Carbonate precipitation in artificial soils produced from basaltic quarry fines and composts: An opportunity for passive carbon sequestration
Open accessAbstract
The proportions of different carbon pools within artificial soils prepared by blending composts with dolerite and basalt quarry fines has changed over a period of 7 years, accumulating inorganic carbon as carbonate minerals newly formed within the soils. With no artificial energy inputs following construction, this is regarded as a passive mineral carbonation process. Carbon isotope data show that up to 40% of the carbon within the soil carbonate is derived from photosynthesis, mixed with carbon from geological sources (limestone present in the quarry fines). Organic matter within the soils shows very variable composition, with an apparent increase with time in the relative proportion of labile carbon relative to more stable forms, reflecting a change in the soil organic matter composition associated with the establishment of new plant communities. The rate of accumulation of inorganic carbon as carbonate minerals is estimated to be equivalent to 4.8 t C ha−1 annually to a depth of 0.3 m, consistent with rates observed for accumulations of carbonate carbon in urban soils containing demolition wastes (annually 3.0 t C ha−1 to 0.3 m). There appears to be substantial potential for artificial soils to be designed expressly for the purpose of carbon capture. The process is analogous to the use of reed beds for the removal of pollutants from contaminated waters.
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Similar observations have been found at other sites, where the rate of CO2 removal has been estimated on the basis of the assumption that calcium carbonate content in soil was zero at the time of demolition or soil formation.
“Similar observations have been found at other sites, where the rate of CO 2 removal has been estimated on the basis of the assumption that calcium carbonate content in soil was zero at the time of demolition 9 or soil formation.14”
From Rapid Removal of Atmospheric CO2 by Urban Soils (2015) · cites this paper as [14]
Calcite precipitation has also been observed in artificial soils prepared by blending natural calcium silicate rocks with compost.
“Although reported here for urban soils with artificial mineral inputs, calcite precipitation has also been observed in artificial soils prepared by blending natural calcium silicate rocks with compost.14”
From Rapid Removal of Atmospheric CO2 by Urban Soils (2015) · cites this paper as [14]
Carbonation appears to decrease with depth, likely due to isolation of materials from the atmosphere; therefore, management that increases atmospheric exposure is likely to increase carbonation rates throughout the site.
“Carbonation appears to decrease with depth, likely due to the isolation of materials from the atmosphere; therefore, management that increases atmospheric exposure (e.g., through appropriate planting that takes CO 2 to depth via plant root systems and associated metabolism) is likely to increase carbonation rates throughout the site.14,45,46”
From Rapid Removal of Atmospheric CO2 by Urban Soils (2015) · cites this paper as [14]
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Coull, M. C., Butler, B. M., Hough, R. L., & Beesley, L. (2021) · Agronomy · doi:10.3390/agronomy11040649 · Cited by 21 · see citing works
Mineral stabilities in soils: how minerals can feed the world and mitigate climate change
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Khalidy, R., Chiang, Y. W., & Santos, R. M. (2023) · CATENA · doi:10.1016/j.catena.2023.107524 · Cited by 21 · see citing works
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Son, Y., Stott, K., Manning, D. A. C., & Cooper, J. M. (2020) · European Journal of Soil Science · doi:10.1111/ejss.13058 · Cited by 18 · see citing works
Rueda, M. P., Comino, F., Aranda, V., Ayora‐Cañada, M. J., & Domínguez‐Vidal, A. (2023) · Spectrochimica Acta Part A Molecular and Biomolecular Spectroscopy · doi:10.1016/j.saa.2023.122450 · Cited by 18 · see citing works
A feasible way to increase carbon sequestration by adding dolomite and K-feldspar to soil
Xiao, L., Sun, Q., Yuan, H., Li, X., Chu, Y., Ruan, Y., Chang-mei, L., & Lian, B. (2016) · Cogent Geoscience · doi:10.1080/23312041.2016.1205324 · Cited by 17 · see citing works
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Sequestering Atmospheric CO2 Inorganically: A Solution for Malaysia’s CO2 Emission
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Craw, D., Rufaut, C., & Pillai, D. (2023) · Mine Water and the Environment · doi:10.1007/s10230-023-00913-x · Cited by 16 · see citing works
Iff, N., Renforth, P., & von Strandmann, P. A. E. P. (2024) · Frontiers in Climate · doi:10.3389/fclim.2024.1252210 · Cited by 16 · see citing works
Santos, R. M., Araujo, F. S. M., Jariwala, H., Khalidy, R., Haque, F., & Chiang, Y. W. (2023) · Frontiers in Earth Science · doi:10.3389/feart.2023.1215930 · Cited by 14 · see citing works
Casas, C. C., Graf, A., Brüggemann, N., Schaschke, C. J., & Jorat, M. E. (2020) · Frontiers in Microbiology · doi:10.3389/fmicb.2020.557119 · Cited by 14 · see citing works
Combining organic amendments with enhanced rock weathering shifts soil carbon storage in croplands
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Kolosz, B. W., Sohi, S., & Manning, D. A. C. (2019) · Computers & Geosciences · doi:10.1016/j.cageo.2018.12.012 · Cited by 12 · see citing works
Brantley, S. L. (2025) · Reviews of Geophysics · doi:10.1029/2025rg000881 · Cited by 11 · see citing works
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Abdalqadir, M. O., Gomari, S. R., Hughes, D. J., Sidiq, A., & Shifa, F. (2023) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2023.138914 · Cited by 11 · see citing works
Calcium carbonate accumulations in Technosols of Moscow city
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Casas, C. C., Schaschke, C. J., Akunna, J. C., & Ehsan Jorat, M. (2019) · Environmental Geotechnics · doi:10.1680/jenge.19.00067 · Cited by 10 · see citing works
In-situ mineral carbonation of ultramafic tailings for carbon dioxide removal: A critical review
Lu, X., Xu, L., Li, X., Hou, Y., Chen, Q., & Li, Q. (2025) · Process Safety and Environmental Protection · doi:10.1016/j.psep.2025.108046 · Cited by 10 · see citing works
Weathering without realizing inorganic CO 2 removal revealed through base cation monitoring
Vienne, A., Frings, P. J., Rijnders, J., Suhrhoff, T. J., Reershemius, T., Poetra, R. P., Hartmann, J., Niron, H., Estrada, M. P., Steinwidder, L., et al. (2026) · SOIL · doi:10.5194/soil-12-421-2026 · Cited by 20 · see citing works
Oladele, S. O., Curaqueo, G., & Awodun, M. A. (2024) · Geoderma Regional · doi:10.1016/j.geodrs.2024.e00887 · Cited by 8 · see citing works
Khalidy, R., Haque, F., Chiang, Y. W., & Santos, R. M. (2025) · Geoderma Regional · doi:10.1016/j.geodrs.2025.e00918 · Cited by 7 · see citing works
Impact of soil erosion on soil organic carbon loss and its implications for carbon neutrality
Yoon, J.-H., Jung, S. S., Kim, H. S., Park, Y., Kim, H., Mishra, U., Gautam, S., Alewell, C., Panagos, P., Kirkham, M. B., et al. (2025) · Advances in agronomy · doi:10.1016/bs.agron.2025.01.005 · Cited by 5 · see citing works
Prole, J. R., Allenby, N., Manning, D. A. C., & Goodfellow, M. (2025) · INTERNATIONAL JOURNAL OF SYSTEMATIC AND EVOLUTIONARY MICROBIOLOGY · doi:10.1099/ijsem.0.006736 · Cited by 5 · see citing works
A sustainability framework for engineering carbon capture soil in transport infrastructure
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Schaffer, Z. R., Rausis, K., Power, I., & Paulo, C. (2025) · Frontiers in Climate · doi:10.3389/fclim.2025.1592626 · Cited by 3 · see citing works
Ali, A., Chiang, Y. W., & Santos, R. M. (2023) · Springer eBooks · doi:10.1007/978-3-031-17425-4_10 · Cited by 2 · see citing works
Ecosystem Services Provided by Agroforestry Systems
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Weathering features of a remineralizer in soil under different land uses
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Greenhouse Gas Emission: Problems, Global Reality, and Future Perspectives
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Wollastonite enhances microbial diversity and ecological network stability
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A Multipurpose Soil Inorganic Carbon Prediction Model
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Geochemical Negative Emission Technologies
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Pó de diabásio e disponibilidade do P no solo
Beltran, M. L. F. (2022) · doi:10.11606/d.11.2022.tde-09022023-175722
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Carbon sequestration of mine waste and utilization as supplementary cementitious material
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- Authors
- Manning, D. A. C., Renforth, P., Lopez-Capel, E., Robertson, S., & Ghazireh, N.
- Affiliations
- Newcastle University (GB)
- University of Oxford (GB)
- Durham University (GB)
- Corresponding author
- Manning, D.A.C.
- Venue
- International journal of greenhouse gas control
- Publisher
- Elsevier BV
- Published
- 2013-09
- Volume
- 17
- Pages
- 309-317
- ISSN
- 1750-5836 (ISSN-L)
- OpenAlex
- W2131652913
- Cited by
- 106
- References
- 56
- Citations by year
- 2026: 6 · 2025: 10 · 2024: 16 · 2023: 15 · 2022: 10 · 2021: 9 · 2020: 10 · 2019: 11 · 2018: 4 · 2017: 6 · 2016: 4 · 2015: 4 · 2014: 1
- FWCI
- 4.34
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Licence
- Locations
- International journal of greenhouse gas control (publishedVersion, cc-by)
- ORCA Online Research @Cardiff (Cardiff University) (submittedVersion)
- Newcastle University ePrints (Newcastle Univesity) (cc-by)
- Funders
- Engineering and Physical Sciences Research Council (EP/F02777X/1)
- Topics
- Life Sciences › Agricultural and Biological Sciences › Soil Science › Soil Carbon and Nitrogen Dynamics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Life Sciences › Agricultural and Biological Sciences › Soil Science › Soil and Environmental Studies
- Keywords
- carbonate precipitation, CO2 mineralization, artificial soil, compost, soil organic matter, labile carbon, carbon isotope analysis, diabase, demolition waste, urban soils, CO2 capture
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