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Construction of Ultrastable Porphyrin Zr Metal–Organic Frameworks through Linker Elimination
Abstract
A series of highly stable MOFs with 3-D nanochannels, namely PCN-224 (no metal, Ni, Co, Fe), have been assembled with six-connected Zr6 cluster and metalloporphyrins by a linker-elimination strategy. The PCN-224 series not only exhibits the highest BET surface area (2600 m(2)/g) among all the reported porphyrinic MOFs but also remains intact in pH = 0 to pH = 11 aqueous solution. Remarkably, PCN-224(Co) exhibits high catalytic activity for the CO2/propylene oxide coupling reaction and can be used as a recoverable heterogeneous catalyst.
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Metadata
- Authors
- Feng, D., Chung, W.-C., Wei, Z., Gu, Z.-Y., Jiang, H.-L., Chen, Y.-P., Darensbourg, D. J., & Zhou, H.-C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-10-31
- Volume
- 135
- Issue
- 45
- Pages
- 17105-17110
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2072701796
- Cited by
- 1,126
- References
- 0
- FWCI
- 31.58
- Type
- journal article
- Language
- en
- Open access
- closed
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