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Cited by 207

The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.

Trifunctional Single‐Atomic Ru Sites Enable Efficient Overall Water Splitting and Oxygen Reduction in Acidic Media

Open access
Peng, Xianyun, Zhao, Shunzheng, Mi, Yuying, Han, Lili, Liu, Xijun, Qi, Defeng, Sun, Jiaqiang, Liu, Yifan, Bao, Haihong, Zhuo, Longchao, Xin, Huolin L., Luo, Jun, Sun, Xiaoming·2020·Small

Abstract

Development of cost‐effective, active trifunctional catalysts for acidic oxygen reduction (ORR) as well as hydrogen and oxygen evolution reactions (HER and OER, respectively) is highly desirable, albeit challenging. Herein, single‐atomic Ru sites anchored onto Ti 3 C 2 Tx MXene nanosheets are first reported to serve as trifunctional electrocatalysts for simultaneously catalyzing acidic HER, OER, and ORR. A half‐wave potential of 0.80 V for ORR and small overpotentials of 290 and 70 mV for OER and HER, respectively, at 10 mA cm−2 are achieved. Hence, a low cell voltage of 1.56 V is required for the acidic overall water splitting. The maximum power density of an H 2–O 2 fuel cell using the as‐prepared catalyst can reach as high as 941 mW cm−2. Theoretical calculations reveal that isolated Ru–O 2 sites can effectively optimize the adsorption of reactants/intermediates and lower the energy barriers for the potential‐determining steps, thereby accelerating the HER, ORR, and OER kinetics.

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Metadata

Authors
Peng, X., Zhao, S., Mi, Y., Han, L., Liu, X., Qi, D., Sun, J., Liu, Y., Bao, H., Zhuo, L., Xin, H. L., Luo, J., & Sun, X.
Venue
Small
Publisher
Wiley
Published
2020-07-14
Volume
16
Issue
33
Pages
e2002888-e2002888
ISSN
  • 1613-6810 (ISSN-L)
  • 1613-6829
OpenAlex
W3043132186
Cited by
207
References
10
FWCI
5.59
Type
journal article
Language
en
Open access
green
Funders
  • National Natural Science Foundation of China (51971157, 21601136, 51808037, 51761165012)
  • Office of Science (DE‐SC0012704)

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CoChat. (2026). Citation check: Trifunctional Single‐Atomic Ru Sites Enable Efficient Overall Water Splitting and Oxygen Reduction in Acidic Media. https://app.cochat.ai/papers/10.1002/smll.202002888
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Peng, X., Zhao, S., Mi, Y., Han, L., Liu, X., Qi, D., Sun, J., Liu, Y., Bao, H., Zhuo, L., Xin, H. L., Luo, J., & Sun, X. (2020). Trifunctional Single‐Atomic Ru Sites Enable Efficient Overall Water Splitting and Oxygen Reduction in Acidic Media. Small. https://doi.org/10.1002/smll.202002888

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