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Combining theory and experiment in electrocatalysis: Insights into materials design
Open accessAbstract
Better living through water-splitting: Chemists have known how to use electricity to split water into hydrogen and oxygen for more than 200 years. Nonetheless, because the electrochemical route is inefficient, most of the hydrogen made nowadays comes from natural gas. Seh et al. review recent progress in electrocatalyst development to accelerate water-splitting, the reverse reactions that underlie fuel cells, and related oxygen, nitrogen, and carbon dioxide reductions. A unified theoretical framework highlights the need for catalyst design strategies that selectively stabilize distinct reaction intermediates relative to each other. Science , this issue p. 10.1126/science.aad4998
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“However, in terms of the production cost of H 2 as per the price of Pt catalysts, the production of H 2 from noble Pt materials is not effective [8,9].”
From Hierarchically Ordinated Two-Dimensional MoS2 Nanosheets on Three-Dimensional Reduced Graphene Oxide Aerogels as Highly Active and Stable Catalysts for Hydrogen Evolution Reaction (2021) · cites this paper as [9]
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“which has been considered as a key descriptor for HER activity.[ 33 , 34 , 35 , 36 ]”
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“According to Sabatier's principle, the most optimized catalytic phenomena can be observed when interaction between the catalyst surface and intermediate hydrogen atoms (H*) is neither too weak nor too strong.”
From Highly Dispersed Pt Clusters on F-Doped Tin(IV) Oxide Aerogel Matrix: An Ultra-Robust Hybrid Catalyst for Enhanced Hydrogen Evolution (2022) · cites this paper as [4]
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Metadata
- Authors
- Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F.
- Affiliations
- Agency for Science, Technology and Research (SG)
- SLAC National Accelerator Laboratory (US)
- Technical University of Denmark (DK)
- Corresponding author
- Jaramillo, Thomas F.
- ORCID
- Venue
- Science
- Published
- 2017-01-13
- Volume
- 355
- Issue
- 6321
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2573377826
- Cited by
- 12,114
- References
- 174
- Citations by year
- 2026: 1162 · 2025: 1440 · 2024: 1571 · 2023: 1512 · 2022: 1552 · 2021: 1501 · 2020: 1338 · 2019: 1100 · 2018: 722 · 2017: 210
- FWCI
- 36.99
- Type
- journal article
- Language
- en
- Open access
- green
- www.osti.gov
- Locations
- Science (publishedVersion)
- PubMed (publishedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Technical University of Denmark, DTU Orbit (Technical University of Denmark, DTU) (submittedVersion, other-oa)
- Funders
- National Science Foundation ((DGE-114747)
- U.S. Department of Energy (76SF00515, DE–AC02–76SF00515, DGE-114747, AC02‐76SF00515, DE-AC02-)
- Villum Fonden (00009455)
- National Research Foundation (DGE-114747)
- National Research Foundation Singapore
- Office of Science (AC02-76SF00515, DE-AC02-76SF0051 5, DE-AC02, 76SF00515)
- Basic Energy Sciences (DE-AC02, 76SF00515, AC02-76SF00515, DE-AC-02-76SF00515)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Keywords
- electrocatalysis, heterogeneous electrocatalysts, integration of theory and experiment, water oxidation, hydrogen evolution reaction, oxygen reduction reaction, hydrogen peroxide production, carbon dioxide reduction, nitrogen reduction, clean energy conversion
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