Kapitza conductance and heat flow between solids at temperatures from 50 to 300 K
Abstract
Measurements of the Kapitza conductance ${\mathrm{\ensuremath{\sigma}}}_{\mathit{K}}$ made using a picosecond optical technique at temperatures between 50 and 300 K are presented for interfaces between metals and dielectrics. The Debye temperatures ${\mathit{FTHETA}}_{\mathit{D}}$ of the metals (Pb, Au, Al, and Ti) were in the range from 102 to 426 K, while those of the dielectrics (${\mathrm{BaF}}_{2}$, sapphire, and diamond) varied from 287 to 2200 K. Conductances measured between materials with ${\mathit{FTHETA}}_{\mathit{D}}$ differing by less than about a factor of 5 were found to be in reasonable agreement with calculations based on a lattice dynamical theory. However, for more widely mismatched solids the measured conductances were found to be greatly in excess of the lattice dynamical calculations. In some of these cases the conductances exceeded even the phonon radiation limit, indicating that much of the heat flow between the solids was via an inelastic channel. It was demonstrated experimentally that the inelastic channel does not involve an interaction between the phonons in the dielectric and electrons in the metal. We show that the anomalously large conductance can be understood in terms of a model in which the anharmonicity of the metal plays an important role.
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For all four materials (GaAs, GaN, AlN, 4H-SiC), the thermal interface conductance G increased with temperature.
“For all four materials the thermal interface conductance, G, increased with temperature in agreement with prior studies of metal-dielectric interfaces28.”
From Universal phonon mean free path spectra in crystalline semiconductors at high temperature (2013) · cites this paper as [28]
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- Authors
- Stoner, R. J., & Maris, H. J.
- Affiliations
- Brown University (US)
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 1993-12-01
- Volume
- 48
- Issue
- 22
- Pages
- 16373-16387
- ISSN
- 0163-1829 (ISSN-L)
- 1095-3795
- OpenAlex
- W2091830839
- Cited by
- 646
- References
- 39
- Citations by year
- 2026: 18 · 2025: 18 · 2024: 19 · 2023: 28 · 2022: 28 · 2021: 26 · 2020: 30 · 2019: 37 · 2018: 26 · 2017: 32 · 2016: 28 · 2015: 33 · 2014: 26 · 2013: 23 · 2012: 34
- FWCI
- 3.21
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Physical review. B, Condensed matter (publishedVersion)
- PubMed (publishedVersion)
- Funders
- U.S. Department of Energy (FG0286ER45267)
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › Thermal properties of materials
- Physical Sciences › Engineering › Mechanics of Materials › Thermoelastic and Magnetoelastic Phenomena
- Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Advanced Condensed Matter Physics
- Keywords
- Kapitza conductance, metal-dielectric interface, Debye temperature, lattice dynamics, lead, gold, aluminum, titanium, barium fluoride, sapphire, diamond
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