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Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction

Li, Leigang, Wang, Pengtang, Shao, Qi, Huang, Xiaoqing·2021·Advanced Materials
DOI 10.1002/adma.202004243
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Abstract

Proton exchange membrane (PEM) water electrolyzers hold great significance for renewable energy storage and conversion. The acidic oxygen evolution reaction (OER) is one of the main roadblocks that hinder the practical application of PEM water electrolyzers. Highly active, cost‐effective, and durable electrocatalysts are indispensable for lowering the high kinetic barrier of OER to achieve boosted reaction kinetics. To date, a wide spectrum of advanced electrocatalysts has been designed and synthesized for enhanced acidic OER performance, though Ir and Ru based nanostructures still represent the state‐of‐the‐art catalysts. In this Progress Report, recent research progress in advanced electrocatalysts for improved acidic OER performance is summarized. First, fundamental understanding about acidic OER including reaction mechanisms and atomic understanding to acidic OER for rational design of efficient electrocatalysts are discussed. Thereafter, an overview of the progress in the design and synthesis of advanced acidic OER electrocatalysts is provided in terms of catalyst category, i.e., metallic nanostructures (Ir and Ru based), precious metal oxides, nonprecious metal oxides, and carbon based nanomaterials. Finally, perspectives to the future development of acidic OER are provided from the aspects of reaction mechanism investigation and more efficient electrocatalyst design.

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Metadata

Authors
Li, L., Wang, P., Shao, Q., & Huang, X.
Venue
Advanced Materials
Publisher
Wiley
Published
2021-03-21
Volume
33
Issue
50
Pages
e2004243-e2004243
ISSN
  • 0935-9648 (ISSN-L)
  • 1521-4095
DOI
10.1002/adma.202004243
OpenAlex
W3137843768
Cited by
672
References
14
FWCI
20.77
Type
journal article
Language
en
Open access
closed
Licence
onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Funders
  • Ministry of Science and Technology (2016YFA0204100, 2017YFA0208200)
  • National Natural Science Foundation of China (21571135)
  • Xiamen University

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Li, L., Wang, P., Shao, Q., & Huang, X. (2021). Recent Progress in Advanced Electrocatalyst Design for Acidic Oxygen Evolution Reaction. Advanced Materials. https://doi.org/10.1002/adma.202004243

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