermal conductance of interfaces with Bi, a semimetal, and interfaces with Pb, a metal, are similar, we conclude that the coupling of electrons in a metal to phonons in a dielectric substrate does not contribute significantly to the thermal transport at interfaces. For Pb or Bi on hydrogen-terminated diamond, the measured conductance greatly exceeds the radiation limit and decreases approximately linearly with decreasing temperature, suggesting that anharmonic processes dominate the transfer of thermal energy across interfaces between materials with highly dissimilar spectra of lattice vibrations.

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Authors: Lyeo, H.-K., & Cahill, D. G.
Affiliations: University of Illinois Urbana-Champaign (US)
ORCID: Lyeo, Ho-Ki
Cahill, David G.
Venue: Physical Review B
Publisher: American Physical Society (APS)
Published: 2006-04-03
Volume: 73
Issue: 14
ISSN: 1098-0121 (ISSN-L)
1550-235X
DOI: 10.1103/physrevb.73.144301
OpenAlex: W2004164487
Cited by: 576
References: 28
Citations by year: 2026: 19 · 2025: 33 · 2024: 26 · 2023: 19 · 2022: 38 · 2021: 34 · 2020: 31 · 2019: 47 · 2018: 48 · 2017: 31 · 2016: 34 · 2015: 31 · 2014: 26 · 2013: 30 · 2012: 26
FWCI: 9.83
Type: journal article
Language: en
Open access: closed
Licence: link.aps.org/licenses/aps-default-license (vor)
Locations: Physical Review B (publishedVersion)
Funders: National Science Foundation
U.S. Department of Energy
Topics: Physical Sciences › Materials Science › Materials Chemistry › Thermal properties of materials
Physical Sciences › Engineering › Civil and Structural Engineering › Thermal Radiation and Cooling Technologies
Physical Sciences › Engineering › Mechanics of Materials › Thermography and Photoacoustic Techniques
Keywords: interface thermal conductance, metal-dielectric interface, lead, bismuth, hydrogen-terminated diamond, hydrogen-terminated silicon, silica, beryllium oxide, sapphire, electron-phonon coupling, radiation dose limits, lattice vibrations, time-domain thermoreflectance

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Thermal conductance of interfaces between highly dissimilar materials

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