Potential for large-scale CO2 removal via enhanced rock weathering with croplands
Open accessAbstract
Enhanced silicate rock weathering (ERW), deployable with croplands, has potential use for atmospheric carbon dioxide (CO 2) removal (CDR), which is now necessary to mitigate anthropogenic climate change 1. ERW also has possible co-benefits for improved food and soil security, and reduced ocean acidification 2-4. Here we use an integrated performance modelling approach to make an initial techno-economic assessment for 2050, quantifying how CDR potential and costs vary among nations in relation to business-as-usual energy policies and policies consistent with limiting future warming to 2 degrees Celsius 5. China, India, the USA and Brazil have great potential to help achieve average global CDR goals of 0.5 to 2 gigatonnes of carbon dioxide (CO 2) per year with extraction costs of approximately US$80-180 per tonne of CO 2. These goals and costs are robust, regardless of future energy policies. Deployment within existing croplands offers opportunities to align agriculture and climate policy. However, success will depend upon overcoming political and social inertia to develop regulatory and incentive frameworks. We discuss the challenges and opportunities of ERW deployment, including the potential for excess industrial silicate materials (basalt mine overburden, concrete, and iron and steel slag) to obviate the need for new mining, as well as uncertainties in soil weathering rates and land-ocean transfer of weathered products.
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TL;DR
Enhanced silicate rock weathering (ERW) on existing croplands could remove 0.5–2 Gt CO₂ yr⁻¹ by 2050, with China, India, the USA and Brazil having the largest potential. Estimated extraction costs of ~$80–180 t⁻¹ CO₂ are robust across business-as-usual and 2°C energy scenarios, but deployment depends on policy, social acceptance and field validation.
Key findings
- ERW could contribute 0.5–2 Gt CO₂ yr⁻¹ globally by 2050; aggregate CDR of 25–100 Gt CO₂ over five decades would save up to 10% of the remaining ~900 Gt CO₂ budget for limiting warming to below 2°C.
- The top three ranked countries for CDR potential are China, USA and India; Indonesia and Brazil also have relatively high potential due to extensive agricultural lands and suitable climates, while European countries have an order-of-magnitude lower potential than China, USA and India.
- Costs vary by nation: USA $160–180 t⁻¹ CO₂, Canada and European nations $160–190 t⁻¹ CO₂, and China, India, Mexico, Indonesia and Brazil $55–120 t⁻¹ CO₂. A carbon price of $100–150 t⁻¹ CO₂ would cover most ERW costs for key nations.
- ERW could augment 2030 NDCs by ~5–10% for China and the USA, 40% for India, and 100% of Brazil’s pledged 2030 CO₂ emissions plus some fraction of other countries’ emissions; France and Spain up to ~40%, and Poland, Italy and Germany ~10%.
Methods
- Integrated performance model with sub-national detail for major economies (USA, India, China, Brazil, Europe, plus Indonesia, Canada, Mexico), using a 1-D vertical reactive transport model with steady-state flow and a rock-grain dissolution source term.
- Baseline application rate of 40 t ha⁻¹ yr⁻¹; two basalt types (fast- and slow-weathering) and two log-normal particle size distributions; optimization of p80 for maximum net CDR; Monte Carlo sampling (n ≈ 100) for fractal-dimension uncertainty; BAU and 2°C energy scenarios for 2050.
- Cost assessment includes mining, processing, distribution/transport and spreading, using GIS origin-destination rail/road network analysis and country-specific diesel, labour and electricity costs; silicate waste production forecast using SSP2 GDP projections.
Limitations
- Stated: uncertainties in baseline application rate and basalt mineralogy; extrapolation of laboratory weathering rates to field scale; surface passivation not treated in detail; need for long-term field-scale ERW trials; potential trapping of weathered cations on ion exchange surfaces or in secondary minerals; poorly constrained duration of carbon sequestration and possible CO₂ sink saturation; possible CO₂ degassing in large river systems not considered; no account of wider impacts of ERW supply chains on other markets; recycling penetration for steel not considered beyond current rate.
- Stated: success depends on overcoming political and social inertia, developing regulatory and incentive frameworks, and wider public acceptance.
- Evident from the text: the analysis is a techno-economic modelling assessment, not field-validated; the performance model does not explicitly account for secondary clay minerals, which the authors note makes it conservative with respect to basalt dissolution.
Model-written summary. Check it against the paper before relying on it.
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- Findingown data§ The potential for large-scale CO 2 removal via rock weathering on croplands
Extraction costs for China, India, the United States and Brazil are ~$80-180 t -1 CO2.
“China, India, the United States and Brazil have large potential to help achieve average global CDR targets of 0.5 to 2 Gt CO2 yr -1 with extraction costs of ~$80-180 t -1 CO2.”
Quote in the paperSubstantial claim - Findingown data§ The potential for large-scale CO 2 removal via rock weathering on croplands
China, India, the United States and Brazil have large potential to help achieve average global CDR targets of 0.5 to 2 Gt CO2 yr -1.
“China, India, the United States and Brazil have large potential to help achieve average global CDR targets of 0.5 to 2 Gt CO2 yr -1 with extraction costs of ~$80-180 t -1 CO2.”
Quote in the paperSubstantial claim - Findingcitation
The three top ranked countries with the highest CDR potential are coincidentally the highest fossil fuel CO2 emitters (China, USA and India).
“Overall, we find the three top ranked countries with the highest CDR potential are coincidentally the highest fossil fuel CO2 emitters (China, USA and India) 6 (Figure 1).”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [6] Le Quéré, C. et al. Global carbon budget 2018. Earth Syst. Sci. Data 10, 2141–2194 (2018).
Not checked in the free run.
- Findingown data
In Europe, ERW could aid significant decarbonisation of France and Spain (up to approximately 40%).
“In Europe, ERW could aid significant decarbonisation of France and Spain (up to approximately 40%), and to a lesser extent Poland, Italy and Germany (all ~10%) (Figure 2).”
Quote in the paperSubstantial claim - Findingcitation
ERW has a similar potential to that of other CDR strategies estimated for 2050, including BECCS (0.5-5 Gt CO2 yr -1), DAC (0.5-5), biochar (0.5-2), SOC (0.5-5), and afforestation/reforestation (0.5-3.6).
“In the context of our CDR targets, ERW has a similar potential to that of other CDR strategies 23 estimated for 2050, including bio-energy with carbon capture and storage (BECCS), widely adopted in IPCC future scenarios (0.5-5 Gt CO2 yr -1 ), direct air carbon capture and storage (DAC) (0.5-5 Gt CO2 yr -1 ), biochar (0.5 to 2 Gt CO2 yr -1 ), soil organic carbon (SOC) sequestration (0.5-5 Gt CO2 yr”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
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- Findingcitation
Our ERW CDR range is comparable with large-scale implementation of BECCS in USA by 2040 (0.3-0.6 Gt CO2 yr -1), as constrained by biomass productivity, location and capacity of CO2 storage sites.
“For example, our ERW CDR range is comparable with large-scale implementation of BECCS in USA by 2040 (0.3-0.6 Gt CO2 yr -1 ), as constrained by biomass productivity, location and capacity of CO2 storage sites 24 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [24] Baik, E. et al. Geospatial analysis of near-term potential for carbon-negative bioenergy in the United States. Proc. Natl Acad. Sci. USA 115, 3290–3295 (2018). source
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- Findingown data
China may be able to augment its pledged 2030 NDCs by ~5-10% through ERW with agricultural lands.
“Results show that China may be able to augment its pledged 2030 NDCs by ~5-10%, with similar gains for the USA, which has opted-out of the Paris agreement.”
Quote in the paperSubstantial claim - Findingcitation
The top three European countries with highest CDR potential are also the largest European emitters of CO2 from fossil fuels (Germany, Spain and Poland).
“the top three European countries with highest CDR potential are also the largest European emitters of CO2 from fossil fuels (Germany, Spain and Poland) 6 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [6] Le Quéré, C. et al. Global carbon budget 2018. Earth Syst. Sci. Data 10, 2141–2194 (2018).
Not checked in the free run.
- Findingown data
The USA may be able to augment its pledged 2030 NDCs by ~5-10% through ERW with agricultural lands.
“Results show that China may be able to augment its pledged 2030 NDCs by ~5-10%, with similar gains for the USA, which has opted-out of the Paris agreement.”
Quote in the paperSubstantial claim - Findingown data
India may be able to augment its pledged 2030 NDCs by 40% of its current pledged emissions through ERW.
“For India, the gain rises to 40% of its current pledged emissions, and Brazil may be able to offset 100% of its pledged 2030 CO2 emissions plus some fraction of those from other countries (Figure 2).”
Quote in the paperSubstantial claim - Findingown data
Other countries outside Europe considered in the analysis (Indonesia, Canada, Mexico) may be able to augment their NDCs by up to 30% through ERW.
“Other countries outside Europe considered in our analysis (Indonesia, Canada, Mexico) may be able to augment their NDCs by up to 30% (Figure 2).”
Quote in the paperSubstantial claim - Findingown data
Our geospatial analyses define a new technical potential CDR range for those nations with high capacity for ERW deployment on cropland.
“Our geospatial analyses define a new technical potential CDR range for those nations with high capacity for ERW deployment on cropland (Figure 1; SI figs.S13-S15).”
Quote in the paperSubstantial claim - Findingcitation
China is the exception because its large increase in low carbon energy usage projected under the 2°C scenario allows net CDR to rise by substantially reducing secondary CO2 emissions from logistical operations.
“China is the exception because its large increase in low carbon energy usage projected under the 2°C scenario 5 allows net CDR to rise by substantially reducing secondary CO2 emissions from logistical operations (Figure 1).”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [5] Mercure, J.-F. et al. Macroeconomic impact of stranded fossil fuel assests. Nat. Clim. Chang. 8, 588–593 (2018). source
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- Findingreasoning
Overall trends in national CDR curves are relatively insensitive to the choice of energy scenario.
“Overall trends in national CDR curves are relatively insensitive to the choice of energy scenario.”
Quote in the paperNot a substantial claim - Findingnone given§ The potential for large-scale CO 2 removal via rock weathering on croplands
These targets and costs are robust regardless of future energy policies.
“These targets and costs are robust regardless of future energy policies.”
Quote in the paperNot a substantial claim - Findingown data
Our ERW scenarios correspond to an aggregate CDR of 25-100 Gt CO2 if sustained over 5 decades.
“Our ERW scenarios (Table 1) correspond to an aggregate CDR of 25-100 Gt CO2 if sustained over 5 decades.”
Quote in the paperSubstantial claim - Findingcitation
The top five European nations with the highest net CDR potential could offset 30% of the EU27's current emissions.
“The top five European nations with the highest net CDR potential could offset 30% of the EU27's current emissions”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [6] Le Quéré, C. et al. Global carbon budget 2018. Earth Syst. Sci. Data 10, 2141–2194 (2018).
Not checked in the free run.
- Findingown data
Unit costs increase when cropland area exceeds the optimal fraction.
“Costs per t CO2 removed are generally within this projected carbon price range in all nations, but unit costs increase when cropland area exceeds the optimal fraction, because the efficiency of weathering and CDR falls (Figure 3; Table 1).”
Quote in the paperSubstantial claim - Findingown data
In Europe, ERW could aid decarbonisation of Poland, Italy and Germany (all ~10%).
“In Europe, ERW could aid significant decarbonisation of France and Spain (up to approximately 40%), and to a lesser extent Poland, Italy and Germany (all ~10%) (Figure 2).”
Quote in the paperSubstantial claim - Findingown data
Average costs in USA ($160-180 t-1 CO2), Canada and European nations ($160-190 t-1 CO2) are almost 50% higher than those in China, India, Mexico, Indonesia, and Brazil ($55-120 t-1 CO2).
“Average costs in USA ($160-180 t -1 CO2), Canada and European nations ($160-190 t -1 CO2) are almost 50% higher than those in China, India, Mexico, Indonesia, and Brazil ($55-120 t -1 CO2).”
Quote in the paperSubstantial claim - Findingown data
Costs per t CO2 removed are generally within the projected carbon price range in all nations.
“Costs per t CO2 removed are generally within this projected carbon price range in all nations, but unit costs increase when cropland area exceeds the optimal fraction, because the efficiency of weathering and CDR falls (Figure 3; Table 1).”
Quote in the paperSubstantial claim - Findingreasoning
The per capita annual cost of achieving zero net emissions falls substantially for citizens in Brazil ($300), Indonesia ($103) and India ($135).
“Costs fall substantially for citizens in Brazil ($300), Indonesia ($103) and India ($135) (Table 1).”
Quote in the paperNot a substantial claim - Findingown data
National demand for crushed silicate rock is contingent on extent of ERW deployment.
“National demand for crushed silicate rock is contingent on extent of ERW deployment (Extended Data Fig. 5).”
Quote in the paperNot a substantial claim - Findingcitation
Our analysis identifies engineering challenges if ERW were to be scaled-up to help meet ambitious CDR targets as part of a wider portfolio of options.
“Our analysis identifies engineering challenges if ERW were to be scaled-up to help meet ambitious CDR targets as part of a wider portfolio of options 1,7,11,12 .”
Quote in the paperSubstantial claim0 of 4 sources checked- cites [1] Intergovernmental Panel on Climate Change (IPCC). Global Warming Of 1.5 °C. An IPCC Special Report on the Impacts of Global Warming of 1.5 °C Above Pre-Industrial Levels and Related Global Greenhouse Gas Emission Pathways (World Meteorological Organization, 2018).
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- cites [7] United Nations Environment Programme The Emissions Gap Report 2018 (United Nations Environment Programme, 2018).
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- cites [11] The Royal Society Greenhouse Gas Removal Technologies (The Royal Society, 2018).
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- cites [12] Pacala, S. et al. Negative Emissions Technologies And Reliable Sequestration (National Academy of Sciences, 2018).
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- Findingcitation
For average ocean temperature (17 °C), salinity (35%) and an RCP8.5 2050 dissolved pCO2 of 600 μatm, the CO2 removal efficiency is 0.86, i.e., 0.86 mole of CO2 removal per mole of monovalent cation and 1.72 mol of CO2 removed per mol of divalent cation added to the oceans.
“We calculate ƞ for average ocean temperature (17 °C), salinity (35%) and an RCP8.5 2050 dissolved pCO2 of 600 µatm, giving ƞ = 0.86, i.e., 0.86 mole of CO2 removal per mole of monovalent cation and 1.72 mol of CO2 removed per mol of divalent cation added to the oceans 20 .”
- Also stated in: § 2.1 Carbon dioxide removal. · plain
“We calculate ƞ for average ocean temperature (17 °C), salinity (35%) and an RCP8.5 2050 dissolved pCO2 of 600 µatm, giving ƞ = 0.86, i.e., 0.86 mole of CO2 removal per mole of monovalent cation and 1.72 mol of CO2 removed per mol of divalent cation added to the oceans 23 .”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [20] Smith, P. et al. Land-based options for greenhouse gas removal and their impacts on ecosystem services and the sustainable development goals. Annu. Rev. Environ. Res. 44, 255–286 (2019). source
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- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
Not checked in the free run.
- The authors state this as an assumption: Weathering products liberated from primary minerals are assumed to subsequently reach the surface ocean via continental runoff.
- Also stated in: § 2.1 Carbon dioxide removal. · plain
- Findingown data
The simplified mass transfer inhibition term in equations 1-3 successfully described the same kinetic behaviour calculated by the RTM.
“We demonstrate with this approach that the simplified mass transfer inhibition term in equations 1-3 successfully described the same kinetic behaviour calculated by the RTM (Figs.S10-S12).”
Quote in the paperSubstantial claim - Findingown data
For the basalts considered and under the soil conditions simulated, labradorite was the only mineral constituent that exhibited notable chemical inhibition.
“For the basalts we considered, and under the soil conditions simulated, labradorite was the only mineral constituent that exhibited notable chemical inhibition.”
Quote in the paperNot a substantial claim - Findingown data
Allowing formation of either secondary clay mineral accelerated dissolution of basaltic minerals through suppression of Al ion activity in solution resulting in less kinetic inhibition of the dissolution reactions.
“Allowing formation of either secondary clay mineral accelerated dissolution of basaltic minerals through suppression of Al ion activity in solution resulting in less kinetic inhibition of the dissolution reactions (Fig. S8, S9).”
Quote in the paperSubstantial claim - Findingown data
When affinity effects for primary minerals are neglected, secondary mineral accumulation is more rapid.
“These results show that when affinity effects for primary minerals are neglected, that secondary mineral accumulation is more rapid.”
- Also stated in: § Capital · plain
“These results show that when affinity effects for primary minerals are neglected, that secondary mineral accumulation is more rapid.”
Quote in the paperNot a substantial claim - Also stated in: § Capital · plain
- Findingnone given
Uncertainty in net CDR increases as ERW deploys onto croplands occupying a wider range of environmental conditions.
“Uncertainty in net CDR increases as ERW deploys onto croplands occupying a wider range of environmental conditions.”
Quote in the paperNot a substantial claim - Findingreasoning
The chemical affinity effect is greatest during the first 100 days, especially under a low flow rate (200 mm yr-1), because there is little dilution of the weathered products, resulting in higher pore water concentrations exerting a stronger affinity effect.
“This is greatest during the first 100 days, especially under a low flow rate (200 mm yr -1 top panels) because there is little dilution of the weathered products, resulting in higher pore water concentrations exerting a stronger affinity effect.”
Quote in the paperNot a substantial claim - Findingown data
Under the 2°C energy policy scenario, secondary CO2 emissions generally drop for most nations as they transition to low carbon energy sources in 2050 and implement negative emissions.
“Under the 2°C energy policy scenario, (c) and (d), secondary CO2 emisssion generally drop for most nations as they transition to low carbon energy sources in 2050 and implement negative emissions.”
Quote in the paperNot a substantial claim - Findingown data
Comparison shows close similarities between the simulated changes in pH, alkalinity flux, formation of pedogenic carbonate and efficiency of CO2 removal for the RTM and the performance model.
“Comparison shows the close similarities between the simulated changes in pH, alkalinity flux (Ca 2+ + Mg 2+ + Na + + K + ), formation of pedogenic carbonate (CaCO3) and efficiency of CO2 removal (RCO2) for the reactive transport model ('RTM') and the performance model ('simple').”
Quote in the paperSubstantial claim - Findingnone given
Cumulative silicate demand curves are the same irrespective of energy policy scenario.
“Curves are the same irrespective of energy policy scenario.”
Quote in the paperNot a substantial claim - Findingown data
The results show close correspondence between the RTM and the calibrated performance model across all three flow regimes for alkali basalt.
“The results show close correspondence between models across all three flow regimes.”
Quote in the paperNot a substantial claim - Findingown data
Agreement between modelling approaches holds across a wide range of flows.
“Agreement between modelling approaches holds across a wide range of flows.”
Quote in the paperSubstantial claim - Findingown data
Under the 2°C scenario, low carbon energy production used for rock grinding allows a simulated reduction in p80s for the same cropland fractional area.
“Under the 2°C scenario, low carbon energy production used for rock ginding allows a simulated reduction in p80s for the same cropland fractional area.”
Quote in the paperNot a substantial claim - Findingown data
Only labradorite in these basalts exhibits noticeable effects of chemical affinity.
“Only labradorite (green line) in these basalts exhibits noticeable effects.”
Quote in the paperNot a substantial claim - Findingown data
We show close correspondence between the results of the RTM with full chemical speciation and our simplified performance model for the weathering of either type of basalt (tholeiitic and alkaline) being considered.
“We show close correspondence between the results of the RTM with full chemical speciation and our simplified performance model for the weathering of either type of basalt (tholeiitic and alkaline) being considered (Figs S10, S11).”
Quote in the paperSubstantial claim - Findingown data
The two approaches (RTM and performance model) give similar patterns of alkalinity release, pedogenic carbonate formation and CO2 removal to underpin our modelling approach.
“As a result, the two approaches (RTM and performance model), give similar patterns of alkalinity release, pedogenic carbonate formation and CO2 removal (Fig. S12) to underpin our modelling approach.”
Quote in the paperSubstantial claim - Findingreasoning
Kfeldspar also exerts a minor affinity effect but is present in such low concentrations that its influence on the basalt-porewater system can be considered to be negligible.
“Kfeldspar also exerts a minor affinity effect but is present in such low concentrations that its influence on the basalt-porewater system can be considered to be negligible.”
Quote in the paperNot a substantial claim - Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplands
Even the most ambitious emission phase-outs fail to achieve the United Nations Framework Convention on Climate Change Paris Agreement targets for limiting global warming without the help of massive atmospheric Carbon Dioxide Removal (CDR).
“Even the most ambitious emission phase-outs 9,10 fail to achieve the United Nations Framework Convention on Climate Change Paris Agreement targets for limiting global warming without the help of massive atmospheric Carbon Dioxide Removal (CDR).”
Quote in the paperSubstantial claim0 of 2 sources checked - Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplands
Depending on soil type, atmospheric CO2-derived dissolved inorganic carbon may also be sequestered through the formation of soil carbonate minerals, which reduces the efficiency of carbon sequestration by ~50%.
“Depending on soil type, atmospheric CO2-derived dissolved inorganic carbon may also be sequestered through the formation of soil carbonate minerals, which reduces the efficiency of carbon sequestration by ~50% 19 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [19] Renforth, P. & Henderson, G. Assessing ocean alkalinity for carbon sequestration. Rev. Geophys. 55, 636–674 (2017). source
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- Interpretationreasoning
Co-deployment of ERW and SOC sequestration at large-scale might contribute substantially to the 5 Gt CO2 yr -1 carbon removal target suggested in decarbonization scenarios for 2050.
“Co-deployment of ERW and SOC sequestration at large-scale might, therefore, contribute substantially to the 5 Gt CO2 yr -1 carbon removal target suggested in decarbonization scenarios 10 for 2050.”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [10] Rockström, J. et al. A roadmap for rapid decarbonisation. Science 355, 1269–1271 (2017). source
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- Interpretationreasoning
This would save up to 10% of the remaining cumulative carbon emission budget (~900 Gt CO2) that gives a likely chance of limiting global warming to less than 2°C above the pre-industrial average surface temperature.
“This would save up to 10% of the remaining cumulative carbon emission budget (~900 Gt CO2) that gives a likely chance of limiting global warming to less than 2°C above the pre-industrial average surface temperature 10 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [10] Rockström, J. et al. A roadmap for rapid decarbonisation. Science 355, 1269–1271 (2017). source
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- Premisecitation
Amendment of acidic organic-rich soils with silicate minerals, and resultant pH increase, had no effect on respiratory CO2 fluxes.
“Compatibility of ERW and SOC sequestration may be realistic given that amendment of acidic organic-rich soils with silicate minerals, and resultant pH increase, had no effect on respiratory CO2 fluxes 28,29 , contrary to concerns that increased soil pH may accelerate organic matter decomposition 30 .”
Quote in the paperSubstantial claim0 of 3 sources checked- cites [28] Groffman, P. M. et al. Calcium additions and microbial nitrogen cycle processes in a northern hardwood forest. Ecosystems 9, 1289–1305 (2006). source
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- cites [29] Dietzen, C., Harrison, R. & Michelsen-Correa, S. Effectiveness of enhanced mineral weathering as a carbon sequestration tool and alternative to agricultural lime: an incubation experiment. Int. J. Greenhouse Gas Control 74, 251–258 (2018). source
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- cites [30] Smith, P., Haszeldine, R. S. & Smith, S. M. Preliminary assessment of the potential for, and limitations to, terrestrial negative emissions technologies in the UK. Environ. Sci. Process. Impacts 18, 1400–1405 (2016). source
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- Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplands
These weathering products are transported via land surface runoff to the oceans with a storage lifetime exceeding 100,000 years.
“These weathering products are transported via land surface runoff to the oceans with a storage lifetime exceeding 100,000 years 19 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [19] Renforth, P. & Henderson, G. Assessing ocean alkalinity for carbon sequestration. Rev. Geophys. 55, 636–674 (2017). source
Not checked in the free run.
- Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplands
Most studies project extraction goals later this century of at least 10 Gt CO2 yr -1.
“Extraction goals 1,7,9,10 later this century in most studies are on the order of at least 10 Gt CO2 yr -1”
Quote in the paperNot a substantial claim0 of 4 sources checked- cites [1] Intergovernmental Panel on Climate Change (IPCC). Global Warming Of 1.5 °C. An IPCC Special Report on the Impacts of Global Warming of 1.5 °C Above Pre-Industrial Levels and Related Global Greenhouse Gas Emission Pathways (World Meteorological Organization, 2018).
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- cites [7] United Nations Environment Programme The Emissions Gap Report 2018 (United Nations Environment Programme, 2018).
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- cites [9] Hansen, J. et al. Young people’s burden: requirement of negative CO2 emissions. Earth Syst. Dyn 8, 577–616 (2017). source
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- cites [10] Rockström, J. et al. A roadmap for rapid decarbonisation. Science 355, 1269–1271 (2017). source
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- Interpretationcitation
Co-deployment of ERW with feedstock crops for BECCS and biochar could enhance the feasibility and carbon sequestration potential of these strategies.
“Co-deployment of ERW with feedstock crops for BECCS and biochar could enhance the feasibility and carbon sequestration potential of these strategies 4,26 .”
Quote in the paperNot a substantial claim0 of 2 sources checked- cites [4] Beerling, D. J. et al. Farming with crops and rocks to address global climate, food and soil security. Nat. Plants 4, 138–147 (2018). source
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- cites [26] Amann, T. & Hartmann, J. Ideas and perspectives: synergies from co-deployment of negative emissions technologies. Biogeosciences 16, 2949–2960 (2019). source
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- Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplands
Logistical infrastructure to apply basaltic rock dust to managed croplands already exists due to the common need to apply crushed limestone to reverse soil acidification from intensive cropping.
“Logistical infrastructure to apply basaltic rock dust to managed croplands already exists due to the common need to apply crushed limestone to reverse soil acidification from intensive cropping [2][3][4] .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [2][3][4]
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- Interpretationcitation
Innovative ERW practices via soil amendments with targeted silicate minerals could help rebuild rapidly deteriorating agricultural soils on which over six billion people depend directly for food.
“More broadly, innovative ERW practices via soil amendments with targeted silicate minerals could help rebuild rapidly deteriorating agricultural soils on which over six billion people depend directly for food 48 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [48] United Nations Global Land Outlook 1st edn (United Nations Convention to Combat Desertification, 2017).
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- Premisecitation
Intensification of food production across 24 million hectares of productive agricultural land in South Asia and China is creating acidified, desilicated soils exhausted in plant nutrients (potassium, zinc and available phosphorus) that limit yields.
“Intensification of food production across 24 million hectares of productive agricultural land in South Asia and China, for example, is creating acidified, desilicated soils exhausted in plant nutrients (potassium, zinc and available phosphorus) that limit yields 45 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [45] Savant, N. K., Datnoff, L. E. & Snyder, G. H. Depletion of plant-available silicon in soils: a possible cause of declining rice yields. Commun. Soil Sci. Plant Anal. 28, 1245–1252 (1997). source
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- Interpretationnone given
ERW cannot offset all fossil fuel emissions.
“ERW cannot offset all fossil fuel emissions, but using its cost as a guide, the per capita annual cost of achieving zero net emissions, a goal for decarbonisation, would be highest for Canada ($3004), the USA ($2780), China ($832) and EU28 nations ($1288).”
Quote in the paperNot a substantial claim - Interpretationreasoning
A carbon price of $100-150 t-1 CO2 would make ERW an economically attractive option for fast-growing nations such as India, China, Indonesia, Brazil and Mexico given their estimated CO2 extraction costs of ~$75-100 t-1 CO2.
“It would make ERW an economically attractive option for fastgrowing nations, such as India, China, Indonesia, Brazil and Mexico given their estimated CO2 extraction costs of ~ $75-100 t -1 CO2 (Figure 3).”
Quote in the paperSubstantial claim - Interpretationreasoning
A carbon price of $100-150 t-1 CO2 would cover most of the ERW costs for the key nations reported here.
“A carbon price of $100-150 t -1 CO2 would cover most of the ERW costs for the key nations reported here.”
Quote in the paperSubstantial claim - Interpretationcitation
Requirement for mining may be further reduced by utilizing artificial silicate by-products from industrial processes, including calcium-rich silicates produced by iron and steel manufacturing (slags) with a long history of agricultural usage.
“Requirement for mining may be further reduced by utilizing artificial silicate by-products from industrial processes 37,38 , including calcium-rich silicates produced by iron and steel manufacturing (slags) with a long history of agricultural usage 4,39 .”
Quote in the paperNot a substantial claim0 of 4 sources checked- cites [37] Renforth, P. et al. Silicate production and availability for mineral carbonation. Environ. Sci. Technol. 45, 2035–2041 (2011). source
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- cites [38] Renforth, P. The negative emission potential of alkaline materials. Nat. Commun. 10, 1401 (2019). source
Not checked in the free run.
- cites [4] Beerling, D. J. et al. Farming with crops and rocks to address global climate, food and soil security. Nat. Plants 4, 138–147 (2018). source
Not checked in the free run.
- cites [39] Tubana, B. S., Babu, T. & Datnoff, L. E. A review of silicon in soils and plants and its role in US agriculture: history and future perspectives. Soil Sci. 181, 393–411 (2016). source
Not checked in the free run.
- Interpretationcitation
ERW may therefore also have a role in remediation of toxic metal contaminated soils and sediments across 20 million hectares of cultivated land in southern China and elsewhere.
“ERW may therefore also have a role in remediation of toxic metal contaminated soils and sediments across 20 million hectares of cultivated land in southern China and elsewhere 47 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [47] Chen, J. Rapid urbanization in China: a real challenge to soil protection and food security. Catena 69, 1–15 (2007). source
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- Premisecitation
Undertaking ERW practices with these materials addresses a critical need to fertilise soils with silica and other nutrients lost by harvesting that gradually depletes plant-available pools.
“Undertaking ERW practices with these materials addresses a critical need to fertilise soils with silica and other nutrients lost by harvesting that gradually depletes plant-available pools 39 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [39] Tubana, B. S., Babu, T. & Datnoff, L. E. A review of silicon in soils and plants and its role in US agriculture: history and future perspectives. Soil Sci. 181, 393–411 (2016). source
Not checked in the free run.
- Interpretationcitation
ERW has a role to play in compensating for residual carbon emissions from sectors recognized as difficult to decarbonize, such as aviation, shipping, and agriculture.
“ERW, therefore, has a role to play in compensating for residual carbon emissions from sectors recognized as being difficult to decarbonize, e.g., transportation by aviation, shipping, and agriculture 1,11 .”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [1] Intergovernmental Panel on Climate Change (IPCC). Global Warming Of 1.5 °C. An IPCC Special Report on the Impacts of Global Warming of 1.5 °C Above Pre-Industrial Levels and Related Global Greenhouse Gas Emission Pathways (World Meteorological Organization, 2018).
Not checked in the free run.
- cites [11] The Royal Society Greenhouse Gas Removal Technologies (The Royal Society, 2018).
Not checked in the free run.
- Interpretationcitation
Net cost of ERW may be lower if rock dust is used as a fertilizer in organic agriculture because it adds economic value by improving soil health, fertility and ecosystem services.
“Net cost of ERW may be lower if rock dust is used as a fertilizer in organic agriculture, which currently occupies 57.8 million hectares, because it adds economic value by improving soil health, fertility and ecosystem services 35 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [35] Crowder, D. W. & Reganold, J. P. Financial competitiveness of organic agriculture on a global scale. Proc. Natl Acad. Sci. USA 112, 7611–7616 (2015). source
Not checked in the free run.
- Premisecitation
Afforestation/reforestation and practices that increase soil carbon in natural ecosystems, including wetland restoration, have lower estimated costs (<$100 t-1 CO2).
“Afforestation/reforestation and practices that increase soil carbon in natural ecosystems, including wetland restoration, have lower estimated costs (<$100 t -1 CO2) 23 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
Not checked in the free run.
- Premisecitation
Carbon price is forecast by the World Bank to reach $100-150 t-1 CO2 by 2050.
“Carbon price is forecast by the World Bank 11 to reach $100-150 t -1 CO2 by 2050.”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [11] The Royal Society Greenhouse Gas Removal Technologies (The Royal Society, 2018).
Not checked in the free run.
- Interpretationreasoning
The difference in average ERW costs between nations largely reflects labour, diesel and electricity costs.
“The difference largely reflects labour, diesel and electricity costs.”
Quote in the paperNot a substantial claim - Interpretationown data
The increase in unit costs when cropland area exceeds the optimal fraction is because the efficiency of weathering and CDR falls.
“Costs per t CO2 removed are generally within this projected carbon price range in all nations, but unit costs increase when cropland area exceeds the optimal fraction, because the efficiency of weathering and CDR falls (Figure 3; Table 1).”
Quote in the paperSubstantial claim - Interpretationreasoning
Bulk silicate production of China and India could meet the demand for ERW with large CDR potential.
“Thus, bulk silicate production of these two nations could meet the demand for ERW with large CDR potential (Table 1).”
Quote in the paperSubstantial claim - Premisecitation
The reaction rate of a mineral undergoing dissolution in soil is governed by the law of kinetic mass action and is proportional to the moles of reactive sites on the mineral surface in contact with the reacting aqueous solution.
“The reaction rate of a mineral undergoing dissolution in soil is governed by the law of kinetic mass action and is proportional to the moles of reactive sites on the mineral surface in contact with the reacting aqueous solution 14 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [14] Schuiling, R. D. & Krijgsman, P. Enhanced weathering: an effective and cheap tool to sequester CO2. Clim. Change 74, 349–354 (2006). source
Not checked in the free run.
- Premiseown data
Monovalent and divalent base cations are released from basaltic minerals by dissolution based on stoichiometry.
“Monovalent and divalent base cations are released from basaltic minerals by dissolution based on stoichiometry (SI Table S2).”
- Also stated in: § 2.1 Carbon dioxide removal. · plain
“Monovalent and divalent base cations are released from basaltic minerals by dissolution based on stoichiometry (Table S2).”
Quote in the paperSubstantial claim0 of 2 sources checked- cites SI Table S2
Not checked in the free run.
- cites Table S2
Not checked in the free run.
- Also stated in: § 2.1 Carbon dioxide removal. · plain
- Study design and conductreasoning
Together with the chemical affinity effects accounted for in our model, we constrain some of the systematic errors embedded in prior ERW assessments.
“Together with the chemical affinity effects accounted for in our model, we constrain some of the systematic errors embedded in prior ERW assessments [15][16][17]21,22 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [15][16][17]21,22
Not checked in the free run.
- Study design and conductown data
This version of the model (equation 7) is well-validated against flask-dissolution experiments.
“This version of the model (equation 7) is well-validated against flask-dissolution experiments (Fig. S3).”
Quote in the paperSubstantial claim - Premisecitation
SSP2 potentially represents the largest material production pathway, as other SSPs forecast lower consumption or economic growth producing 30-50% less material globally.
“SSP2 potentially represents the largest material production pathway, as other SSPs forecast lower consumption or economic growth producing 30-50% less material globally.”
- Also stated in: § 2.4 Forecasting bulk silicate waste production. · hedged
“SSP2 potentially represents the largest material production pathway, as other SSPs forecast lower consumption or economic growth producing 30-50% less material globally.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [40] Washbourne, C.-L. et al. Rapid removal of atmospheric CO2 in urban soils. Environ. Sci. Technol. 49, 5434–5440 (2015). source
Not checked in the free run.
- Also stated in: § 2.4 Forecasting bulk silicate waste production. · hedged
- Premisecitation
Deployment of any CDR strategy is inhibited by concern that it may erode society's perception of the climate threat and the urgency of mitigation measures.
“Deployment of any CDR strategy is inhibited by concern that it may erode society's perception of the climate threat and the urgency of mitigation measures 54 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [54] Cox, E., Pidgeon, N. F., Spence, E. M. & Thomas, G. Blurred lines: the ethics and policy of greenhouse gas removal at scale. Front. Environ. Sci. https://doi.org/10.3389/fenvs.2018.00038 (2018). source
Not checked in the free run.
- Premisecitation
Ocean carbonate chemistry reduces the efficiency of CO2 removal to an extent depending on ocean temperature, salinity and the surface ocean dissolved CO2 concentration.
“However, ocean carbonate chemistry reduces the efficiency of CO2 removal (ƞ) to an extent depending on ocean temperature, salinity and the surface ocean dissolved CO2 concentration.”
- Also stated in: § 2.1 Carbon dioxide removal. · plain
“However, ocean carbonate chemistry reduces the efficiency of CO2 removal (ƞ) to an extent depending on ocean temperature, salinity and the surface ocean dissolved CO2 concentration.”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
Not checked in the free run.
- Also stated in: § 2.1 Carbon dioxide removal. · plain
- Interpretationcitation
Our approach improves on prior analyses that assumed a fixed radius between rock dust source and site of application.
“Our approach improves on prior analyses, which assumed a fixed radius between rock dust source and site of application 73 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [73] Moosdorf, N., Renforth, P. & Hartmann, J. Carbon dioxide efficiency of terrestrial weathering. Environ. Sci. Technol. 48, 4809–4816 (2014). source
Not checked in the free run.
- Premisecitation
Rock grinding to reduce particle size and maximise CDR is the primary energy consuming operation in ERW.
“Rock grinding to reduce particle size and maximise CDR is the primary energy consuming operation in ERW 22,23,73 .”
Quote in the paperNot a substantial claim0 of 3 sources checked- cites [22] Strefler, J. et al. Potential and costs of carbon dioxide removal by enhanced weathering of rocks. Environ. Res. Lett. 13, 034010 (2018). source
Not checked in the free run.
- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
Not checked in the free run.
- cites [73] Moosdorf, N., Renforth, P. & Hartmann, J. Carbon dioxide efficiency of terrestrial weathering. Environ. Sci. Technol. 48, 4809–4816 (2014). source
Not checked in the free run.
- Premisecitation
Extrapolation of laboratory weathering rates to the field scale is a recognized potential source of uncertainty in calculated CDR rates by ERW.
“Extrapolation of laboratory weathering rates to the field scale is a recognized potential source of uncertainty in calculated CDR rates by ERW [2][3][4][22][23][24] .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [2][3][4][22][23][24]
Not checked in the free run.
- Interpretationreasoning
Our analysis represents the first technoeconomic assessment in which detailed ERW carbon and economic costs vary within and between nations and account for socio-technical uncertainties in energy production.
“Our analysis thus represents the first technoeconomic assessment in which detailed ERW carbon and economic costs vary within and between nations and account for socio-technical uncertainties in energy production.”
Quote in the paperSubstantial claim - Premisecitation
The measured SSA of a granular material is typically much higher than estimates of the surface area by geometric models of particle shapes, due to surface topography and porosity effects.
“The measured SSA of a granular material is typically much higher than estimates of the surface area by geometric models of particle shapes, due to surface topography and porosity effects 15 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [15] Kohler, P., Hartmann, J. & Wolf-Gladrow, D. A. Geoengineering potential of artificially enhanced silicate weathering of olivine. Proc. Natl Acad. Sci. USA 107, 20228–20233 (2010). source
Not checked in the free run.
- Interpretationcitation
Using log-normal particle size distributions of basalt grains improves on the simplified case of a single mean particle diameter previously used in ERW calculations.
“This conceptualisation improves on the simplified case of a single mean particle diameter, previously used in ERW calculations [16][17][18]22,23 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [16][17][18]22,23
Not checked in the free run.
- Premisecitation
A baseline application rate of 40 t ha−1 yr−1 falls within the range of basalt amendments shown to improve crop production in field trials.
“Using this modelling framework, we analysed a baseline application rate of 40 t ha -1 yr -1 (equivalent to a <2 mm layer of rock powder distributed on croplands), which falls within the range of basalt amendments shown to improve crop production in field trials 4 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [4] Beerling, D. J. et al. Farming with crops and rocks to address global climate, food and soil security. Nat. Plants 4, 138–147 (2018). source
Not checked in the free run.
- Interpretationreasoning
CDR via pathway 1 potentially sequesters two moles of CO2 from the atmosphere per mole of divalent cation.
“CDR, via pathway 1, potentially sequesters two moles of CO2 from the atmosphere per mole of divalent cation.”
- Also stated in: § 2.1 Carbon dioxide removal. · hedged
“CDR, via pathway 1, potentially sequesters two moles of CO2 from the atmosphere per mole of divalent cation.”
Quote in the paperSubstantial claim- The authors state this as an assumption: Weathering products liberated from primary minerals are assumed to subsequently reach the surface ocean via continental runoff.
- Also stated in: § 2.1 Carbon dioxide removal. · hedged
- Premisecitation
Industrialized nations (e.g., Canada) consume up to ~2% of their total energy production on rock comminution processes.
“Industrialized nations (e.g., Canada) consume up to ~2% of their total energy production on rock comminution (crushing and grinding) processes 77 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [77] Tromans, D. Mineral comminution: energy efficiency considerations. Min. Eng. 21, 613–620 (2008). source
Not checked in the free run.
- Premisecitation
Between 2006-2014, 185 kg of blast furnace slag and 117 kg of steel slag was produced for every tonne of crude steel.
“Between 2006-2014, 185 kg of blast furnace slag and 117 kg of steel slag was produced for every tonne of crude steel 87 .”
- Also stated in: § 2.4 Forecasting bulk silicate waste production. · plain
“Between 2006-2014, 185 kg of blast furnace slag and 117 kg of steel slag was produced for every tonne of crude steel 42 .”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [87] U.S. Geological Survey. Mineral Commodity Summaries 2006 (US Geological Survey, 2006).
Not checked in the free run.
- cites [42] Haynes, R. J., Belyaeva, O. N. & Kingston, G. Evaluation of industrial waste sources of fertilizer silicon using chemical extractions and plant uptake. J. Plant Nutr. Soil Sci. 176, 238–248 (2013). source
Not checked in the free run.
- Also stated in: § 2.4 Forecasting bulk silicate waste production. · plain
- Premisecitation
Current state-of-knowledge precludes a detailed treatment of the role of surface passivation by formation of amorphous silica-rich surfaces for basalt grains added to agricultural soils.
“Current state-of-knowledge 52 precludes a detailed treatment of the role of surface passivation by formation of amorphous silica-rich surfaces for basalt grains added to agricultural soils.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [52] Daval, D., Calvarusa, C., Guyut, F. & Turpault, M.-P. Time-dependent feldspar dissolution rates resulting from surface passivation: experimental evidence and geochemical implications. Earth Planet. Sci. Lett. 498, 226–236 (2018). source
Not checked in the free run.
- Rests on an assumption: Surface passivation occurs as weathering proceeds, creating leached layers and relatively stable secondary minerals, which potentially inhibit the mass transfer kinetics of elements from the dissolving surfaces of primary minerals.
- Premisecitation
Mechanical comminution produces an approximately log-normal particle size distribution that varies with different grinding and milling technologies.
“However, mechanical comminution produces an approximately log-normal psd 16 that varies with different grinding and milling technologies.”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [16] Hartmann, J. et al. Enhanced chemical weathering as a geoengineering strategy to reduce atmospheric carbon dioxide, supply nutrients, and mitigate ocean acidification. Rev. Geophys. 51, 113–149 (2013). source
Not checked in the free run.
- Premisecitation
Even without separating out cement waste from other materials, very little of the leachate contained elemental concentrations above typical water quality standard ranges.
“Even without separating out cement waste from other materials 59 , very little of the leachate contained elemental concentrations above typical water quality standard ranges [60][61][62] .”
Quote in the paperNot a substantial claim0 of 2 sources checked- cites [59] Siebert, S. & Doll, P. Quantifying blue and green virtual water contents in global crop production as well as potential production losses without irrigation. J. Hydrol. 384, 198–217 (2010). source
Not checked in the free run.
- cites [60][61][62]
Not checked in the free run.
- Premisecitation
For the USA, mining cost is 6.99 $ t-1 as obtained from prior analysis.
“For the USA, mining cost is 6.99 $ t -1 as obtained from prior analysis 22 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [22] Strefler, J. et al. Potential and costs of carbon dioxide removal by enhanced weathering of rocks. Environ. Res. Lett. 13, 034010 (2018). source
Not checked in the free run.
- Premisecitation
Industrialized nations (e.g., Canada) consume up to ~2% of their total energy production on rock comminution (crushing and grinding) processes.
“Industrialized nations (e.g., Canada) consume up to ~2% of their total energy production on rock comminution (crushing and grinding) processes 36 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [36] Bebbington, A. J. & Bury, J. T. Institutional challenges for mining and sustainability in Peru. Proc. Natl Acad. Sci. USA 106, 17296–17301 (2009). source
Not checked in the free run.
- Interpretationown data
Our approach, which does not explicitly account for the effects of secondary clay minerals on acceleration of primary mineral dissolution, is conservative with respect to calculating basalt dissolution.
“These results suggest that our approach, which does not explicitly account for the effects of secondary clay minerals on acceleration of primary mineral dissolution, is conservative with respect to calculating basalt dissolution.”
Quote in the paperSubstantial claim - Interpretationown data
Allowing kaolinite formation accelerates dissolution of labradorite and augite through suppression of Al ion activity in solution resulting in less kinetic inhibition of the dissolution reactions.
“Results indicate allowing kaolinite formation accelerates dissolution of labradorite (dashed vs solid green lines) and augite (dashed vs solid red lines) through suppression of Al ion activity in solution resulting in less kinetic inhibition of the dissolution reactions.”
Quote in the paperNot a substantial claim - Interpretationown data
Allowing montmorillonite formation accelerates dissolution of labradorite and augite through suppression of Al ion activity in solution resulting in less kinetic inhibition of the dissolution reactions.
“Results indicate allowing montmorillonite formation accelerates dissolution of labradorite (dashed vs solid green lines) and augite (dashed vs solid red lines) through suppression of Al ion activity in solution resulting in less kinetic inhibition of the dissolution reactions.”
Quote in the paperNot a substantial claim - Study design and conductown data
The k-means clustering approximation proved robust with small error and bias when tested at low resolution due to small intra-class variability.
“Although the number of grid cells to be optimized is reduced by orders of magnitude during the classification, the approximation proved robust with small error and bias when tested at low resolution due to small intra-class variability.”
Quote in the paperSubstantial claim
- May combine two claims. 59
- Classified as probably not a substantial claim. 34
- The quote only partly states this claim. 3
May combine two claims.
FindingreasoningNational median CO2 removal curves typically show CDR capacity rising with increasing cropland area, with carbon removal by silicate soil amendment reaching a plateau or declining in the case of Canada.
“National median CO2 removal curves typically show CDR capacity rising with increasing cropland area, with carbon removal by silicate soil amendment reaching a plateau or declining in the case of Canada (Figure 1).”
Quote in the paperSubstantial claimMay combine two claims.
Findingown dataBrazil may be able to offset 100% of its pledged 2030 CO2 emissions plus some fraction of those from other countries through ERW.
“For India, the gain rises to 40% of its current pledged emissions, and Brazil may be able to offset 100% of its pledged 2030 CO2 emissions plus some fraction of those from other countries (Figure 2).”
Quote in the paperSubstantial claimMay combine two claims.
FindingreasoningEuropean countries have an order-of-magnitude lower CDR potential than China, USA, and India, mainly because of lower agricultural land area.
“European countries have an order-of-magnitude lower CDR potential than China, USA, and India, mainly because of lower agricultural land area.”
Quote in the paperNot a substantial claimMay combine two claims.
FindingreasoningIndonesia and Brazil, with CO2 emissions 10-20 times lower than the USA and China, have relatively high CDR potential due to extensive agricultural lands and climates suitable for high silicate rock weathering efficiency.
“Indonesia and Brazil, with CO2 emissions 10-20 times lower than the USA and China, have relatively high CDR potential due to extensive agricultural lands and climates suitable for high silicate rock weathering efficiency.”
Quote in the paperNot a substantial claimMay combine two claims.
FindingreasoningIndia's total energy production falls by ~40% with a transition to low carbon energy production in the 2°C scenario, lowering energy available for grinding basalt, and thus the potential for increased CDR by ERW.
“This contrasts with results for India, whose total energy production falls by ~40% with a transition to low carbon energy production in the 2 o C scenario, lowering energy available for grinding basalt, and thus the potential for increased CDR by ERW.”
Quote in the paperSubstantial claimMay combine two claims.
Findingown dataWithin our scenarios, the demand for basalt required for ERW rises with an increasing CDR target and scales with agricultural land area.
“Within our scenarios, the demand for basalt required for ERW rises with an increasing CDR target and scales with agricultural land area (Table 1).”
Quote in the paperSubstantial claimMay combine two claims.
FindingreasoningUsing ERW cost as a guide, the per capita annual cost of achieving zero net emissions would be highest for Canada ($3004), the USA ($2780), China ($832) and EU28 nations ($1288).
“ERW cannot offset all fossil fuel emissions, but using its cost as a guide, the per capita annual cost of achieving zero net emissions, a goal for decarbonisation, would be highest for Canada ($3004), the USA ($2780), China ($832) and EU28 nations ($1288).”
Quote in the paperNot a substantial claimMay combine two claims.
FindingcitationOur estimated ERW costs of carbon removal for nations are comparable to estimates summarized for BECCS ($100-200 t-1 CO2), DAC ($100-300 t-1 CO2), and biochar ($30-$120 t-1 CO2), but higher than estimates for SOC sequestration ($0-10 t-1 CO2).
“Our estimated ERW costs of carbon removal for nations are comparable to estimates summarized for BECCS ($100 to 200 t -1 CO2), DAC ($100-300 t -1 CO2), and biochar ($30-$120 t -1 CO2), but higher than estimates for SOC sequestration ($0-10 t -1 CO2) 23 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
Not checked in the free run.
May combine two claims.
Findingown dataBulk silicate production, linked to the construction and demolition sector, is modelled to increase substantially in all four nations, with China and India having combined production by 2060 of ~13 Gt yr-1.
“Bulk silicate production, linked to the construction and demolition sector, is modelled to increase substantially in all four nations, with China and India having combined production by 2060 of ~13 Gt yr -1 (Figure 4).”
Quote in the paperSubstantial claimMay combine two claims.
Findingown dataOur cost estimates based on current prices fall within the range of prior ERW assessments ($75-250 tCO2-1) while resolving differences among nations.
“Our cost estimates based on current prices fall within the range of prior ERW assessments ($75-250 tCO2 -1 ) [21][22][23] while resolving differences among nations (Figure 3; Table 1; SI figs.S16-S25; SI tables S13-S14).”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [21][22][23]
Not checked in the free run.
Probably not a substantial claim: may not pass S4 (based). May combine two claims.
Findingnone givenERW has potential for ancillary benefits by limiting coastal zone acidification and improving food and soil security.
“with potential for ancillary benefits by limiting coastal zone acidification and improving food and soil security”
Quote in the paperNot a substantial claimMay combine two claims.
FindingreasoningBasaltic minerals undergo dissolution at different rates, with some minerals continuing to undergo dissolution and capture CO2 after the first year of application.
“Basaltic minerals undergo dissolution at different rates, with some minerals continuing to undergo dissolution and capture CO2 after the first year of application.”
- Also stated in: § Extended · plain
“Basaltic minerals undergo dissolution at different rates, with some minerals continuing to undergo dissolution and capture CO2 after the first year of application.”
Quote in the paperSubstantial claim- Also stated in: § Extended · plain
May combine two claims.
FindingreasoningCarbon emissions per unit mass of ground rock depend on particle size, the CO2 emissions per kilowatt-hour of electricity generated from component energy sources, and the carbon costs of sourcing and transporting the silicate materials.
“Carbon emissions per unit mass of ground rock depend on particle size (Extended Data Fig. 10), the CO2 emissions per kilowatt-hour of electricity generated from component energy sources (fossil fuels, nuclear and renewables), as well as the carbon costs of sourcing and transporting the silicate materials.”
Quote in the paperSubstantial claimMay combine two claims.
Findingnone givenGrinding to finer particles requires greater energy and results in higher carbon emissions.
“Grinding to finer particles requires greater energy and results in higher carbon emissions.”
Quote in the paperSubstantial claimProbably not a substantial claim: may not pass S4 (based).
Findingnone givenERW estimated costs are comparable to current estimates for the intensive carbon removal technologies, BECCS and DAC.
“ERW estimated costs are comparable to current estimates for the intensive carbon removal technologies, BECCS and DAC”
Quote in the paperNot a substantial claimThe quote only partly states this claim.
Findingown dataThe results show close correspondence between the RTM and the calibrated performance model across all three flow regimes for tholeiitic basalt.
“The results show close correspondence between models across all three flow regimes.”
Quote in the paperNot a substantial claimMay combine two claims.
FindingreasoningAt the two higher flow rates, shorter residence times result in less solute accumulation within the soil profile and a weaker chemical affinity effect.
“At the two higher flow rates, shorter residence times result in less solute accumulation within the soil profile and a weaker chemical affinity effect.”
- Also stated in: § Capital · plain
“At the two higher flow rates, shorter residence times result in less solute accumulation within the soil profile and a weaker chemical affinity effect.”
Quote in the paperNot a substantial claim- Also stated in: § Capital · plain
May combine two claims.
Findingown dataWeathering inhibition appears negligible over the 1 year duration of soil weathering, other than for laboradorite, with the performance model realistically capturing the effects of chemical affinity.
“Weathering inhibition appears negligible over the 1 year duration of soil weathering, other than for laboradorite, with the performance model realistically capturing the effects of chemical affinity.”
Quote in the paperSubstantial claimMay combine two claims.
FindingreasoningLabradorite dissolves to completion after 365 days, and the results of the simulations that include and neglect affinity effects converge.
“Consequently, labradorite dissolves to completion after 365 days, and the results of the simulations that include and neglect affinity effects converge.”
- Also stated in: § Capital · plain
“Consequently, labradorite dissolves to completion after 365 days, and the results of the simulations that include and neglect affinity effects converge.”
Quote in the paperNot a substantial claim- Also stated in: § Capital · plain
May combine two claims.
Findingown dataKfeldspar exerts a minor affinity effect but is present in such low concentrations that its influence on the basalt-porewater system can be considered negligible.
“Kfeldspar also exerts a minor affinity effect but is present in such low concentrations that its influence on the basalt-porewater system can be considered to be negligible.”
Quote in the paperNot a substantial claimMay combine two claims.
FindingreasoningMining costs calculated using the method were 5.33, 4.44, 3.97, 4.88, 6.79 and 5.42 $ t-1 for China, India, Indonesia, Mexico, Canada and Brazil, respectively, and 7.90, 8.26, 6.76, 8.30 and 7.31 $ t-1 for France, Germany, Poland, Italy and Spain, respectively.
“Mining costs for China, India, Indonesia, Mexico, Canada and Brazil calculated using the method were 5.33, 4.44, 3.97, 4.88, 6.79 and 5.42 $ t -1 , respectively and for France, Germany, Poland, Italy and Spain 7.90, 8.26, 6.76, 8.30 and 7.31 $ t -1 , respectively.”
Quote in the paperSubstantial claimMay combine two claims.
Findingown dataUnder the BAU scenario, CO2 emissions from grinding dominate secondary emissions associated with ERW, except for France where low carbon nuclear power dominates.
“Under the BAU scenario, CO2 emissions from grinding dominate secondary emissions associated with ERW, except for France where low carbon nuclear power dominates.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S3 (load-bearing).
FindingcitationRail CO2 emissions were the same for both the business-as-usual (BAU) and 2°C scenarios.
“Rail CO2 emissions were thus the same for both the business-as-usual (BAU) and 2°C scenarios.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [31] DeLucia, E., Kantola, I., Blanc-Betes, E., Bernacchi, C. & Beerling, D. J. Basalt application for carbon sequestration reduces nitrous oxide fluxes from cropland. Geophys. Res. Abstr. 21, EGU2019–EGU4500 (2019).
Not checked in the free run.
The quote only partly states this claim.
Findingown dataResults for the 2°C energy policy scenario are very similar to the business-as-usual scenario.
“Results for the 2°C energy policy scenario are very similar.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S3 (load-bearing).
Findingown dataOnly labradorite in these basalts exhibits noticeable effects of the chemical affinity term.
“Only labradorite (green line) in these basalts exhibits noticeable effects.”
Quote in the paperNot a substantial claimMay combine two claims.
Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplandsERW has potential co-benefits for improved food and soil security and reduced ocean acidification.
“ERW has potential co-benefits for improved food and soil security and reduced ocean acidification [2][3][4] .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [2][3][4]
Not checked in the free run.
May combine two claims.
InterpretationreasoningSuch effects would further lower adverse impacts of agriculture on climate per unit yield, amplifying the climate mitigation potential of ERW.
“Such effects would further lower adverse impacts of agriculture on climate per unit yield, amplifying the climate mitigation potential of ERW.”
Quote in the paperSubstantial claimMay combine two claims.
Interpretationown dataThese patterns reflect expansion of ERW into climatically unfavourable agricultural land, causing CDR potential to slow relative to the carbon penalty of logistical operations, and the 3% limit in national energy available for grinding.
“These patterns reflect expansion of ERW into climatically unfavourable agricultural land, causing CDR potential to slow relative to the carbon penalty of logistical operations, and the 3% limit in national energy available for grinding (Extended Data Fig. 2).”
Quote in the paperSubstantial claimProbably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing), S4 (based).
Interpretationnone given§ The potential for large-scale CO 2 removal via rock weathering on croplandsDeployment with existing croplands offers opportunities to align agriculture and climate policy.
“Deployment with existing croplands offers opportunities to align agriculture and climate policy.”
Quote in the paperNot a substantial claimMay combine two claims.
Interpretationcitation§ The potential for large-scale CO 2 removal via rock weathering on croplandsRapid deployment at large scale appears feasible within decades, with important ancillary benefits including mitigation of ocean acidification.
“Thus, rapid deployment at large scale appears feasible within decades, with important ancillary benefits including mitigation of ocean acidification [15][16][17][18] .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [15][16][17][18]
Not checked in the free run.
May combine two claims.
PremisecitationEfficacy of CO2 removal, sink saturation, and permanency of storage with these approaches, separately and interactively, are uncertain.
“However, efficacy of CO2 removal, sink saturation, and permanency of storage with these approaches, separately and interactively, are uncertain 11,23 .”
Quote in the paperNot a substantial claim0 of 2 sources checked- cites [11] The Royal Society Greenhouse Gas Removal Technologies (The Royal Society, 2018).
Not checked in the free run.
- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
Not checked in the free run.
May combine two claims.
PremisecitationAbatement of soil N2O emissions by basalt application to conventionally managed arable and perennial crops, and of N2O and CH4 emissions by application of artificial silicates to rice agriculture, is possible.
“Abatement of soil N2O emissions by basalt application to conventionally managed arable and perennial crops 31 , and of N2O and CH4 emissions by application of artificial silicates to rice agriculture 32 , is possible.”
Quote in the paperNot a substantial claim0 of 2 sources checked- cites [31] DeLucia, E., Kantola, I., Blanc-Betes, E., Bernacchi, C. & Beerling, D. J. Basalt application for carbon sequestration reduces nitrous oxide fluxes from cropland. Geophys. Res. Abstr. 21, EGU2019–EGU4500 (2019).
Not checked in the free run.
- cites [32] Das, S. et al. Cropping with slag to address soil, environment, and food security. Front. Microbiol. 10, 1320 (2019). source
Not checked in the free run.
Probably not a substantial claim: may not pass S1 (asserted), S3 (load-bearing).
Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplandsProjections of rapid technological change suggest a lower requirement of 2-2.5 Gt CO2 yr -1.
“although projections of rapid technological change 5 suggest a lower requirement of 2-2.5 Gt CO2 yr -1”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [5] Mercure, J.-F. et al. Macroeconomic impact of stranded fossil fuel assests. Nat. Clim. Chang. 8, 588–593 (2018). source
Not checked in the free run.
May combine two claims.
PremisecitationMost of the top 10 fossil carbon emitting nations are failing to meet their 2030 NDC pledges, which even if met imply a median warming of 2.6-3.1 °C, exceeding the Paris Agreement.
“As yet, most of the top 10 fossil carbon emitting nations are failing to meet their 2030 NDC pledges which, even if met, imply a median warming (2.6-3.1 °C) exceeding the Paris agreement 33 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [33] Rogelj, J. et al. Paris Agreement climate proposals need a boost to keep warming well below 2 °C. Nature 534, 631–639 (2016). source
Not checked in the free run.
May combine two claims.
InterpretationcitationERW avoids competition for land used in food production, and related increased demands of BECCS for freshwater and polluting fertilizers, with CO2 being treated as a resource for mineral weathering.
“ERW avoids competition for land used in food production, and related increased demands of BECCS for freshwater and polluting fertilizers 25 , with CO2 being treated as a resource for mineral weathering.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [25] Heck, V., Gerten, D., Lucht, W. & Popp, A. Biomass-based negative emissions difficult to reconcile with planetary boundaries. Nat. Clim. Chang. 8, 151–155 (2018). source
Not checked in the free run.
May combine two claims.
Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplandsBasalt is an abundant fast-weathering rock with the required mineral chemistry, and is a prime target for implementing land-based ERW because of its potential co-benefits for crop production and soil health.
“Basalt, an abundant fast-weathering rock with the required mineral chemistry, is a prime target for implementing land-based ERW because of its potential cobenefits for crop production 18 and soil health [2][3][4] .”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [18] Kelland, M. E. et al. Increased yield and CO2 sequestration potential with the C4 cereal crop Sorghum bicolor cultivated in basaltic rock dust amended agricultural soil. Glob. Change Biol. 26, 3658–3676 (2020). source
Not checked in the free run.
- cites [2][3][4]
Not checked in the free run.
May combine two claims.
InterpretationcitationInorganic carbon sequestration by ERW appears comparable to SOC sequestration (~2.5 Gt CO2 yr -1 by 2100) using agricultural land, but with potentially greater long-term security of C-storage.
“Inorganic carbon sequestration by ERW appears comparable to SOC sequestration, another proposed CDR strategy (~2.5 Gt CO2 yr -1 by 2100) 27 using agricultural land, but with potentially greater long-term security of C-storage.”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [27] Mayer, A. et al. The potential of agricultural land management to contribute to lower global surface temperature. Sci. Adv. 4, eaaq0932 (2018). source
Not checked in the free run.
May combine two claims.
PremisecitationNDC pledged carbon emission reductions undergo periodic revision in response to trends in greenhouse gas emissions, uptake of low-carbon energy technology, and climate, and hence are not set for 2050.
“NDC pledged carbon emission reductions undergo periodic revision in response to trends in greenhouse gas emissions, uptake of low-carbon energy technology, and climate 33 and hence are not set for 2050.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [33] Rogelj, J. et al. Paris Agreement climate proposals need a boost to keep warming well below 2 °C. Nature 534, 631–639 (2016). source
Not checked in the free run.
May combine two claims.
Premisecitation§ The potential for large-scale CO 2 removal via rock weathering on croplandsERW liberates base cations, generating alkalinity such that atmospheric CO2 is converted into dissolved inorganic carbon (principally hydrogen carbonate ions; HCO3-) that is removed via soil drainage waters.
“ERW liberates base cations, generating alkalinity such that atmospheric CO2 is converted into dissolved inorganic carbon (principally hydrogen carbonate ions; HCO3 -) that is removed via soil drainage waters.”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [2][3][4][13][14][15][16][17]
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing).
PremisecitationCement contributes ~6% to global CO2 emissions.
“Cement contributes ~6% to global CO2 emissions 6 and ERW may represent a land management option for valorising by-products to capture carbon and improve the sustainability of this worldwide industry.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [6] Le Quéré, C. et al. Global carbon budget 2018. Earth Syst. Sci. Data 10, 2141–2194 (2018).
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing), S4 (based). May combine two claims.
InterpretationreasoningThis increases the potential to bring smallholders out of extreme poverty and, in regions with climates suitable for non-irrigated agriculture, restore highly degraded soils not suitable currently for food production.
“This increases the potential to bring smallholders out of extreme poverty and, in the regions with climates suitable for non-irrigated agriculture, restore highly degraded soils not suitable currently for food production.”
Quote in the paperNot a substantial claimMay combine two claims.
InterpretationcitationThese negative effects may be reversible with ERW treatments given fertilization of irrigated rice using either natural and/or artificial silicates replenishing plant available silica pools, increasing yields and soil pH, and decreasing the mobility of potentially toxic trace elements (e.g., arsenic).
“Yet these negative effects may be reversible with ERW treatments given fertilization of irrigated rice using either natural and/or artificial silicates (e.g., recycled steel slags) replenishing plant available silica pools, increasing yields and soil pH, and decreasing the mobility of potentially toxic trace elements (e.g., arsenic) 46 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [46] Ning, D. et al. Impacts of steel-slag-based fertilizer on soil acidity and silicon availability and metals-immobilization in a paddy soil. PLoS One 11, e0168163 (2016). source
Not checked in the free run.
Probably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing), S4 (based).
Interpretationnone givenUnderstanding the balance between positive and negative outcomes in terms of public acceptance of the inevitable trade-offs between local mining activities versus global sequestered carbon requires empirical testing with stakeholders and the wider public.
“Understanding the balance between positive and negative outcomes in terms of public acceptance of the inevitable trade-offs between local mining activities versus global sequestered carbon, requires empirical testing with stakeholders and the wider public.”
Quote in the paperNot a substantial claimMay combine two claims.
PremisecitationMining generates a continuous but usually discarded finely powered silicate byproduct utilizable for ERW without embodied CO2 emissions that reduce CDR efficiency, and which has been accumulating worldwide for decades.
“Mining generates a continuous but usually discarded finely powered silicate byproduct utilizable for ERW without embodied CO2 emissions that reduce CDR efficiency (Extended Data Fig. 6) [21][22][23] , and which has been accumulating worldwide for decades.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [21][22][23]
Not checked in the free run.
Probably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing), S4 (based). May combine two claims.
Interpretationnone givenRealizing the potential of ERW as a biogeochemical approach to sequester CO2 by altering land management practices depends on the commitment of farmers and governments, implementation of the right policy frameworks, and wider public acceptance.
“Realizing the potential of ERW as a biogeochemical approach to sequester CO2 by altering land management practices will depend on the commitment of farmers and governments, implementation of the right policy frameworks, and wider public acceptance.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S3 (load-bearing). May combine two claims.
PremisecitationFarming practices for increasing sustainable productivity have transformed agriculture across 37 million hectares in China, increasing profits by $12.2 billion over a decade.
“Farming practices adopted for increasing sustainable productivity, for example, have transformed agriculture across 37 million hectares in China, increasing profits by $12.2 billion over a decade 50 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [50] Cui, Z. et al. Pursuing sustainable productivity with millions of smallholder farmers. Nature 555, 363–366 (2018). source
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing). May combine two claims.
PremisecitationThe current substantial rate of agricultural top-soil depletion requires urgent remedial action, with significant economic costs apparent already in China where degradation of soils supporting wheat, maize and rice production costs an estimated $12 billion annually.
“The current substantial rate of agricultural top-soil depletion requires urgent remedial action, with significant economic costs apparent already in China where degradation of soils supporting wheat, maize and rice production costs an estimated $12 billion annually 48 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [48] United Nations Global Land Outlook 1st edn (United Nations Convention to Combat Desertification, 2017).
Not checked in the free run.
May combine two claims.
PremisecitationAgricultural production can benefit substantially from increased resource use efficiency, reducing consumption of raw materials and recovering mineral nutrients from silicate byproducts and overburden legacy reserves.
“Agricultural production can benefit substantially from increased resource use efficiency, reducing consumption of raw materials and recovering mineral nutrients from silicate byproducts 32,42,43 , and overburden legacy reserves 44 .”
Quote in the paperNot a substantial claim0 of 4 sources checked- cites [32] Das, S. et al. Cropping with slag to address soil, environment, and food security. Front. Microbiol. 10, 1320 (2019). source
Not checked in the free run.
- cites [42] Haynes, R. J., Belyaeva, O. N. & Kingston, G. Evaluation of industrial waste sources of fertilizer silicon using chemical extractions and plant uptake. J. Plant Nutr. Soil Sci. 176, 238–248 (2013). source
Not checked in the free run.
- cites [43] Rodd, A. V. et al. Surface application of cement kiln dust and lime to forage land: effect on forage yield, tissue concentration and accumulation of nutrients. Can. J. Soil Sci. 90, 201–213 (2010). source
Not checked in the free run.
- cites [44] Ramos, C.G. et al. Evaluation of soil re-mineralizer from by-product of volcanic rock mining: experimental proof using black oats and maize crops. Nat. Res. Res. 10.1007/s11053–019–09529-x (2019). source
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing). May combine two claims.
InterpretationreasoningERW may represent a land management option for valorising by-products to capture carbon and improve the sustainability of the cement industry.
“Cement contributes ~6% to global CO2 emissions 6 and ERW may represent a land management option for valorising by-products to capture carbon and improve the sustainability of this worldwide industry.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S3 (load-bearing).
InterpretationcitationAddition of trace amounts of zinc and iron could also improve public health by reversing the effect of rising CO2 levels on the declining nutritional value of food crops.
“Addition of trace amounts of zinc and iron could also improve public health by reversing the effect of rising CO2 levels on the declining nutritional value of food crops 49 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [49] Smith, M. R. & Myers, S. S. Impact of anthropogenic CO2 emissions on global human nutrition. Nat. Clim. Chang. 8, 834–839 (2018). source
Not checked in the free run.
May combine two claims.
PremisecitationChina and India dominate with above-average per capita cement consumption compared to the global average, and substantially larger populations than the USA and Brazil.
“China and India dominate with above-average per capita cement consumption compared to the global average, and substantially larger populations than the USA and Brazil 38 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [38] Renforth, P. The negative emission potential of alkaline materials. Nat. Commun. 10, 1401 (2019). source
Not checked in the free run.
Probably not a substantial claim: may not pass S4 (based). May combine two claims.
Interpretationnone givenFeasibility of mobilizing millions of smallholder communities to adopt ERW practices in China and India depends on demonstrating that soil improvements can reverse yield declines and on government subsidies.
“Feasibility of mobilizing millions of smallholder communities to adopt ERW practices in China and India will depend on demonstrating soil improvements can reverse yield declines, and on government subsidies.”
Quote in the paperNot a substantial claimMay combine two claims.
InterpretationcitationTargeted amendment of agricultural soils for CO2 removal may have a role in slowing rates of soil loss by up to 45%, with the accelerated weathering of added minerals replacing inorganic nutrients and resultant formation of clays and mineral organic aggregates increasing the cation exchange capacity and water storage capacity of rebuilt soils.
“Targeted amendment of agricultural soils for CO2 removal may have a role in slowing rates of soil loss by up to 45%, with the accelerated weathering of added minerals replacing inorganic nutrients and resultant formation of clays and mineral organic aggregates increasing the cation exchange capacity and water storage capacity of rebuilt soils 4,20 .”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [4] Beerling, D. J. et al. Farming with crops and rocks to address global climate, food and soil security. Nat. Plants 4, 138–147 (2018). source
Not checked in the free run.
- cites [20] Smith, P. et al. Land-based options for greenhouse gas removal and their impacts on ecosystem services and the sustainable development goals. Annu. Rev. Environ. Res. 44, 255–286 (2019). source
Not checked in the free run.
Probably not a substantial claim: may not pass S2 (checkable). May combine two claims.
InterpretationcitationA similar outreach programme to that used for sustainable productivity farming could be used throughout Asia, with farmers earning more profits from higher yields while sequestering CO2.
“With 2.5 billion smallholders farming 60% of the world's arable land, a similar outreach programme could be used throughout Asia, with farmers earning more profits from higher yields while sequestering CO2.”
Quote in the paperNot a substantial claim- Rests on an assumption: There are 2.5 billion smallholders farming 60% of the world's arable land.
May combine two claims.
PremisecitationAlthough chemically similar to basalt, artificial calcium-rich silicates contain minerals that dissolve several orders of magnitude faster, react rapidly with CO2 in soils under ambient conditions, and are produced in fine particle sizes that facilitate accelerated weathering.
“Although chemically similar to basalt, these artificial calcium-rich silicates contain minerals that dissolve several orders of magnitude faster, react rapidly with CO2 in soils under ambient conditions 40 , and are produced in fine particle sizes that facilitate accelerated weathering 41 .”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [40] Washbourne, C.-L. et al. Rapid removal of atmospheric CO2 in urban soils. Environ. Sci. Technol. 49, 5434–5440 (2015). source
Not checked in the free run.
- cites [41] Lekakh, S. N. et al. Kinetics of aqueous leaching and carbonization of steelmaking slag. Metallurg. Mater. Trans. B 39, 125–134 (2008). source
Not checked in the free run.
May combine two claims.
PremisecitationCurrent fossil fuel emissions per person per year are 16.5 t CO2 (USA), 15.1 t CO2 (Canada), 7.5 t CO2 (China), 7.3 t CO2 (EU28), 2.6 t CO2 (Brazil), 1.8 t CO2 (Indonesia) and 1.7 t CO2 (India).
“Current fossil fuel emissions per person per year 6 are 16.5 t CO2 (USA), 15.1 t CO2 (Canada), 7.5 t CO2 (China), 7.3 t CO2 (EU28), 2.6 t CO2 (Brazil), 1.8 t CO2 (Indonesia) and 1.7 t CO2 (India).”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [6] Le Quéré, C. et al. Global carbon budget 2018. Earth Syst. Sci. Data 10, 2141–2194 (2018).
Not checked in the free run.
Probably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing).
InterpretationcitationSuch testing needs to understand the conditions that society might place upon the development and large-scale deployment of ERW technologies, as part of a wider responsible research and innovation programme.
“Crucially, such testing needs to understand the conditions that society might place upon the development and large-scale deployment of ERW technologies, as part of a wider responsible research and innovation programme 51 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [51] Pidgeon, N. F. & Spence, E. Perceptions of enhanced weathering as a biological negative emissions option. Biol. Lett. 13, 20170024 (2017). source
Not checked in the free run.
May combine two claims.
InterpretationcitationAt this early stage of research and development, ERW costs are uncertain and in need of demonstration projects.
“At this early stage of research and development, costs are uncertain and in need of demonstration projects 7,11,12 .”
Quote in the paperNot a substantial claim0 of 3 sources checked- cites [7] United Nations Environment Programme The Emissions Gap Report 2018 (United Nations Environment Programme, 2018).
Not checked in the free run.
- cites [11] The Royal Society Greenhouse Gas Removal Technologies (The Royal Society, 2018).
Not checked in the free run.
- cites [12] Pacala, S. et al. Negative Emissions Technologies And Reliable Sequestration (National Academy of Sciences, 2018).
Not checked in the free run.
Classified as probably not a substantial claim. May combine two claims.
InterpretationreasoningThe ancillary benefits of ERW may aid its early use and relieve concern about erosion of climate threat perception.
“The ancillary benefits of ERW may aid its early use and relieve such concern.”
Quote in the paperSubstantial claimMay combine two claims.
PremisecitationThese functions represent the effects of a range of rhizosphere processes that accelerate the physical breakdown and chemical dissolution of minerals, including the activities of nutrient scavenging mycorrhizal fungi that physically disrupt and chemically etch mineral surfaces, and bio-production of low molecular weight organic compounds and chelating agents.
“These functions represent the effects of a range of rhizosphere processes that accelerate the physical breakdown and chemical dissolution of minerals, including the activities of nutrient scavenging mycorrhizal fungi that physically disrupt and chemically etch mineral surfaces, and bio-production of low molecular weight organic compounds and chelating agents 63,64 .”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [63] Harley, A. D. & Gilkes, R. J. Factors influencing the release of plant nutrient elements from silicate rock powders: a geochemical overview. Nutr. Cycl. Agroecosyst. 56, 11–36 (2000). source
Not checked in the free run.
- cites [64] Taylor, L. L. et al. Biological evolution and the long-term carbon cycle: integrating mycorrhizal evolution and function into the current paradigm. Geobiology 7, 171–191 (2009). source
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing).
PremisecitationNations that may have large ERW potential, including China, the United States and India, are all vulnerable to climate change and resultant sea-level rise.
“Nations that may have large ERW potential, including China, the United States and India, are all vulnerable to climate change and resultant sea-level rise 34 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [34] Clark, P. U. et al. Consequences of twenty-first-century policy for multi-millennial climate and sea-level change. Nat. Clim. Chang. 6, 360–369 (2016). source
Not checked in the free run.
May combine two claims.
PremisecitationThe fractal dimension for surface roughness provides a means of consolidating measurements taken at different scales and accounts for uncertainties in grain topography and porosity and mass transfer rates from rock grains to flowing soil water.
“The fractal dimension effectively provides a means of consolidating measurements taken at different scales and accounts for uncertainties in grain topography and porosity 72 , and mass transfer rates from rock grains to flowing soil water.”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [72] Brantley, S. L. & Mellott, N. P. Surface area and porosity of primary silicate minerals. Am. Mineral. 85, 1767–1783 (2000). source
Not checked in the free run.
May combine two claims.
InterpretationreasoningCDR via pathway 2 sequesters 1 mol of CO2 per mole of Ca2+ and is therefore less efficient than pathway 1.
“CDR via pathway 2 can occur if dissolved inorganic carbon derived from atmospheric CO2 precipitates as pedogenic carbonate, and sequesters 1 mol of CO2 per mole of Ca 2+ instead of 1.72 mol of CO2 via pathway 2 and is therefore less efficient.”
Quote in the paperSubstantial claim- The authors state this as an assumption: Weathering products liberated from primary minerals are assumed to subsequently reach the surface ocean via continental runoff.
Probably not a substantial claim: may not pass S3 (load-bearing), S4 (based).
Interpretationnone givenThe potential for trapping of weathered cations on ion exchange surfaces or within secondary minerals other than carbonates delaying, or even preventing, land-ocean transfer will depend on soil type, climate, hydrological conditions, application rate and management practices.
“The potential for trapping of weathered cations on ion exchange surfaces or within secondary minerals other than carbonates delaying, or even preventing, land-ocean transfer will depend on soil type, climate, hydrological conditions, application rate and management practices.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S3 (load-bearing).
Study design and conductnone givenPossible CO2 degassing due to changes in surface water chemistry during transport in large river systems is not considered.
“Possible CO2 degassing due to changes in surface water chemistry during transport in large river systems 74 is not considered.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [74] Salisbury, J. E. et al. Seasonal observations of surface waters in two Gulf of Maine estuary-plume systems: relationships between watershed attributes, optical measurements and surface p CO2. Estuar. Coast. Shelf Sci. 77, 245–252 (2008). source
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing).
Study design and conductnone givenOur analysis of the techno-economic potential of CDR by ERW is subject to several uncertainties, particularly variation in our baseline application rate and basalt mineralogy.
“Our analysis of the techno-economic potential of CDR by ERW is subject to several uncertainties, particularly variation in our baseline application rate and basalt mineralogy.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S3 (load-bearing), S4 (based).
Study design and conductnone givenWe have not considered the penetration of recycling into steel production beyond its current rate.
“We have not considered the penetration of recycling into steel production beyond its current rate.”
Quote in the paperNot a substantial claimMay combine two claims.
InterpretationcitationInnovative 'climate-smart' farming practices can be designed with ERW to draw down CO2 and other greenhouse gases while recycling nutrients, aiding soil water storage, and supporting crop production.
“Innovative 'climate-smart' farming practices can be designed with ERW to draw down CO2 and other greenhouse gases while recycling nutrients, aiding soil water storage, and supporting crop production 4,18,20 .”
Quote in the paperSubstantial claim0 of 3 sources checked- cites [4] Beerling, D. J. et al. Farming with crops and rocks to address global climate, food and soil security. Nat. Plants 4, 138–147 (2018). source
Not checked in the free run.
- cites [18] Kelland, M. E. et al. Increased yield and CO2 sequestration potential with the C4 cereal crop Sorghum bicolor cultivated in basaltic rock dust amended agricultural soil. Glob. Change Biol. 26, 3658–3676 (2020). source
Not checked in the free run.
- cites [20] Smith, P. et al. Land-based options for greenhouse gas removal and their impacts on ecosystem services and the sustainable development goals. Annu. Rev. Environ. Res. 44, 255–286 (2019). source
Not checked in the free run.
The quote only partly states this claim.
Study design and conductown dataWe addressed the uncertainty from extrapolation of laboratory weathering rates by Monte Carlo analysis of the fractal dimension accounting for uncertainty in the apparent reacting surface area of grains for ERW conducted at large geographical scales.
“We addressed this by Monte Carlo analysis of the fractal dimension accounting for uncertainty in the apparent reacting surface area of grains for ERW conducted at large geographical scales.”
Quote in the paperSubstantial claimMay combine two claims.
PremisecitationDuration of carbon sequestration rate, and possibility for CO2 sink saturation with ERW on croplands, are both poorly constrained by data, in common with other land-based CDR strategies, and affect cumulative CDR potential in coming decades.
“Duration of carbon sequestration rate, and possibility for CO2 sink saturation with ERW on croplands, are both poorly constrained by data, in common with other land-based CDR strategies 11,23 , and affect cumulative CDR potential in coming decades.”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [11] The Royal Society Greenhouse Gas Removal Technologies (The Royal Society, 2018).
Not checked in the free run.
- cites [23] Fuss, S. et al. Negative emissions—Part 2: Costs, potentials and side effects. Environ. Res. Lett. 13, 063002 (2018). source
Not checked in the free run.
Probably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing).
InterpretationcitationTheir high risks of economic damage and social disruption provide impetus for creative co-design of agricultural and climate policies.
“Their high risks of economic damage 53 and social disruption provide impetus for creative co-design of agricultural and climate policies.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [53] Ricke, K., Drout, L., Caldeira, K. & Tavoni, M. Country-level social cost of carbon. Nat. Clim. Chang. 8, 895–900 (2018). source
Not checked in the free run.
May combine two claims.
InterpretationcitationSuch practices can help restore deteriorating top-soils that underpin food security for billions of people while maximizing societal co-benefits needed to incentivise deployment.
“Such practices can help restore deteriorating top-soils that underpin food security for billions of people while maximizing societal co-benefits needed to incentivise deployment 20 .”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [20] Smith, P. et al. Land-based options for greenhouse gas removal and their impacts on ecosystem services and the sustainable development goals. Annu. Rev. Environ. Res. 44, 255–286 (2019). source
Not checked in the free run.
Classified as probably not a substantial claim.
InterpretationreasoningCalculating representative annual CO2 removal rates requires computing average rates derived from repeated basaltic rock dust applications.
“Thus calculating representative annual CO2 removal rates requires computing average rates derived from repeated basaltic rock dust applications (Extended Data Fig. 7).”
- Also stated in: § Extended · plain
“Thus calculating representative annual CO2 removal rates requires computing average rates derived from repeated basaltic rock dust applications.”
Quote in the paperSubstantial claim- Also stated in: § Extended · plain
May combine two claims.
InterpretationreasoningCDR via pathway 2 sequesters 1 mol of CO2 per mole of Ca2+ instead of 1.72 mol of CO2 via pathway 1 and is therefore less efficient.
“CDR via pathway 2 occurs if dissolved inorganic CO2 precipitates as pedogenic carbonate, and sequesters 1 mol of CO2 per mole of Ca 2+ instead of 1.72 mol of CO2 via pathway 1 and is therefore less efficient.”
Quote in the paperSubstantial claimClassified as probably not a substantial claim.
Study design and conductcitationThe fractal dimension and its uncertainty are determined from a linear regression analysis performed on measurements from a range of spatial scales (10−10-103 m).
“The fractal dimension and its uncertainty are determined from a linear regression analysis performed on measurements from a range of spatial scales 3 (10 -10 -10 3 m).”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [3] Zhang, G., Kang, J., Wang, T. & Zhu, C. Review and outlook for agromineral research in agriculture and climate change mitigation. Soil Res. 56, 113–122 (2018). source
Not checked in the free run.
Classified as probably not a substantial claim. May combine two claims.
PremisecitationFunctions are fitted to mesocosm data for three species of agricultural crops (maize, rice and soybean) and four species of mycorrhizal tree saplings.
“Functions are fitted to mesocosm data for (a) three speies of agricultural crops (maize, rice and soybean) 46,47 , and (b) four species of mycorrhizal tree saplings 48,49 .”
Quote in the paperSubstantial claim0 of 4 sources checked- cites [46] Ning, D. et al. Impacts of steel-slag-based fertilizer on soil acidity and silicon availability and metals-immobilization in a paddy soil. PLoS One 11, e0168163 (2016). source
Not checked in the free run.
- cites [47] Chen, J. Rapid urbanization in China: a real challenge to soil protection and food security. Catena 69, 1–15 (2007). source
Not checked in the free run.
- cites [48] United Nations Global Land Outlook 1st edn (United Nations Convention to Combat Desertification, 2017).
Not checked in the free run.
- cites [49] Smith, M. R. & Myers, S. S. Impact of anthropogenic CO2 emissions on global human nutrition. Nat. Clim. Chang. 8, 834–839 (2018). source
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing), S4 (based).
Interpretationnone givenThe extent to which simulated pH increases promote or adversely affect crop production depends on the initial topsoil pH, crop functional traits, weathering rates, climate, flushing rates and fertiliser treatments.
“The extent to which simulated pH increases promote or adversely affect crop production depends on the initial topsoil pH, crop functional traits, weathering rates, climate, flushing rates and fertiliser treatments.”
Quote in the paperNot a substantial claimClassified as probably not a substantial claim.
Interpretationnone givenThese functions represent the lumped effects of rhizosphere biological processes accelerating weathering.
“These functions represent the lumped effects of rhizosphere biological processes accelerating weathering (Section 1.9).”
Quote in the paperSubstantial claimMay combine two claims.
InterpretationreasoningThe lower price for China, India and Brazil reflects low labour costs while the higher price for France and Germany reflects higher diesel costs.
“The lower price for China, India and Brazil reflects low labour costs while the higher price for France and Germany reflects higher diesel costs.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing), S4 (based). May combine two claims.
Interpretationnone givenOur costs are indicative of key features of an ERW supply chain and consistent with previous global approaches.
“Our cost are indicative of key features of an ERW supply chain and consistent with previous global approaches.”
Quote in the paperNot a substantial claim- The authors state this as an assumption: Cost of spreading rock with farming machinery is equivalent to that of spreading lime ($15.18/t).
Probably not a substantial claim: may not pass S3 (load-bearing).
Premiseown dataThe exceptions to the low leachate elemental concentrations are Sb and Se.
“The exceptions are Sb and Se.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S3 (load-bearing).
PremisecitationBasaltic glass powder with a diameter of 40-120 μm has a roughness factor (lambda) of ~92.
“For comparison, basaltic glass powder with a diameter of 40 -120µm has a lambda 50 of ~92.”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [50] Cui, Z. et al. Pursuing sustainable productivity with millions of smallholder farmers. Nature 555, 363–366 (2018). source
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing).
PremisecitationSb and Se are less concentrated in the unmixed cement waste.
“However, these are less concentrated in the unmixed cement waste 59 .”
Quote in the paperNot a substantial claim0 of 1 sources checked- cites [59] Siebert, S. & Doll, P. Quantifying blue and green virtual water contents in global crop production as well as potential production losses without irrigation. J. Hydrol. 384, 198–217 (2010). source
Not checked in the free run.
Probably not a substantial claim: may not pass S3 (load-bearing).
InterpretationreasoningUncertainty in the fractal dimension affects weathering rate and consequently, through the optimization, the p80 grid cell vector.
“Uncertainty in the fractal dimension affects weathering rate and consequently, through the optimization, the p80 grid cell vector.”
Quote in the paperNot a substantial claimMay combine two claims.
InterpretationreasoningThe affinity effect on labradorite is greatest during the first 100 days, especially under a low flow rate (200 mm yr -1), because there is little dilution of the weathered products, resulting in higher pore water concentrations exerting a stronger affinity effect.
“This is greatest during the first 100 days, especially under a low flow rate (200 mm yr -1 top panels) because there is little dilution of the weathered products, resulting in higher pore water concentrations exerting a stronger affinity effect.”
Quote in the paperNot a substantial claim
The paper relies on this without support.
There are 2.5 billion smallholders farming 60% of the world's arable land.
“With 2.5 billion smallholders farming 60% of the world's arable land”
The paper relies on this without support.
Surface passivation occurs as weathering proceeds, creating leached layers and relatively stable secondary minerals, which potentially inhibit the mass transfer kinetics of elements from the dissolving surfaces of primary minerals.
“Surface passivation, a component of chemical inhibition, occurs as weathering proceeds, creating leached layers and relatively stable secondary minerals, which potentially inhibit the mass transfer kinetics of elements from the dissolving surfaces of primary minerals.”
The authors state this as an assumption.
Weathering products liberated from primary minerals are assumed to subsequently reach the surface ocean via continental runoff.
“Carbon dioxide removal (CDR) results from the mass transport of enhanced weathering products liberated from the primary minerals, which are assumed to subsequently reach the surface ocean via continental runoff, or can be precipitated as secondary carbonate minerals in the terrestrial environment.”
The authors state this as an assumption.
Particles are assumed to be spherical.
“As particles are assumed to be spherical, we reformulate equation 14 in terms radius rather than mass to give:”
The authors state this as an assumption.
The scrap ratio remains unchanged.
“The ratio of pig iron to steel production (0.72) was obtained using linear regression of 1960-2014 data, negating the need to explicitly model pig iron displacement from scrap recycling, and assuming the scrap ratio remains unchanged.”
“assuming the scrap ratio remains unchanged.”
The authors state this as an assumption.
All steel and blast furnace slag is available for reaction with CO2.
“All steel and blast furnace slag was considered available for reaction with CO2.”
“All steel and blast furnace slag was considered available for reaction with CO2.”
The paper relies on this without support.
Cement and cement kiln dust have no capacity to be recycled as cement.
“Cement and cement kiln dust have no capacity to be recycled as cement.”
“Cement and cement kiln dust have no capacity to be recycled as cement.”
The paper relies on this without support.
In the tropics and subtropics, annual temperature variation is relatively low.
“In the tropics and subtropics, where perennial crops dominate, annual temperature variation is relatively low.”
The paper relies on this without support.
The soil surface temperature at 5 cm depth of the 8 warmest months for 2050 represents conditions during the main growth period of most crop types found outside the tropics.
“This value is taken to represent conditions during the main growth period of most crop types found outside the tropics.”
The paper relies on this without support.
Standard calculations of rate of mineral dissolution ignore size differences in reacting particles and simulate the mineral with a surface area that corresponds to the mean diameter of a particle size distribution.
“Standard calculations of rate of mineral dissolution ignore size differences in reacting particles and simulate the mineral with a surface area that corresponds to the mean diameter of a particle size distribution (psd).”
The authors state this as an assumption.
Land management practices for annual crops return cations released during dissolution, and taken up by crops back to soils via biomass decomposition.
“We assume land management practices for annual crops return cations released during dissolution, and taken up by crops back to soils via biomass decomposition.”
The authors state this as an assumption.
Cost of spreading rock with farming machinery is equivalent to that of spreading lime ($15.18/t).
“Cost of spreading rock with farming machinery was considered equivalent to that of spreading lime ($15.18/t).”
The authors state this as an assumption.
A future limit of 3% of total energy production for rock comminution for all nations.
“We assume a future limit of 3% for all nations, based on the rationale that current rates for developed nations grow from around 2% today in-line with future energy scenarios 33 .”
The authors state this as an assumption.
115 kg of cement kiln dust is produced as a by-product in kilns for every tonne of clinker, and demolition waste follows an average 50-year service life (normally distributed with standard deviation 10 years).
“We assume 115 kg of cement kiln dust is produced as a by-product in kilns for every tonne of clinker, and have modelled the production of demolition waste following an average 50-year service life (normally distributed with a standard deviation of 10 years) 41 .”
The authors state this as an assumption.
Interstitial waters are in equilibrium with dissolved weathering products, inorganic and organic soil cation exchange surfaces and secondary minerals.
“Interstitial waters are calculated to be in equilibrium with the dissolved weathering products, inorganic and organic soil cation exchange surfaces and secondary minerals.”
The authors state this as an assumption.
Secondary minerals form and dissolve instantaneously to maintain thermodynamic equilibrium between the fluid and mineral phases.
“These were calculated to form and dissolve instantaneously to maintain thermodynamic equilibrium between the fluid and mineral phases.”
The authors state this as an assumption.
The soil solution is in equilibrium with atmospheric pO2(g).
“The soil solution was equilibrated with dissolved O2 and CO2; assuming equilibrium with atmospheric pO2(g) (atm).”
Claims other papers make about this one
Each is checked against this paper’s own text: does it say what the citing paper says it does?
Application of crushed calcium- and magnesium-rich silicate rocks to soils (enhanced rock weathering) increases soil alkalinity, converting atmospheric CO2 into dissolved inorganic C transported to the ocean where stored C has a long lifespan.
“Application of crushed calcium- and magnesium-rich silicate rocks to soils is proposed for large-scale CO2 removal.191 This technology was called enhanced rock weathering, which increases soil alkalinity, and thus atmospheric CO2 can be converted into dissolved inorganic C to be finally transported to the ocean, where the stored C has a long lifespan via land surface runoff.”
From Technologies and perspectives for achieving carbon neutrality (2021) · cites this paper as [191]
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
Each contradiction between two passages listed here was confirmed by an independent check.
Carbon-price range is said to cover costs in all nations despite higher reported costs
MajorThe projected carbon-price range is $100-150 per tonne, but the paper reports average costs of $160-180 for the USA and $160-190 for Canada and European nations. Those averages are outside the range, contrary to the claim that costs are generally within it in all nations.
“Costs per t CO2 removed are generally within this projected carbon price range in all nations”
“Average costs in USA ($160-180 t -1 CO2), Canada and European nations ($160-190 t -1 CO2) are almost 50% higher than those in China, India, Mexico, Indonesia, and Brazil ($55-120 t -1 CO2).”
Optimization uses 2030 electricity production in a 2050 assessment
MinorThe optimization constraint specifies projected grid electricity production for 2030, whereas the stated optimization inputs and national energy projections are for 2050.
“the country's projected grid electricity production PGrid (Energy) for the year 2030”
“We used country-specific electricity production (PGrid) and the forecast fractional contributions to electricity production by different energy sources (coal, natural gas, oil, solar PV, concentrated solar power, hydropower, wind, marine) for 2050”
Carbonate pathway is mislabeled as the comparison pathway
MinorThe sentence contrasts carbonate formation (pathway 2) with ocean-bound cations but calls the latter pathway 2 as well. The paper elsewhere assigns ocean-bound cations to pathway 1.
“sequesters 1 mol of CO2 per mole of Ca 2+ instead of 1.72 mol of CO2 via pathway 2”
“CDR, via pathway 1, potentially sequesters two moles of CO2 from the atmosphere per mole of divalent cation.”
Water-quality exceptions omit three elements above their listed standards
MinorTable S15 lists aluminium, calcium and potassium concentrations above their respective stated water-quality standards. The accompanying text identifies only Sb and Se as exceptions.
“The exceptions are Sb and Se.”
“Aluminium (mg l -1 ) 1.6 0.2 Calcium (mg l -1 ) 395 250 Iron (mg l -1 ) 0.085 0.2 to 1 Potassium (mg l -1 ) 125 10 to 12”
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The potential of agricultural land management to contribute to lower global surface temperatures
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Blurred Lines: The Ethics and Policy of Greenhouse Gas Removal at Scale
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Ideas and perspectives: Synergies from co-deployment of negative emission technologies
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Perceptions of enhanced weathering as a biological negative emissions option
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Self-citationReview and outlook for agromineral research in agriculture and climate mitigation
Zhang, G., Kang, J., Wang, T., & Zhu, C. (2018) · Soil Research · doi:10.1071/sr17157 · Cited by 32 · see citing works
Effect of Fine Root Contact on Plant-Induced Weathering of Basalt
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Dependence of plant-induced weathering of basalt and andesite on nutrient conditions
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Modelling a Logistic Problem by Creating an Origin-Destination Cost Matrix using GIS Technology
ROTAR, A. M., Pop, I., Matei, F., Andronie, L., Vâtcă, A., & Cioban, A. (2014) · Bulletin of University of Agricultural Sciences and Veterinary Medicine Cluj-Napoca Horticulture · doi:10.15835/buasvmcn-hort:9697 · Cited by 4 · see citing works
Basalt application for carbon sequestration reduces nitrous oxide fluxes from cropland
DeLucia, E. H., Kantola, I. B., Blanc‐Betes, E., Bernacchi, C. J., & Beerling, D. J. (2019) · EGU General Assembly Conference Abstracts · Cited by 3 · see citing works
Self-citation
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Technologies and perspectives for achieving carbon neutrality
Wang, F., Harindintwali, J. D., Yuan, Z., Wang, M., Wang, F., Li, S., Yin, Z., Huang, L., Fu, Y., Li, L., et al. (2021) · The Innovation · doi:10.1016/j.xinn.2021.100180 · Cited by 1,330 · see citing works
Biochar in climate change mitigation
Lehmann, J., Cowie, A., Masiello, C. A., Kammann, C., Woolf, D., Amonette, J. E., Cayuela, M. L., Camps-Arbestain, M., & Whitman, T. (2021) · Nature Geoscience · doi:10.1038/s41561-021-00852-8 · Cited by 970 · see citing works
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Life cycle assessment of carbon dioxide removal technologies: a critical review
Terlouw, T., Bauer, C., Rosa, L., & Mazzotti, M. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03757e · Cited by 366 · see citing works
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The role of soil in regulation of climate
Lal, R., Monger, C., Nave, L., & Smith, P. (2021) · Philosophical Transactions of the Royal Society B Biological Sciences · doi:10.1098/rstb.2021.0084 · Cited by 304 · see citing works
“Enhanced weathering involves (i) the mining of rocks containing minerals that naturally lead to CO2 absorption from the atmosphere over geological timescales (as they become exposed to the atmosphere through geological weathering), (i) the grinding of these rocks to increase the surface area and (iii) the spreading of…”
BackgroundSilicon Cycling in Soils Revisited
Schaller, J., Puppe, D., Kaczorek, D., Ellerbrock, R. H., & Sommer, M. (2021) · Plants · doi:10.3390/plants10020295 · Cited by 276 · see citing works
“Weathering of specific minerals is also discussed as an important sink for CO2, because calcium carbonate formation from calcium silicates mobilizes silicic acid and binds CO2 [6,7].”
BackgroundIntroducing the soil mineral carbon pump
Xiao, K., Zhao, Y., Liang, C. C., Zhao, M., Moore, O., Otero-Fariña, A., Zhu, Y., Johnson, K. L., & Peacock, C. L. (2023) · Nature Reviews Earth & Environment · doi:10.1038/s43017-023-00396-y · Cited by 268 · see citing works
Remineralizing soils? The agricultural usage of silicate rock powders: A review
Swoboda, P., Döring, T. F., & Hamer, M. (2021) · The Science of The Total Environment · doi:10.1016/j.scitotenv.2021.150976 · Cited by 259 · see citing works
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“…of practices like the use of deep- rooted annual crops (Kell, 2012), the deployment of perennial grain crops (Culman et al., 2013), or the application of crushed silicate rocks, waste cement, or industrial slags (Beerling et al., 2020) on SOC has so far not been investigated through meta- analysis.”
BackgroundSize, distribution, and vulnerability of the global soil inorganic carbon
Huang, Y., Song, X., Wang, Y., Canadell, J. G., Luo, Y., Ciais, P., Chen, A., Hong, S., Wang, Y., Tao, F., et al. (2024) · Science · doi:10.1126/science.adi7918 · Cited by 206 · see citing works
Diverse carbon dioxide removal approaches could reduce impacts on the energy–water–land system
Fuhrman, J., Bergero, C., Weber, M., Monteith, S., Wang, F. M., Clarens, A. F., Doney, S. C., Shobe, W., & McJeon, H. C. (2023) · Nature Climate Change · doi:10.1038/s41558-023-01604-9 · Cited by 203 · see citing works
Potential CO2 removal from enhanced weathering by ecosystem responses to powdered rock
Goll, D. S., Ciais, P., Amann, T., Buermann, W., Chang, J., Eker, S., Hartmann, J., Janssens, I., Li, W., Obersteiner, M., et al. (2021) · Nature Geoscience · doi:10.1038/s41561-021-00798-x · Cited by 197 · see citing works
Self-citationHow temperature-dependent silicate weathering acts as Earth’s geological thermostat
Brantley, S. L., Shaughnessy, A. R., Lebedeva, M. I., & Balashov, V. N. (2023) · Science · doi:10.1126/science.add2922 · Cited by 187 · see citing works
Substantial carbon drawdown potential from enhanced rock weathering in the United Kingdom
Kantzas, E. P., Martin, M. V., Lomas, M. R., Eufrasio, R. M., Renforth, P., Lewis, A. L., Taylor, L. L., Mercure, J.-F., Pollitt, H., Vercoulen, P., et al. (2022) · Nature Geoscience · doi:10.1038/s41561-022-00925-2 · Cited by 169 · see citing works
Self-citationLewis, A. L., Sarkar, B., Wade, P., Kemp, S. J., Hodson, M. E., Taylor, L. L., Yeong, K. L., Davies, K., Nelson, P. N., Bird, M. I., et al. (2021) · Applied Geochemistry · doi:10.1016/j.apgeochem.2021.105023 · Cited by 168 · see citing works
Self-citationDual role of silt and clay in the formation and accrual of stabilized soil organic carbon
Mao, H., Cotrufo, M. F., Hart, S. C., Sullivan, B. W., Zhu, X., Zhang, J., Liang, C., & Zhu, M. (2024) · Soil Biology and Biochemistry · doi:10.1016/j.soilbio.2024.109390 · Cited by 156 · see citing works
A review on the possible factors influencing soil inorganic carbon under elevated CO2
Ferdush, J., & Paul, V. G. (2021) · CATENA · doi:10.1016/j.catena.2021.105434 · Cited by 157 · see citing works
Enhanced weathering in the US Corn Belt delivers carbon removal with agronomic benefits
Beerling, D. J., Epihov, D. Z., Kantola, I. B., Masters, M. D., Reershemius, T., Planavsky, N. J., Reinhard, C. T., Jordan, J. S., Thorne, S. J., Weber, J., et al. (2024) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.2319436121 · Cited by 150 · see citing works
“Biogeochemical modeling suggests that deployment of EW with basalt across major agricultural regions worldwide could sequester up to two billion metric tons of CO 2 annually, after accounting for operational carbon emissions (mining, grinding, transport, and spreading of rock dust on fields) (4).”
Self-citationKazemifar, F. (2021) · Greenhouse Gases Science and Technology · doi:10.1002/ghg.2131 · Cited by 145 · see citing works
Achieving net-zero emissions in agriculture: a review
Rosa, L., & Gabrielli, P. (2023) · Environmental Research Letters · doi:10.1088/1748-9326/acd5e8 · Cited by 154 · see citing works
“Fertilizer 1.05 Gt CO 2-eq from global BECCS potential; 1.56 Gt CO 2-eq from avoided methane and nitrous oxide emissions from agricultural waste and residues, (range: 0.9–1.2 Gt CO 2-eq ) [51] 0.2% of global BECCS potential [52] Enhanced rock weathering Pilot [53] 2 Gt CO 2-eq , (range: 0.5–2 Gt CO 2-eq ) [53] 0% prod…”
BackgroundInfluentialRecent Advances in Interface Engineering for Electrocatalytic CO2 Reduction Reaction
Li, J., Abbas, S. U., Wang, H., Zhang, Z., & Hu, W. (2021) · Nano-Micro Letters · doi:10.1007/s40820-021-00738-9 · Cited by 140 · see citing works
Vicca, S., Goll, D. S., Hagens, M., Hartmann, J., Janssens, I. A., Neubeck, A., Peñuelas, J., Poblador, S., Rijnders, J., Sardans, J., et al. (2021) · Global Change Biology · doi:10.1111/gcb.15993 · Cited by 145 · see citing works
Self-citationMineral security essential to achieving the Sustainable Development Goals
Franks, D. M., Keenan, J., & Hailu, D. (2022) · Nature Sustainability · doi:10.1038/s41893-022-00967-9 · Cited by 131 · see citing works
Vienne, A., Poblador, S., Portillo‐Estrada, M., Hartmann, J., Ijiehon, S., Wade, P., & Vicca, S. (2022) · Frontiers in Climate · doi:10.3389/fclim.2022.869456 · Cited by 129 · see citing works
“However, costs of C sequestration through enhanced weathering of basalt are estimated at about US$80–180 t−1 CO2 (Beerling et al., 2020), which corresponds roughly to the world bank estimate of the carbon price in 2050 (100–150$ tCO2) and current EU-ETS carbon price, which already exceeded 100 US$ t−1 CO2 in 2022.”
BackgroundSelf-citationMineral-enriched biochar delivers enhanced nutrient recovery and carbon dioxide removal
Buss, W., Wurzer, C., Manning, D. A. C., Rohling, E. J., Borevitz, J., & Mašek, O. (2022) · Communications Earth & Environment · doi:10.1038/s43247-022-00394-w · Cited by 123 · see citing works
Sharififar, A., Minasny, B., Arrouays, D., Boulonne, L., Chevallier, T., van Deventer, P., Field, D. J., Cécile Gomez, A., Jang, H.-J., Jeon, S.-H., et al. (2023) · Advances in agronomy · doi:10.1016/bs.agron.2022.11.005 · Cited by 117 · see citing works
The contribution of living organisms to rock weathering in the critical zone
Wild, B., Gerrits, R., & Bonneville, S. (2022) · npj Materials Degradation · doi:10.1038/s41529-022-00312-7 · Cited by 118 · see citing works
Optimizing cover crop practices as a sustainable solution for global agroecosystem services
Qiu, T., Shi, Y., Peñuelas, J., Liu, J., Cui, Q., Sardans, J., Zhou, F., Xia, L., Yan, W., Zhao, S., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-54536-z · Cited by 115 · see citing works
Multi-objective energy planning for China's dual carbon goals
Jia, X., Zhang, Y., Tan, R. R., Li, Z., Wang, S., Wang, F., & Fang, K. (2022) · Sustainable Production and Consumption · doi:10.1016/j.spc.2022.10.009 · Cited by 112 · see citing works
Technologies to deliver food and climate security through agriculture
Horton, P., Long, S. P., Smith, P., Banwart, S. A., & Beerling, D. J. (2021) · Nature Plants · doi:10.1038/s41477-021-00877-2 · Cited by 106 · see citing works
Self-citationEnvironmental sustainability of negative emissions technologies: A review
Jeswani, H. K., Saharudin, D. M., & Azapagic, A. (2022) · Sustainable Production and Consumption · doi:10.1016/j.spc.2022.06.028 · Cited by 109 · see citing works
Global chemical weathering dominated by continental arcs since the mid-Palaeozoic
Gernon, T., Hincks, T. K., Merdith, A., Rohling, E. J., Palmer, M. R., Foster, G. L., Bataille, C. P., & Müller, R. D. (2021) · Nature Geoscience · doi:10.1038/s41561-021-00806-0 · Cited by 103 · see citing works
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A comparative analysis of the efficiency, timing, and permanence of CO 2 removal pathways
Chiquier, S., Patrizio, P., Bui, M., Sunny, N., & Dowell, N. M. (2022) · Energy & Environmental Science · doi:10.1039/d2ee01021f · Cited by 102 · see citing works
Possibilities of using silicate rock powder: An overview
Ramos, C. G., Hower, J. C., Donado, E. B., Oliveira, M. L. S., & Theodoro, S. H. (2021) · Geoscience Frontiers · doi:10.1016/j.gsf.2021.101185 · Cited by 100 · see citing works
Evidence linking calcium to increased organo-mineral association in soils
Rowley, M. C., Grand, S., Spangenberg, J. E., & Verrecchia, É. P. (2021) · Biogeochemistry · doi:10.1007/s10533-021-00779-7 · Cited by 99 · see citing works
“2017), and their potential interactions with management practices that aim to sequester C inorganically (Beerling et al. 2020).”
BackgroundRinder, T., & von Hagke, C. (2021) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2021.128178 · Cited by 101 · see citing works
Hu, P., Zhang, W., Nottingham, A. T., Xiao, D., Kuzyakov, Y. V., Xu, L., Chen, H., Xiao, J., Duan, P., Tang, T., et al. (2024) · Environmental Science & Technology · doi:10.1021/acs.est.4c07264 · Cited by 93 · see citing works
Pas, E. E. E. M. T., Hagens, M., & Comans, R. N. J. (2023) · Frontiers in Climate · doi:10.3389/fclim.2022.954064 · Cited by 92 · see citing works
“We should note here that chemical weathering rates measured in laboratory experiments likely differ from those measured in field conditions, and differ per soil type and climatic region (Renforth et al., 2015; Beerling et al., 2020), and that the application of a single silicate on global cropland is rather unlikely g…”
BackgroundPotential accumulation of toxic trace elements in soils during enhanced rock weathering
Dupla, X., Möller, B., Baveye, P. C., & Grand, S. (2023) · European Journal of Soil Science · doi:10.1111/ejss.13343 · Cited by 92 · see citing works
Improved net carbon budgets in the US Midwest through direct measured impacts of enhanced weathering
Kantola, I. B., Blanc‐Betes, E., Masters, M. D., Chang, E., Marklein, A., Moore, C. E., von Haden, A. C., Bernacchi, C. J., Wolf, A., Epihov, D. Z., et al. (2023) · Global Change Biology · doi:10.1111/gcb.16903 · Cited by 89 · see citing works
“…accelerating the natural weathering process of Mg-or Ca-rich rocks, enhanced weathering (EW), can potentially sequester atmospheric carbon (Beerling et al., 2020 ; Kantola et al., 2017; Kelland et al., 2020 ; Kohler et al., 2010 ; Schuiling & Krijgsman, 2006; Taylor et al., 2016 ), and…”
BackgroundMethodInfluentialSelf-citationCarbon mineralization with concurrent critical metal recovery from olivine
Wang, F., & Dreisinger, D. B. (2022) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.2203937119 · Cited by 89 · see citing works
Deep CCS: Moving Beyond 90% Carbon Dioxide Capture
Dods, M. N., Kim, E. J., Long, J. R., & Weston, S. C. (2021) · Environmental Science & Technology · doi:10.1021/acs.est.0c07390 · Cited by 83 · see citing works
Nano- to Global-Scale Uncertainties in Terrestrial Enhanced Weathering
Calabrese, S., Wild, B., Bertagni, M. B., Bourg, I. C., White, C. E., Aburto, F. A., Cipolla, G., Noto, L., & Porporato, A. M. (2022) · Environmental Science & Technology · doi:10.1021/acs.est.2c03163 · Cited by 83 · see citing works
Zamanian, K., Taghizadeh‐Mehrjardi, R., Tao, J., Fan, L., Raza, S., Guggenberger, G., & Kuzyakov, Y. V. (2024) · The Science of The Total Environment · doi:10.1016/j.scitotenv.2024.171631 · Cited by 85 · see citing works
Low, S., Baum, C. M., & Sovacool, B. K. (2022) · Energy Research & Social Science · doi:10.1016/j.erss.2022.102594 · Cited by 84 · see citing works
“Emerging enhanced weathering projects have tended to avoid the issues associated with the term “geoengineering” by highlighting entwined relevance for coupling with agriculture, mining operations, carbon crediting (EWT3, EWT4, EWO2), and supposedly addressing issues most in need of climate-mitigation efforts [129,185].”
Adun, H. H., Ampah, J. D., Bamisile, O., & Hu, Y. (2024) · Sustainable Production and Consumption · doi:10.1016/j.spc.2024.01.004 · Cited by 81 · see citing works
The policy implications of an uncertain carbon dioxide removal potential
Grant, N., Hawkes, A. D., Mittal, S., & Gambhir, A. (2021) · Joule · doi:10.1016/j.joule.2021.09.004 · Cited by 80 · see citing works
Larkin, C. S., Andrews, M. G., Pearce, C. R., Yeong, K. L., Beerling, D. J., Bellamy, J., Benedick, S., Freckleton, R. P., Goring-Harford, H. J., Sadekar, S., et al. (2022) · Frontiers in Climate · doi:10.3389/fclim.2022.959229 · Cited by 82 · see citing works
“To date, the potential of enhanced weathering for removing atmospheric CO2 has principally been estimated usingmodeling studies (e.g., Renforth, 2012; Taylor et al., 2016; Beerling et al., 2020; Bullock et al., 2021), or based on results from small-scale mesocosm or laboratory experiments (e.”
BackgroundSelf-citationGlobal Carbon Dioxide Removal Potential of Waste Materials From Metal and Diamond Mining
Bullock, L. A., James, R. H., Matter, J., Renforth, P., & Teagle, D. A. H. (2021) · Frontiers in Climate · doi:10.3389/fclim.2021.694175 · Cited by 76 · see citing works
“An annual application rate of ∼40 t ha−1 of basalt, which is compositionally similar to some tailings generated from PGM, Cr and Ni mines, has been suggested as an effective additive to improve soils (Beerling et al., 2020).”
BackgroundSelf-citationInducing Inorganic Carbon Accrual in Subsoil through Biochar Application on Calcareous Topsoil
Wang, Y., Joseph, S. D., Wang, X., Weng, Z. H., Mitchell, D. R. G., Nancarrow, M. J. B., Taherymoosavi, S., Munroe, P. R., Li, G., Lin, Q., et al. (2023) · Environmental Science & Technology · doi:10.1021/acs.est.2c06419 · Cited by 77 · see citing works
Geochemical Negative Emissions Technologies: Part I. Review
Campbell, J. S., Foteinis, S., Furey, V., Hawrot, O., Pike, D., Aeschlimann, S., Maesano, C. N., Reginato, P., Goodwin, D., Looger, L. L., et al. (2022) · Frontiers in Climate · doi:10.3389/fclim.2022.879133 · Cited by 76 · see citing works
“Enhanced Weathering in Soils Enhanced weathering in soils aims to accelerate the natural process of weathering through the spreading of crushed Mgand Ca-rich silicate rocks in agricultural, urban, and forest soils (Renforth, 2012; Hartmann et al., 2013; Beerling et al., 2020; Haque et al., 2020b).”
BackgroundInfluentialSelf-citationEufrasio, R. M., Kantzas, E. P., Edwards, N. R., Holden, P. B., Pollitt, H., Mercure, J.-F., Koh, S. C. L., & Beerling, D. J. (2022) · Communications Earth & Environment · doi:10.1038/s43247-022-00436-3 · Cited by 71 · see citing works
Self-citationSilicon: A valuable soil element for improving plant growth and CO2 sequestration
Khan, A. L. (2024) · Journal of Advanced Research · doi:10.1016/j.jare.2024.05.027 · Cited by 71 · see citing works
“The weathering of silicates is thus an important sink for atmospheric CO 2 on geological timescales and significantly influences the global climate [157].”
Xu, T., Yuan, Z., Vicca, S., Goll, D. S., Li, G., Lin, L., Chen, H., Bi, B., Chen, Q., Li, C., et al. (2024) · Global Change Biology · doi:10.1111/gcb.17464 · Cited by 70 · see citing works
“In conclusion, our study provides field-experimental evidence that ERW with wollastonite powder increases SOC accumulation of ERW effects on SOC (Beerling et al., 2020; Goll et al., 2021).”
Self-citationReershemius, T., Kelland, M., Jordan, J. S., Davis, I., D’Ascanio, R., Kalderon-Asael, B., Asael, D., Suhrhoff, T. J., Epihov, D. Z., Beerling, D. J., et al. (2023) · Environmental Science & Technology · doi:10.1021/acs.est.3c03609 · Cited by 69 · see citing works
Self-citationA review of measurement for quantification of carbon dioxide removal by enhanced weathering in soil
Clarkson, M. O., Larkin, C. S., Swoboda, P., Reershemius, T., Suhrhoff, T. J., Maesano, C. N., & Campbell, J. S. (2024) · Frontiers in Climate · doi:10.3389/fclim.2024.1345224 · Cited by 77 · see citing works
“86 87 Based on generalist model predictions, EW has a global CDR potential in the range of 0.5–4 Gt CO 2 per year (Fuss et al., 2018; Beerling et al., 2020; IPCC, 2022), which can be optimized through the choice of feedstock and weathering environment (Beerling et al., 2020; Cipolla et al., 2021,…”
BackgroundInfluentialHe, H., Wang, Y., Liu, Z., Bao, Q., Wei, Y., Chen, C., & Sun, H. (2022) · Water Research · doi:10.1016/j.watres.2022.118907 · Cited by 68 · see citing works
Soil core study indicates limited CO2 removal by enhanced weathering in dry croplands in the UK
Buckingham, F., Henderson, G. M., Holdship, P., & Renforth, P. (2022) · Applied Geochemistry · doi:10.1016/j.apgeochem.2022.105482 · Cited by 66 · see citing works
Self-citationA scalable framework for quantifying field-level agricultural carbon outcomes
Guan, K., Jin, Z., Peng, B., Tang, J., DeLucia, E. H., West, P. C., Jiang, C., Wang, S., Kim, T., Zhou, W. M., et al. (2023) · Earth-Science Reviews · doi:10.1016/j.earscirev.2023.104462 · Cited by 69 · see citing works
“…to: no-till, cover cropping, precision nitrogen (N) fertilizer management, biochar and compost application, enhanced mineral weathering, new crop rotations, agro-forestry, controlled drainage and some edge-of-field practices (Beerling et al., 2020; Fargione et al., 2018; Paustian et al., 2016).”
BackgroundSelf-citationBiogeochemical constraints on climate change mitigation through regenerative farming
Schlesinger, W. H. (2022) · Biogeochemistry · doi:10.1007/s10533-022-00942-8 · Cited by 63 · see citing works
“It is attractive to suggest that the application of finely ground silicate minerals to croplands would increase the rate of this reaction, providing a sink for atmospheric CO2 that is not tied to changes in soil organic carbon (Beerling et al. 2020).”
BackgroundRiver chemistry constraints on the carbon capture potential of surficial enhanced rock weathering
Zhang, S., Planavsky, N. J., Katchinoff, J. A. R., Raymond, P. A., Kanzaki, Y., Reershemius, T., & Reinhard, C. T. (2022) · Limnology and Oceanography · doi:10.1002/lno.12244 · Cited by 68 · see citing works
“The global riverine CTP estimates for fl ood basalt application surpass recent estimates of CDR via ERW in agricultural settings (Stre fl er et al. 2018; Beerling et al. 2020), even when our model is run at relatively low saturation state thresholds.”
BackgroundResultInfluentialTransforming US agriculture for carbon removal with enhanced weathering
Beerling, D. J., Kantzas, E. P., Lomas, M. R., Taylor, L. L., Zhang, S., Kanzaki, Y., Eufrasio, R. M., Renforth, P., Mercure, J.-F., Pollitt, H., et al. (2025) · Nature · doi:10.1038/s41586-024-08429-2 · Cited by 62 · see citing works
“EW releases crop nutrients phosphorus (P) and potassium (K), as basaltic minerals undergo dissolution, with the potential to reduce the requirement for supplemental P and K amendment.”
InfluentialSelf-citationA comprehensive review of efficient capacity estimation for large-scale CO2 geological storage
Leng, J., Bump, A. P., Hosseini, S. A., Meckel, T. A., Wang, Z. W., & Wang, H. (2024) · Gas Science and Engineering · doi:10.1016/j.jgsce.2024.205339 · Cited by 61 · see citing works
Enhanced weathering potentials—the role of in situ CO2 and grain size distribution
Amann, T., Hartmann, J., Hellmann, R., Pedrosa, E. T., & Malik, A. (2022) · Frontiers in Climate · doi:10.3389/fclim.2022.929268 · Cited by 63 · see citing works
Fakhraee, M., Li, Z., Planavsky, N. J., & Reinhard, C. T. (2023) · Environmental Research Letters · doi:10.1088/1748-9326/acc9d4 · Cited by 79 · see citing works
“Our default model builds from recent work on enhanced silicate weathering in agricultural systems and other terrestrial settings [32, 33], employing a particle size distribution (PSD) rather than a single feedstock particle size.”
BackgroundLal, A., & You, F. (2023) · Science Advances · doi:10.1126/sciadv.adg6740 · Cited by 59 · see citing works
Hutchins, D. A., Fu, F., Yang, S., John, S. G., Romaniello, S. J., Andrews, M. G., & Walworth, N. G. (2023) · Biogeosciences · doi:10.5194/bg-20-4669-2023 · Cited by 59 · see citing works
Self-citationFeng, X., Dai, G., Liu, T., Jia, J., Zhu, E., Liu, C., Zhao, Y., Wang, Y., Kang, E., Xiao, J., et al. (2024) · Science China Earth Sciences · doi:10.1007/s11430-024-1359-9 · Cited by 58 · see citing works
Can arbuscular mycorrhizal fungi speed up carbon sequestration by enhanced weathering?
Verbruggen, E., Struyf, E., & Vicca, S. (2021) · Plants People Planet · doi:10.1002/ppp3.10179 · Cited by 58 · see citing works
“The global carbon sequestration potential of EW has been estimated at 0.5–5 Gt CO2 per year in a synthesis study (Fuss et al., 2018) and at 0.5–2 Gt CO2 per year in a recent nation-by-nation quantitative analysis, including various costs involved (Beerling et al., 2020).”
BackgroundInfluentialThe environmental controls on efficiency of enhanced rock weathering in soils
Deng, H., Sonnenthal, E., Arora, B., Breunig, H. M., Brodie, E., Kleber, M., Spycher, N. F., & Nico, P. (2023) · Scientific Reports · doi:10.1038/s41598-023-36113-4 · Cited by 59 · see citing works
Pang, Z., Peng, H., Lin, S., & Liang, Y. (2023) · Critical Reviews in Environmental Science and Technology · doi:10.1080/10643389.2023.2267939 · Cited by 58 · see citing works
“Similar methods are proposed to sequester carbon by applying silicate powder in farmland (Beerling et al., 2020).”
MethodRecycling of ferrous slag in agriculture: Potentials and challenges
Das, S., Galgo, S. J. C., Alam, M. A., Lee, J. G., Hwang, H. Y., Lee, C., & Kim, P. J. (2020) · Critical Reviews in Environmental Science and Technology · doi:10.1080/10643389.2020.1853458 · Cited by 57 · see citing works
Vulnerability and driving factors of soil inorganic carbon stocks in Chinese croplands
Tao, J., Raza, S., Zhao, M., Cui, J., Wang, P., Sui, Y., Zamanian, K., Kuzyakov, Y. V., Xu, M., Chen, Z., et al. (2022) · The Science of The Total Environment · doi:10.1016/j.scitotenv.2022.154087 · Cited by 59 · see citing works
Microalgal Carbon Dioxide (CO2) Capture and Utilization from the European Union Perspective
Zieliński, M., Dębowski, M., Kazimierowicz, J., & Świca, I. (2023) · Energies · doi:10.3390/en16031446 · Cited by 56 · see citing works
The Carbon-Capture Efficiency of Natural Water Alkalinization: Implications For Enhanced weathering
Bertagni, M. B., & Porporato, A. M. (2022) · The Science of The Total Environment · doi:10.1016/j.scitotenv.2022.156524 · Cited by 56 · see citing works
Spence, E., Cox, E., & Pidgeon, N. (2021) · Climatic Change · doi:10.1007/s10584-021-03050-y · Cited by 55 · see citing works
Self-citationRate and capacity of cation release from ultramafic mine tailings for carbon capture and storage
Lu, X., Carroll, K., Turvey, C., & Dipple, G. M. (2022) · Applied Geochemistry · doi:10.1016/j.apgeochem.2022.105285 · Cited by 55 · see citing works
Sustainable scale-up of negative emissions technologies and practices: where to focus
Cobo, S., Negri, V., Valente, A., Reiner, D. M., Hamelin, L., Dowell, N. M., & Guillén‐Gosálbez, G. (2022) · Environmental Research Letters · doi:10.1088/1748-9326/acacb3 · Cited by 56 · see citing works
Satterfield, T. A., Nawaz, S., & St‐Laurent, G. P. (2023) · Climatic Change · doi:10.1007/s10584-023-03483-7 · Cited by 55 · see citing works
Zhu, E., Liu, Z., Ma, L., Luo, J., Kang, E., Wang, Y., Zhao, Y., Jia, J., & Feng, X. (2024) · Geophysical Research Letters · doi:10.1029/2024gl108466 · Cited by 56 · see citing works
The effects of sealing on urban soil carbon and nutrients
O’Riordan, R., Davies, J. A. C., Stevens, C. J., & Quinton, J. N. (2021) · SOIL · doi:10.5194/soil-7-661-2021 · Cited by 53 · see citing works
Buss, W., Hasemer, H., Sokol, N. W., Rohling, E. J., & Borevitz, J. (2024) · Communications Earth & Environment · doi:10.1038/s43247-024-01771-3 · Cited by 53 · see citing works
“In practice, this CDR method involves the crushing of Ca-and Mg-rich silicate rocks, followed by their application in an environment suitableforweathering,suchasagriculturalsoils,oceans,ormorecontrolled closedpitsorreactors 15 .”
InfluentialKinetics-informed global assessment of mine tailings for CO2 removal
Bullock, L. A., Yang, A., & Darton, R. C. (2021) · The Science of The Total Environment · doi:10.1016/j.scitotenv.2021.152111 · Cited by 52 · see citing works
Skov, K., Wardman, J., Healey, M., McBride, A. L., Bierowiec, T., Cooper, J. M., Edeh, I. G., George, D., Kelland, M., Mann, J. I., et al. (2024) · PLoS ONE · doi:10.1371/journal.pone.0295031 · Cited by 51 · see citing works
Self-citationBi, B., Li, G., Goll, D. S., Lin, L., Chen, H., Xu, T., Chen, Q., Li, C., Wang, X., Hao, Z., et al. (2024) · Global Change Biology · doi:10.1111/gcb.17310 · Cited by 50 · see citing works
New insights into Mn2+ and Mg2+ inhibition of calcite growth
Mills, J. V., Barnhart, H. A., DePaolo, D. J., & Lammers, L. N. (2022) · Geochimica et Cosmochimica Acta · doi:10.1016/j.gca.2022.06.015 · Cited by 48 · see citing works
Khalidy, R., Arnaud, E., & Santos, R. M. (2022) · Land · doi:10.3390/land11091448 · Cited by 48 · see citing works
Yan, Y., Dong, X., Li, R., Zhang, Y., Yan, S., Guan, X., Yang, Q., Chen, L., Fang, Y., Zhang, W., et al. (2023) · CATENA · doi:10.1016/j.catena.2023.107031 · Cited by 48 · see citing works
Levy, C. R., Almaraz, M., Beerling, D. J., Raymond, P. A., Reinhard, C. T., Suhrhoff, T. J., & Taylor, L. L. (2024) · Environmental Science & Technology · doi:10.1021/acs.est.4c02368 · Cited by 48 · see citing works
Self-citationInorganic Carbon Pools and Their Drivers in Grassland and Desert Soils
Dong, L., Ran, J., Luo, J., Bai, L., Sun, Y., Aqeel, M. A., Zhang, Y., Wang, X., Du, Q., Xiong, J., et al. (2024) · Global Change Biology · doi:10.1111/gcb.17536 · Cited by 48 · see citing works
Development of sorbent materials for direct air capture of CO2
Shi, X., Lin, Y., & Chen, X. (2022) · MRS Bulletin · doi:10.1557/s43577-022-00320-7 · Cited by 47 · see citing works
Fingerprinting hydrological and biogeochemical drivers of freshwater quality
Heathwaite, A. L., & Bieroza, M. (2020) · Hydrological Processes · doi:10.1002/hyp.13973 · Cited by 46 · see citing works
“…of solute in the catchment, for example, agricultural land use for nutrients (Banwart, 2011; Heathwaite, 2010) and bedrock for weathering solutes (Beerling et al., 2020), creates an internal loading that reduces the diversity in the stream c-q responses and increases the frequency of chemostatic…”
BackgroundRates of atmospheric CO2 capture using magnesium oxide powder
Rausis, K., Stubbs, A. R., Power, I., & Paulo, C. (2022) · International journal of greenhouse gas control · doi:10.1016/j.ijggc.2022.103701 · Cited by 45 · see citing works
Zhang, T., Hu, C., Wu, J., Shen, B., Peng, S., Qi, Y., Tao, M., Mao, X., Tao, Y., & Wang, Y. (2023) · Separation and Purification Technology · doi:10.1016/j.seppur.2023.124352 · Cited by 44 · see citing works
Impact of Climate on the Global Capacity for Enhanced Rock Weathering on Croplands
Baek, S. H., Kanzaki, Y., Lora, J. M., Planavsky, N. J., Reinhard, C. T., & Zhang, S. (2023) · Earth s Future · doi:10.1029/2023ef003698 · Cited by 42 · see citing works
“Estimates of carbon capture from ERW on global croplands nevertheless remain sparse, with only one existing study to our knowledge (Beerling et al., 2020).”
BackgroundMethodResultInfluentialHolden, F., Davies, K., Bird, M. I., Hume, R., Green, H., Beerling, D. J., & Nelson, P. N. (2024) · The Science of The Total Environment · doi:10.1016/j.scitotenv.2024.176568 · Cited by 51 · see citing works
Self-citationDirect measurement of fungal contribution to silicate weathering rates in soil
Wild, B., Imfeld, G., & Daval, D. (2021) · Geology · doi:10.1130/g48706.1 · Cited by 42 · see citing works
- Authors
- Beerling, D. J., Kantzas, E. P., Lomas, M. R., Wade, P., Eufrasio, R. M., Renforth, P., Sarkar, B., Andrews, M. G., James, R. H., Pearce, C. R., Mercure, J.-F., Pollitt, H., Holden, P. B., Edwards, N. R., Khanna, M., Koh, L., Quegan, S., Pidgeon, N. F., Janssens, I. A., Hansen, J., & Banwart, S. A.
- Affiliations
- Leverhulme Centre for Climate Change Mitigation (GB)
- University of Sheffield (GB)
- Heriot-Watt University (GB)
- Lancaster University (GB)
- National Oceanography Centre (GB)
- University of Cambridge (GB)
- The Open University (GB)
- University of Illinois Urbana-Champaign (US)
- Cardiff University (GB)
- University of Antwerp (BE)
- Columbia University (US)
- University of Leeds (GB)
- Corresponding author
- Beerling, David J.
- ORCID
- Beerling, David J.
- Kantzas, Euripides P.
- Wade, Peter
- Eufrasio, Rafael M.
- Renforth, Phil
- Sarkar, Binoy
- Andrews, M. Grace
- James, Rachael H.
- Pearce, Christopher R.
- Mercure, Jean-Francois
- Pollitt, Hector
- Holden, Philip B.
- Edwards, Neil R.
- Khanna, Madhu
- Koh, Lenny
- Quegan, Shaun
- Pidgeon, Nick F.
- Janssens, Ivan A.
- Hansen, James
- Banwart, Steven A.
- Venue
- Nature
- Published
- 2020-07-08
- Volume
- 583
- Issue
- 7815
- Pages
- 242-248
- ISSN
- 0028-0836 (ISSN-L)
- 1476-4687
- OpenAlex
- W3041773269
- Semantic Scholar
- 9c00c1ebacb3a72cae19f74c126391c7eb38ebc1
- Cited by
- 700
- References
- 78
- Citations by year
- 2026: 137 · 2025: 144 · 2024: 144 · 2023: 100 · 2022: 94 · 2021: 71 · 2020: 10
- FWCI
- 24.79
- Type
- journal article
- Language
- en
- Open access
- green
- eprints.lancs.ac.uk
- Licence
- Locations
- Nature (publishedVersion)
- PubMed (publishedVersion)
- Lancaster EPrints (Lancaster University) (acceptedVersion)
- ePrints Soton (University of Southampton) (acceptedVersion)
- White Rose Research Online (University of Leeds, The University of Sheffield, University of York) (acceptedVersion)
- NERC Open Research Archive (Natural Environment Research Council) (acceptedVersion)
- Open Research Online - ORO (The Open University) (acceptedVersion)
- Open Research Exeter (University of Exeter) (acceptedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- Adelaide Research & Scholarship (AR&S) (University of Adelaide) (submittedVersion)
- Figshare (submittedVersion)
- ORCA Online Research @Cardiff (Cardiff University) (submittedVersion)
- Funders
- U.S. Department of Energy
- UK Research and Innovation
- Leverhulme Trust (RC-2015-029)
- Royal Academy of Engineering
- Universiteit Antwerpen
- Engineering and Physical Sciences Research Council (EP/K007254/1)
- Natural Environment Research Council (noc010011, NE/P015093/1, NE/P019943/2, NE/S017119/1, NE/P019730/2, NE/P019943/1)
- Topics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Physical Sciences › Environmental Science › Global and Planetary Change › Climate Change and Geoengineering
- Keywords
- carbon dioxide removal, cropland, techno-economic analysis, climate change mitigation, 2°C target, energy policy scenarios
- MeSH terms
- Agriculture, Atmosphere, Brazil, Carbon Dioxide, China, Goals, India, Iron, Mining, Politics, Probability, Steel, Temperature, Time Factors, United States, Silicates, Crops, Agricultural, Geologic Sediments, Global Warming, Environmental Policy
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