Cited by 261Advanced battery technologies researchNanomaterials and Printing TechnologiesAdvanced Sensor and Energy Harvesting Materials

All‐Printed, Stretchable Zn‐Ag2O Rechargeable Battery via Hyperelastic Binder for Self‐Powering Wearable Electronics

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Kumar, Rajan, Shin, Jaewook, Yin, Lu, You, Jung‐Min, Meng, Ying Shirley, Wang, Joseph·2017·Advanced Energy Materials

Abstract

While several stretchable batteries utilizing either deterministic or random composite architectures have been described, none have been fabricated using inexpensive printing technologies. In this study, the authors printed a highly stretchable, zinc‐silver oxide (Zn‐Ag 2 O) battery by incorporating polystyrene‐block‐polyisoprene‐block‐polystyrene (SIS) as a hyperelastic binder for custom‐made printable inks. The remarkable mechanical properties of the SIS binder lead to an all‐printed, stretchable Zn‐Ag 2 O rechargeable battery with a ≈2.5 mA h cm−2 reversible capacity density even after multiple iterations of 100% stretching. This battery offers the highest reversible capacity and discharge current density for intrinsically stretchable batteries reported to date. The electrochemical and mechanical properties are characterized under different strain conditions. The new stress‐enduring printable inks pave ways for further developing stretchable electronics for the wide range of wearable applications.

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  • Wearable batteries have been developed on stretchable and flexible materials for greater wearability, but have not yet demonstrated sufficient energy density for long-term use.

    “Alternatively, wearable batteries have been developed on stretchable and flexible materials for greater wearability, but have not yet demonstrated sufficient energy density for long-term use177-179.”

    From Wearable biosensors for healthcare monitoring (2019) · cites this paper as [179]

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Research works printed but not linked: 60

  1. A. J. Bandodkar, I. Jeerapan, J.-M. You, R. Nuñez-Flores, J. Wang, Nano Lett. 2016, 16, 721.
  2. H. Lee, T. K. Choi, Y. B. Lee, H. R. Cho, R. Ghaffari, L. Wang, H. J. Choi, T. D. Chung, N. Lu, T. Hyeon, S. H. Choi, D.-H. Kim, Nat. Nano 2016, 11, 566.
  3. R. Cánovas, M. Parrilla, P. Mercier, F. J. Andrade, J. Wang, Adv. Mater. Technol. 2016, 1, 1600061;
  4. M. Amjadi, K.-U. Kyung, I. Park, M. Sitti, Adv. Funct. Mater. 2016, 26, 1678;
  5. A. J. Bandodkar, I. Jeerapan, J. Wang, ACS Sens. 2016, 1, 464.
  6. J. Lee, J. Wu, M. Shi, J. Yoon, S.-I. Park, M. Li, Z. Liu, Y. Huang, J. A. Rogers, Adv. Mater. 2011, 23, 986;
  7. D. J. Lipomi, B. C. K. Tee, M. Vosgueritchian, Z. Bao, Adv. Mater. 2011, 23, 1771.
  8. T. Yokota, P. Zalar, M. Kaltenbrunner, H. Jinno, N. Matsuhisa, H. Kitanosako, Y. Tachibana, W. Yukita, M. Koizumi, T. Someya, Sci. Adv. 2016, 2, e1501856;
  9. J. Liang, L. Li, X. Niu, Z. Yu, Q. Pei, Nat. Photonics 2013, 7, 817.
  10. S. Imani, A. J. Bandodkar, A. M. V. Mohan, R. Kumar, S. Yu, J. Wang, P. P. Mercier, Nat. Commun. 2016, 7, 11650;
  11. J. Kim, I. Jeerapan, S. Imani, T. N. Cho, A. Bandodkar, S. Cinti, P. P. Mercier, J. Wang, ACS Sens. 2016, 1, 1011;
  12. A. J. Bandodkar, W. Jia, C. Yardımcı, X. Wang, J. Ramirez, J. Wang, Anal. Chem. 2015, 87, 394;
  13. P. Kassal, J. Kim, R. Kumar, W. R. de Araujo, I. M. Steinberg, M. D. Steinberg, J. Wang, Electrochem. Commun. 2015, 56, 6;
  14. X. Huang, Y. Liu, H. Cheng, W.-J. Shin, J. A. Fan, Z. Liu, C.-J. Lu, G.-W. Kong, K. Chen, D. Patnaik, S.-H. Lee, S. Hage-Ali, Y. Huang, J. A. Rogers, Adv. Funct. Mater. 2014, 24, 3846;
  15. D. Son, J. Lee, S. Qiao, R. Ghaffari, J. Kim, J. E. Lee, C. Song, S. J. Kim, D. J. Lee, S. W. Jun, S. Yang, M. Park, J. Shin, K. Do, M. Lee, K. Kang, C. S. Hwang, N. Lu, T. Hyeon, D.-H. Kim, Nat. Nano 2014, 9, 397.
  16. L. Xu, S. R. Gutbrod, Y. Ma, A. Petrossians, Y. Liu, R. C. Webb, J. A. Fan, Z. Yang, R. Xu, J. J. Whalen, J. D. Weiland, Y. Huang, I. R. Efimov, J. A. Rogers, Adv. Mater. 2015, 27, 1731.
  17. C. Wu, T. W. Kim, F. Li, T. Guo, ACS Nano 2016, 10, 6449;
  18. Y. Meng, Y. Zhao, C. Hu, H. Cheng, Y. Hu, Z. Zhang, G. Shi, L. Qu, Adv. Mater. 2013, 25, 2326.
  19. S. I. Park, D. S. Brenner, G. Shin, C. D. Morgan, B. A. Copits, H. U. Chung, M. Y. Pullen, K. N. Noh, S. Davidson, S. J. Oh, J. Yoon, K.-I. Jang, V. K. Samineni, M. Norman, J. G. Grajales-Reyes, S. K. Vogt, S. S. Sundaram, K. M. Wilson, J. S. Ha, R. Xu, T. Pan, T.-i. Kim, Y. Huang, M. C. Montana, J. P. Golden, M. R. Bruchas, R. W. Gereau Iv, J. A. Rogers, Nat. Biotechnol. 2015, 33, 1280.
  20. N. Lu, D.-H. Kim, Soft Rob. 2013, 1, 53.
  21. D. J. Lipomi, Adv. Mater. 2016, 28, 4180;
  22. D.-H. Kim, J. A. Rogers, Adv. Mater. 2008, 20, 4887.
  23. S. Berchmans, A. J. Bandodkar, W. Jia, J. Ramirez, Y. S. Meng, J. Wang, J. Mater. Chem. A 2014, 2, 15788.
  24. R. E. Sousa, C. M. Costa, S. Lanceros-Méndez, ChemSusChem 2015, 8, 3539;
  25. Stretchable Electronics (Ed: T. Someya), Wiley-VCH Verlag GmbH & Co. KGaA 2012, p. 287.
  26. Z. M. Song, X. Wang, C. Lv, Y. H. An, M. B. Liang, T. Ma, D. He, Y. J. Zheng, S. Q. Huang, H. Y. Yu, H. Q. Jiang, Sci. Rep. 2015, 5, 10988;
  27. S. Jung, S. Hong, J. Kim, S. Lee, T. Hyeon, M. Lee, D. H. Kim, Sci. Rep. 2015, 5, 17081;
  28. S. Xu, Y. H. Zhang, J. Cho, J. Lee, X. Huang, L. Jia, J. A. Fan, Y. W. Su, J. Su, H. G. Zhang, H. Y. Cheng, B. W. Lu, C. J. Yu, C. Chuang, T. I. Kim, T. Song, K. Shigeta, S. Kang, C. Dagdeviren, I. Petrov, P. V. Braun, Y. G. Huang, U. Paik, J. A. Rogers, Nat. Commun. 2013, 4, 4479.
  29. Y. H. Kwon, S. W. Woo, H. R. Jung, H. K. Yu, K. Kim, B. H. Oh, S. Ahn, S. Y. Lee, S. W. Song, J. Cho, H. C. Shin, J. Y. Kim, Adv. Mater. 2012, 24, 5192;
  30. A. M. Zamarayeva, A. M. Gaikwad, I. Deckman, M. Wang, B. Khau, D. A. Steingart, A. C. Arias, Adv. Electron. Mater. 2016, 2, 1500296.
  31. A. M. Gaikwad, A. M. Zamarayeva, J. Rousseau, H. W. Chu, I. Derin, D. A. Steingart, Adv. Mater. 2012, 24, 5071.
  32. S. Berchmans, A. J. Bandodkar, W. Z. Jia, J. Ramirez, Y. S. Meng, J. Wang, J. Mater. Chem. A 2014, 2, 15788.
  33. C. Y. Yan, X. Wang, M. Q. Cui, J. X. Wang, W. B. Kang, C. Y. Foo, P. S. Lee, Adv. Energy Mater. 2014, 4, 1301396.
  34. G. Kettlgruber, M. Kaltenbrunner, C. M. Siket, R. Moser, I. M. Graz, R. Schwodiauer, S. Bauer, J. Mater. Chem. A 2013, 1, 5505.
  35. S. Xu, Y. Zhang, J. Cho, J. Lee, X. Huang, L. Jia, J. A. Fan, Y. Su, J. Su, H. Zhang, H. Cheng, B. Lu, C. Yu, C. Chuang, T.-i. Kim, T. Song, K. Shigeta, S. Kang, C. Dagdeviren, I. Petrov, P. V. Braun, Y. Huang, U. Paik, J. A. Rogers, Nat. Commun. 2013, 4, 1543.
  36. Z. Song, X. Wang, C. Lv, Y. An, M. Liang, T. Ma, D. He, Y.-J. Zheng, S.-Q. Huang, H. Yu, H. Jiang, Sci. Rep. 2015, 5, 10988.
  37. T. F. O'Connor, S. Savagatrup, D. J. Lipomi, in Stretchable Bio- electronics for Medical Devices and Systems, (Eds: A. J. Rogers, R. Ghaffari, D.-H. Kim), Springer International Publishing, Cham, Switzerland 2016, p. 69.
  38. M. D. Dickey, in Stretchable Bioelectronics for Medical Devices and Systems, (Eds: A. J. Rogers, R. Ghaffari, D.-H. Kim), Springer International Publishing, Cham, Switzerland 2016, p. 3;
  39. M. Park, J. Park, U. Jeong, Nano Today 2014, 9, 244.
  40. A. M. Gaikwad, G. L. Whiting, D. A. Steingart, A. C. Arias, Adv. Mater. 2011, 23, 3251.
  41. J. A. Fan, W.-H. Yeo, Y. Su, Y. Hattori, W. Lee, S.-Y. Jung, Y. Zhang, Z. Liu, H. Cheng, L. Falgout, M. Bajema, T. Coleman, D. Gregoire, R. J. Larsen, Y. Huang, J. A. Rogers, Nat. Commun. 2014, 5, 3266;
  42. C. Yan, X. Wang, M. Cui, J. Wang, W. Kang, C. Y. Foo, P. S. Lee, Adv. Energy Mater. 2014, 4, 1301396.
  43. H. Kim, J. Yoon, G. Lee, S.-h. Paik, G. Choi, D. Kim, B.-M. Kim, G. Zi, J. S. Ha, ACS Appl. Mater. Interfaces 2016, 8, 16016.
  44. S. Yang, Y.-C. Chen, L. Nicolini, P. Pasupathy, J. Sacks, B. Su, R. Yang, D. Sanchez, Y.-F. Chang, P. Wang, D. Schnyer, D. Neikirk, N. Lu, Adv. Mater. 2015, 27, 6423.
  45. K. Braam, V. Subramanian, Adv. Mater. 2015, 27, 689.
  46. A. Y. Coran, in The Science and Technology of Rubber, 4th ed., Academic Press, Boston 2013, p. 337.
  47. N. Matsuhisa, M. Kaltenbrunner, T. Yokota, H. Jinno, K. Kuribara, T. Sekitani, T. Someya, Nat. Commun. 2015, 6, 7461.
  48. A. J. Bandodkar, R. Nuñez-Flores, W. Jia, J. Wang, Adv. Mater. 2015, 27, 3060.
  49. M. Hu, X. Cai, Q. Guo, B. Bian, T. Zhang, J. Yang, ACS Nano 2016, 10, 396.
  50. H. Stoyanov, M. Kollosche, S. Risse, R. Waché, G. Kofod, Adv. Mater. 2013, 25, 578.
  51. P. Bing, Q. Kemao, X. Huimin, A. Anand, Meas. Sci. Technol. 2009, 20, 062001.
  52. Q. C. Zhuang, S. D. Xu, X. Y. Qiu, Y. L. Cui, L. A. Fang, S. G. Sun, Prog. Chem. 2010, 22, 1044.
  53. Y. L. Shi, M. F. Shen, S. D. Xu, X. Y. Qiu, L. Jiang, Y. H. Qiang, Q. C. Zhuang, S. G. Sun, Int. J. Electrochem. Sci. 2011, 6, 3399.
  54. B. P. Grady, S. L. Cooper, C. G. Robertson, in The Science and Technology of Rubber, 4th ed., Academic Press, Boston 2013, p. 591.
  55. M. Morton, Rubber Technology, Springer Science & Business Media, Dordrecht 2013.
  56. O. Olabisi, L. M. Robeson, M. T. Shaw, Polymer-Polymer Miscibility, Academic Press, New York 1979, p. 195.
  57. D. Liu, L.-C. Chen, T.-J. Liu, T. Fan, E.-Y. Tsou, C. Tiu, Adv. Chem. Eng. Sci. 2014, 4, 14;
  58. K. Suganuma, Introduction to Printed Electronics, Springer, New York 2014, p. 23.
  59. J.-M. Y. Jaewook Shin, J. Z Lee, R. Kumar, L. Yin, J. Wang, Y. S. Meng, Phys. Chem. Chem. Phys. 2016, 18, 26376.
  60. S. Hong, D. Sycks, H. F. Chan, S. Lin, G. P. Lopez, F. Guilak, K. W. Leong, X. Zhao, Adv. Mater. 2015, 27, 4035.

Cited by

Sorted by citations

Authors
Kumar, R., Shin, J., Yin, L., You, J., Meng, Y. S., & Wang, J.
Affiliations
University of California San Diego (US)
Corresponding author
  • Meng, Ying Shirley
  • Wang, Joseph
Venue
Advanced Energy Materials
Publisher
Wiley
Published
2016-12-19
Volume
7
Issue
8
ISSN
  • 1614-6832 (ISSN-L)
  • 1614-6840
OpenAlex
W2565783693
Cited by
261
References
57
Citations by year
2026: 13 · 2025: 21 · 2024: 16 · 2023: 21 · 2022: 34 · 2021: 38 · 2020: 48 · 2019: 29 · 2018: 31 · 2017: 10
FWCI
10.76
Type
journal article
Language
en
Open access
Locations
  • Advanced Energy Materials (publishedVersion)
  • eScholarship (California Digital Library) (submittedVersion)
  • OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
Funders
  • Advanced Research Projects Agency - Energy (DE‐AR0000535)
  • National Science Foundation (ECCS‐1542148)
Topics
  • Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced battery technologies research
  • Physical Sciences › Engineering › Electrical and Electronic Engineering › Nanomaterials and Printing Technologies
  • Physical Sciences › Engineering › Biomedical Engineering › Advanced Sensor and Energy Harvesting Materials
Keywords
stretchable batteries, printable inks, rechargeable batteries, wearable electronics, self-powering, strain tolerance, reversible capacity, discharge current density

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