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Anion-Containing Noble-Metal-Free Bifunctional Electrocatalysts for Overall Water Splitting
Abstract
With ever-increasing severe environment pollutions and energy demand, it is becoming greatly important to develop sustainable energy resources as alternatives to traditional fossil fuels. As one of the ultimate clean energy sources, hydrogen (H 2 ) energy produced by water splitting using electricity from solar radiation, wind, tide, and nuclear fusion, among other sources, has attracted more and more public attention since the late 18th century. Although noble-metal-based electrocatalysts perform well, they suffer severely from the high cost and rarity from the viewpoint of practical applications. Recently, various kinds of non-noble-metal electrocatalysts based on low cost and earth-abundant transition metals have been developed for both hydrogen evolution reaction (HER) and oxygen (O 2 ) evolution reaction (OER). Among them, non-noble-metal bifunctional electrocatalysts (NHOBEs), showing high performances in both HER and OER, are therefore of great significance and importance in future applications. With NHOBEs, one will be able to significantly simplify the fabrication procedures of electrolyzers, and more importantly, elevate the efficiency of “all in one” electrocatalytic water-splitting systems, which will greatly favor their industrial applications by demanding substantially lowered the production costs. While the laws of NHOBEs from the same main group anionic elements such as oxygen, nitrogen, carbon, and boron families have not been well-reported so far. Herein, the recent significant progresses of NHOBEs classified by different main group anionic elements are summarized, and emphases are placed to the designs, syntheses, electrocatalytic performances in water-splitting, and future possible applications of NHOBEs. Moreover, the prospects of a number of vigorously investigated NHOBE catalysts and the possible trends of future developments are also evaluated. In addition, current challenges facing research with respect to electrocatalysts for water-splitting are discussed.
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Metadata
- Authors
- Xiong, B., Chen, L., & Shi, J.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-02-06
- Volume
- 8
- Issue
- 4
- Pages
- 3688-3707
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2791662045
- Cited by
- 328
- References
- 128
- FWCI
- 7.41
- Type
- journal article
- Language
- en
- Open access
- closed
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
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Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
