From Water Oxidation to Reduction: Homologous Ni–Co Based Nanowires as Complementary Water Splitting Electrocatalysts

Peng, Zheng; Jia, Dingsi; Al‐Enizi, Abdullah M.; Elzatahry, Ahmed A.; Zheng, Gengfeng

doi:10.1002/aenm.201402031

Cited by 494Electrocatalysts for Energy ConversionCO2 Reduction Techniques and CatalystsAdvanced Photocatalysis Techniques

From Water Oxidation to Reduction: Homologous Ni–Co Based Nanowires as Complementary Water Splitting Electrocatalysts

Peng, Zheng, Jia, Dingsi, Al‐Enizi, Abdullah M., Elzatahry, Ahmed A., Zheng, Gengfeng·2015·Advanced Energy Materials

DOI 10.1002/aenm.201402031

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Abstract

A homologous Ni–Co based nanowire system, consisting of both nickel cobalt oxide and nickel cobalt sulfide nanowires, is developed for efficient, complementary water splitting. The spinel‐type nickel cobalt oxide (NiCo2O4) nanowires are hydrothermally synthesized and can serve as an excellent oxygen evolution reaction catalyst. Subsequent sulfurization of the NiCo2O4 nanowires leads to the formation of pyrite‐type nickel cobalt sulfide (Ni0.33Co0.67S2) nanowires. Due to the 1D nanowire morphology and enhanced charge transport capability, the Ni0.33Co0.67S2 nanowires function as an efficient, stable, and robust nonnoble metal electrocatalyst for hydrogen evolution reaction (HER), substantially exceeding CoS2 or NiS2 nanostructures synthesized under similar methods. The Ni0.33Co0.67S2 nanowires exhibit low onset potential of −65, −39, and −50 mV versus reversible hydrogen electrode, Tafel slopes of 44, 68, and 118 mV dec−1 at acidic, neutral, and basic conditions, respectively, and excellent stability, comparable to the best reported non‐noble metal‐based HER catalysts. Furthermore, the homologous Ni0.33Co0.67S2 nanowires and NiCo2O4 nanowires are assembled into an all‐nanowire based water splitting electrolyzer with a current density of 5 mA cm−2 at a voltage as 1.65 V, thus suggesting a unique homologous, earth abundant material system for water splitting.

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The good catalytic activity is attributed to the synergic effect of the bimetallic nature and the three-dimensional porous structure of the rGO aerogel with good conductivity and favorable mass-transfer pathways.
“The above results clearly demonstrate that the good catalytic activity would be attributed to the synergic effect of the bimetallic nature and three-dimensional porous structure of the rGO aerogel with good conductivity and favorable mass-transfer pathways.22,47–49”
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Electrocatalysts: From Water Oxidation to Reduction: Homologous Ni–Co Based Nanowires as Complementary Water Splitting Electrocatalysts (Adv. Energy Mater. 9/2015)
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Self-citation

Authors: Peng, Z., Jia, D., Al‐Enizi, A. M., Elzatahry, A. A., & Zheng, G.
Affiliations: Fudan University (CN)
King Saud University (SA)
Qatar University (QA)
Corresponding author: Zheng, Gengfeng
ORCID: Al‐Enizi, Abdullah M.
Elzatahry, Ahmed A.
Zheng, Gengfeng
Venue: Advanced Energy Materials
Publisher: Wiley
Published: 2015-02-16
Volume: 5
Issue: 9
ISSN: 1614-6832 (ISSN-L)
1614-6840
DOI: 10.1002/aenm.201402031
OpenAlex: W2144307294
Cited by: 494
References: 37
Citations by year: 2026: 10 · 2025: 11 · 2024: 18 · 2023: 26 · 2022: 37 · 2021: 46 · 2020: 40 · 2019: 69 · 2018: 78 · 2017: 84 · 2016: 56 · 2015: 19
FWCI: 23.39
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Advanced Energy Materials (publishedVersion)
Qatar University QSpace (Qatar University) (submittedVersion)
Funders: National Key Basic Research Program of China (2013CB934104)
Natural Science Foundation of China (21322311, 21473038, 21071033)
Science and Technology Commission of Shanghai Municipality (14JC1490500)
Doctoral Fund of Ministry of Education of China (20130071110031)
Program for Professor of Special Appointment
Deanship of Scientific Research at King Saud University (RG#1435-010)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
Keywords: water splitting, oxygen evolution reaction, hydrogen evolution reaction, NiCo2O4 nanowires, nickel cobalt oxide, NiCo2S4, sulfidation, non-noble metal electrocatalysts, spinel oxides, charge transport, earth-abundant catalysts

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From Water Oxidation to Reduction: Homologous Ni–Co Based Nanowires as Complementary Water Splitting Electrocatalysts

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