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Metal-organic framework-derived nanocomposites for electrocatalytic hydrogen evolution reaction

Chen, Ziliang, Qing, Huilin, Zhou, Kun, Sun, Dalin, Wu, Renbing·2020·Progress in Materials Science
DOI 10.1016/j.pmatsci.2019.100618
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Abstract

Abstract The rapid development of hydrogen energy is strongly dependent on the economic and efficient production of hydrogen. The electrocatalytic splitting of water to molecular hydrogen via the hydrogen evolution reaction (HER) provides an appealing solution for producing high-purity hydrogen, but low-cost and highly active electrocatalysts are required for HER. Among currently investigated HER electrocatalysts, metal-organic framework (MOF)-derived nanocomposites constructed from transition metals (TMs)/TM compounds (TMCs) and carbon materials offer extremely promising and attractive HER activities because of their unique properties, such as tunable compositions, readily regulated electronic structures, controllable morphologies, and diverse configuration. Herein, this article provides a comprehensive overview of MOF-derived nanocomposites as HER electrocatalysts for water splitting. It begins with the introduction of the fundamentals of electrocatalytic HER. Afterwards, several ingeniously designed strategies for improved MOF-derived HER electrocatalysts are meticulously summarized and discussed, with special emphasis on the component manipulation of the TMs/TMCs, carbon matrix modifications, morphology tuning and electrode configuration engineering. Finally, future perspectives on the development of these nanocomposites as HER electrocatalysts are proposed.

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Metadata

Authors
Chen, Z., Qing, H., Zhou, K., Sun, D., & Wu, R.
Venue
Progress in Materials Science
Publisher
Elsevier BV
Published
2020-02
Volume
108
Pages
100618
ISSN
0079-6425 (ISSN-L)
DOI
10.1016/j.pmatsci.2019.100618
OpenAlex
W2983671346
Cited by
343
References
31
FWCI
7.16
Type
journal article
Language
en
Open access
closed
Licence
  • www.elsevier.com/tdm/userlicense/1.0/ (tdm)
  • www.elsevier.com/legal/tdmrep-license (tdm)
Funders
National Natural Science Foundation of China

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Chen, Z., Qing, H., Zhou, K., Sun, D., & Wu, R. (2020). Metal-organic framework-derived nanocomposites for electrocatalytic hydrogen evolution reaction. Progress in Materials Science. https://doi.org/10.1016/j.pmatsci.2019.100618

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