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MoS2 Nanosheets: A Designed Structure with High Active Site Density for the Hydrogen Evolution Reaction
Abstract
Two-dimensional MoS 2 nanosheets (NSs) with high active site density were designed for the hydrogen evolution reaction (HER) through a microdomain reaction method. The effect of the annealing temperature on the microstructure and the HER performance of MoS 2 NSs was examined, and a plausible relation between the stack structures of the MoS 2 catalysts and their HER performance was also explored. The MoS 2 NS electrocatalyst obtained at 550 °C reveals the best HER performance with a relatively small Tafel slope of 68 mV/dec. Both the exposed surface area and active site density are very important for providing a large amount of active sites. The present work has been proved to be an efficient route to achieve a high active site density and a relatively large surface area, which might have potential use in photoelectrocatalytic water splitting.
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Metadata
- Authors
- Wu, Z., Fang, B., Wang, Z., Wang, C., Liu, Z., Liu, F., Wang, W., Alfantazi, A., Wang, D., & Wilkinson, D. P.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-08-16
- Volume
- 3
- Issue
- 9
- Pages
- 2101-2107
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2332269594
- Cited by
- 382
- References
- 49
- FWCI
- 13.22
- Type
- journal article
- Language
- en
- Open access
- closed
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