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Designing Adsorbents for CO2 Capture from Flue Gas-Hyperbranched Aminosilicas Capable of Capturing CO2 Reversibly
Abstract
Carbon dioxide adsorption from a simulated flue gas stream was successfully performed with a hyperbranched aminosilica (HAS) material. The HAS was synthesized by a one-step reaction, spontaneous aziridine ring-opening polymerization off of surface silanols, to form a 32 wt % organic/inorganic hybrid material. The adsorption measurements were performed in a fixed-bed flow reactor using humidified CO 2 . The advantage of this adsorbent over previously reported adsorbents is the stability of the organic groups covalently bound to the silica support compared to those made by physisorbed methods. Furthermore, a large CO 2 capacity (∼3 mmol CO 2 /g adsorbent) associated with the high loading of amines was observed.
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Metadata
- Authors
- Hicks, J. C., Drese, J. H., Fauth, D. J., Gray, M. L., Qi, G., & Jones, C. W.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-02-19
- Volume
- 130
- Issue
- 10
- Pages
- 2902-2903
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1967743582
- Cited by
- 758
- References
- 22
- FWCI
- 100.29
- Type
- journal article
- Language
- en
- Open access
- closed
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