Time-domain mid-infrared frequency-comb spectrometer
Abstract
A novel type of Fourier-transform infrared spectrometer (FTIR) is demonstrated. It is based on two Ti:sapphire lasers emitting femtosecond pulse trains with slightly different repetition frequencies. Two mid-infrared beams-derived from those lasers by rectification in GaSe-are superimposed upon a detector to produce purely time-domain interferograms that encode the infrared spectrum. The advantages of this spectrometer compared with the common FTIR include ease of operation (no moving parts), speed of acquisition (100 micros demonstrated), and not-yet-shown collimated long-distance propagation, diffraction-limited microscopic probing, and electronically controllable chemometric factoring. Extending time-domain frequency-comb spectroscopy to lower (terahertz) or higher (visible, ultraviolet) frequencies should be feasible.
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Hillbrand, J., Auth, D., Piccardo, M., Opačak, N., Gornik, E., Strasser, G., Capasso, F., Breuer, S., & Schwarz, B. (2020) · Physical Review Letters · doi:10.1103/physrevlett.124.023901 · Cited by 109 · see citing works
Cavity-enhanced photoacoustic dual-comb spectroscopy
Wang, Z., Nie, Q., Sun, H., Wang, Q., Borri, S., Natale, P. D., & Ren, W. (2024) · Light Science & Applications · doi:10.1038/s41377-023-01353-6 · Cited by 106 · see citing works
Dual electro-optic optical frequency combs for multiheterodyne molecular dispersion spectroscopy
Martín-Mateos, P., Jerez, B., & Acedo, P. (2015) · Optics Express · doi:10.1364/oe.23.021149 · Cited by 105 · see citing works
Development of ultrafast time-resolved dual-comb spectroscopy
Asahara, A., & Minoshima, K. (2017) · APL Photonics · doi:10.1063/1.4976730 · Cited by 103 · see citing works
Retrieval of phase relation and emission profile of quantum cascade laser frequency combs
Cappelli, F., Consolino, L., Campo, G., Galli, I., Mazzotti, D., Campa, A., de Cumis, M. S., Pastor, P. C., Eramo, R., Rösch, M., et al. (2019) · Nature Photonics · doi:10.1038/s41566-019-0451-1 · Cited by 103 · see citing works
Keilmann, F., & Amarie, S. (2012) · Journal of Infrared Millimeter and Terahertz Waves · doi:10.1007/s10762-012-9894-x · Cited by 103 · see citing works
Self-citationDual frequency comb laser absorption spectroscopy in a 16 MW gas turbine exhaust
Schroeder, P. J., Wright, R. J., Coburn, S., Sodergren, B., Cossel, K. C., Droste, S., Truong, G.-W., Baumann, E., Giorgetta, F. R., Coddington, I. R., et al. (2016) · Proceedings of the Combustion Institute · doi:10.1016/j.proci.2016.06.032 · Cited by 102 · see citing works
Nanophotonic supercontinuum-based mid-infrared dual-comb spectroscopy
Guo, H., Weng, W., Liu, J., Yang, F., Hänsel, W., Brès, C., Thévenaz, L., Holzwarth, R., & Kippenberg, T. J. (2020) · Optica · doi:10.1364/optica.396542 · Cited by 102 · see citing works
Self-citationLiao, R., Tian, H., Liu, W., Li, R., Song, Y., & Hu, M. (2020) · Journal of Physics Photonics · doi:10.1088/2515-7647/aba66e · Cited by 102 · see citing works
- Authors
- Keilmann, F., Gohle, C., & Holzwarth, R.
- Affiliations
- Max Planck Society (DE)
- Venue
- Optics Letters
- Publisher
- Optica Publishing Group
- Published
- 2004-07-01
- Volume
- 29
- Issue
- 13
- Pages
- 1542
- ISSN
- 0146-9592 (ISSN-L)
- 1539-4794
- OpenAlex
- W1979221508
- Cited by
- 734
- References
- 10
- Citations by year
- 2026: 22 · 2025: 26 · 2024: 26 · 2023: 50 · 2022: 29 · 2021: 51 · 2020: 56 · 2019: 43 · 2018: 62 · 2017: 40 · 2016: 60 · 2015: 38 · 2014: 41 · 2013: 33 · 2012: 29
- FWCI
- 4.75
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Optics Letters (publishedVersion)
- PubMed (publishedVersion)
- Max Planck Institute for Plasma Physics (submittedVersion)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- Topics
- Physical Sciences › Chemistry › Spectroscopy › Spectroscopy and Laser Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Advanced Fiber Laser Technologies
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Keywords
- time-domain interferometry, mid-infrared spectroscopy, Fourier transform infrared spectrometer, femtosecond pulse trains, Ti:sapphire laser, terahertz spectroscopy
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