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A Critical Review of Modeling Transport Phenomena in Polymer-Electrolyte Fuel Cells

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Weber, Adam Z., Borup, Rodney L., Darling, Robert M., Das, Prodip K., Dursch, Thomas J., Gu, Wenbin, Harvey, David, Kusoglu, Ahmet, Litster, Shawn, Mench, Matthew M., Mukundan, Rangachary, Owejan, Jon P., Pharoah, Jon G., Secanell, Marc, Zenyuk, Iryna V.·2014·Journal of The Electrochemical Society
DOI 10.1149/2.0751412jes
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Abstract

Polymer-electrolyte fuel cells are a promising energy-conversion technology. Over the last several decades significant progress has been made in increasing their performance and durability, of which continuum-level modeling of the transport processes has played an integral part. In this review, we examine the state-of-the-art modeling approaches, with a goal of elucidating the knowledge gaps and needs going forward in the field. In particular, the focus is on multiphase flow, especially in terms of understanding interactions at interfaces, and catalyst layers with a focus on the impacts of ionomer thin-films and multiscale phenomena. Overall, we highlight where there is consensus in terms of modeling approaches as well as opportunities for further improvement and clarification, including identification of several critical areas for future research.

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200 of 501 shown

Cited by

Metadata

Authors
Weber, A. Z., Borup, R. L., Darling, R. M., Das, P. K., Dursch, T. J., Gu, W., Harvey, D., Kusoglu, A., Litster, S., Mench, M. M., Mukundan, R., Owejan, J. P., Pharoah, J. G., Secanell, M., & Zenyuk, I. V.
Venue
Journal of The Electrochemical Society
Publisher
The Electrochemical Society
Published
2014
Volume
161
Issue
12
Pages
F1254-F1299
ISSN
  • 0013-4651 (ISSN-L)
  • 1945-7111
DOI
10.1149/2.0751412jes
OpenAlex
W2150124657
Cited by
598
References
19
FWCI
20.87
Type
journal article
Language
en
Open access
hybrid

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